Two-Phase Change in Thickness and Viscoelasticity of Polyelectrolyte\n Multilayers Swollen with Ionic Liquid Solution Article Swipe
Nagma Parveen
,
Pritam Kumar Jana
,
Monika Schoenhoff
·
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.1811.07226
YOU?
·
· 2018
· Open Access
·
· DOI: https://doi.org/10.48550/arxiv.1811.07226
Polyelectrolyte multilayers (PEM) in combination with good electrolyte\nsolvents, e.g., ionic liquids (ILs) are potential candidates for the new\ngeneration of electrochemical separators. Swelling PEM with aqueous IL\nsolutions is one way to incorporate IL in PEM. In addition to quantifying the\nIL uptake in PEM, physical characterization of the swollen PEM is essential for\ntheir potential applications and to uncover the underlying molecular process of\nthe swelling. In this article, thickness and viscoelasticity of\nPEI(PSS/PADMAC)4PSS and PEI(PSS/PAH)4PSS multilayers were determined upon\nuptake of aqueous solutions of 1-Ethyl-3methylimidazolium chloride, a\nwater-soluble IL. This was done by employing the Kelvin-Voigt model in\ncombination with the frequency and dissipation shifts measured using quartz\ncrystal microbalance with dissipation technique. The modeled thickness and\nviscoelasticity of the multilayers change in two phases with increasing IL\nconcentration. In the first phase, a small increase in PEM thickness\naccompanies a two to three-fold increase in PEM viscoelasticity, whereas the\nchanges are other ways around in the second phase. Two phenomenon contributes\nto the two-phase changes: 1) the exchange between hydrated ions of IL and\nin-situ water of PEM influencing the overall ion and water content in PEM and\n2) the hydrophobic and electrostatic interactions between incorporated IL and\nPEM influencing the structural integrity of PEM.\n
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- Type
- preprint
- Language
- en
- Landing Page
- http://arxiv.org/abs/1811.07226
- https://arxiv.org/pdf/1811.07226
- OA Status
- green
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4289285766
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4289285766Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.48550/arxiv.1811.07226Digital Object Identifier
- Title
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Two-Phase Change in Thickness and Viscoelasticity of Polyelectrolyte\n Multilayers Swollen with Ionic Liquid SolutionWork title
- Type
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preprintOpenAlex work type
- Language
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enPrimary language
- Publication year
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2018Year of publication
- Publication date
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2018-11-17Full publication date if available
- Authors
-
Nagma Parveen, Pritam Kumar Jana, Monika SchoenhoffList of authors in order
- Landing page
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https://arxiv.org/abs/1811.07226Publisher landing page
- PDF URL
-
https://arxiv.org/pdf/1811.07226Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://arxiv.org/pdf/1811.07226Direct OA link when available
- Concepts
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Quartz crystal microbalance, Polyelectrolyte, Viscoelasticity, Swelling, Ionic liquid, Electrolyte, Aqueous solution, Chemical engineering, Phase (matter), Materials science, Chemistry, Composite material, Polymer, Physical chemistry, Organic chemistry, Adsorption, Electrode, Engineering, CatalysisTop concepts (fields/topics) attached by OpenAlex
- Cited by
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.combination | 4 |
| abstract_inverted_index.dissipation | 96, 103 |
| abstract_inverted_index.hydrophobic | 176 |
| abstract_inverted_index.incorporate | 30 |
| abstract_inverted_index.influencing | 165, 184 |
| abstract_inverted_index.multilayers | 1, 71, 111 |
| abstract_inverted_index.quantifying | 37 |
| abstract_inverted_index.separators. | 20 |
| abstract_inverted_index.Kelvin-Voigt | 89 |
| abstract_inverted_index.and\nin-situ | 161 |
| abstract_inverted_index.applications | 52 |
| abstract_inverted_index.incorporated | 181 |
| abstract_inverted_index.interactions | 179 |
| abstract_inverted_index.microbalance | 101 |
| abstract_inverted_index.the\nchanges | 138 |
| abstract_inverted_index.upon\nuptake | 74 |
| abstract_inverted_index.IL\nsolutions | 25 |
| abstract_inverted_index.electrostatic | 178 |
| abstract_inverted_index.Polyelectrolyte | 0 |
| abstract_inverted_index.contributes\nto | 149 |
| abstract_inverted_index.electrochemical | 19 |
| abstract_inverted_index.in\ncombination | 91 |
| abstract_inverted_index.new\ngeneration | 17 |
| abstract_inverted_index.quartz\ncrystal | 100 |
| abstract_inverted_index.viscoelasticity | 67 |
| abstract_inverted_index.PEI(PSS/PAH)4PSS | 70 |
| abstract_inverted_index.a\nwater-soluble | 81 |
| abstract_inverted_index.characterization | 43 |
| abstract_inverted_index.viscoelasticity, | 136 |
| abstract_inverted_index.IL\nconcentration. | 118 |
| abstract_inverted_index.and\nviscoelasticity | 108 |
| abstract_inverted_index.electrolyte\nsolvents, | 7 |
| abstract_inverted_index.thickness\naccompanies | 128 |
| abstract_inverted_index.of\nPEI(PSS/PADMAC)4PSS | 68 |
| abstract_inverted_index.1-Ethyl-3methylimidazolium | 79 |
| cited_by_percentile_year | |
| countries_distinct_count | 0 |
| institutions_distinct_count | 3 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/6 |
| sustainable_development_goals[0].score | 0.8199999928474426 |
| sustainable_development_goals[0].display_name | Clean water and sanitation |
| citation_normalized_percentile.value | 0.29405777 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |