Two-photon double ionization with finite pulses: Application of the virtual sequential model to helium Article Swipe
S. Chattopadhyay
,
Carlos Marante
,
Barry I. Schneider
,
Luca Argenti
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1103/physreva.108.013114
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1103/physreva.108.013114
As a step toward the full ab initio description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the ab initio description of the single ionization scattering states of both the neutral and ionized target system. As a proof of principle and a benchmark, the model is applied to the helium atom using the newstock atomic photoionization code. The results of angularly integrated observables, which are in excellent agreement with existing time-dependent Schrödinger equation (TDSE) simulations, show how the model is able to capture the role of electron correlation in the nonsequential regime, and the influence of autoionizing states in the sequential regime, at a comparatively modest computational cost. The model also reproduces the two-particle interference with ultrashort pulses, which is within reach of current experimental technologies. Furthermore, the model shows the modulation of the joint energy distribution in the vicinity of autoionizing states, which can be probed with extreme-ultraviolet pulses of duration much longer than the characteristic lifetime of the resonance. Furthermore, the formalism discussed here applies also to polyelectronic atoms and molecules, thus opening a window on nonsequential and sequential double ionization in these more complex systems.
Related Topics
Concepts
Atomic physics
Photoionization
Ionization
Physics
Double ionization
Ab initio
Helium
Helium atom
Photon
Electron
Quantum mechanics
Ion
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1103/physreva.108.013114
- OA Status
- green
- Cited By
- 6
- References
- 52
- Related Works
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- OpenAlex ID
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All OpenAlex metadata
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https://openalex.org/W4384934499Canonical identifier for this work in OpenAlex
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https://doi.org/10.1103/physreva.108.013114Digital Object Identifier
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Two-photon double ionization with finite pulses: Application of the virtual sequential model to heliumWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2023Year of publication
- Publication date
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2023-07-20Full publication date if available
- Authors
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S. Chattopadhyay, Carlos Marante, Barry I. Schneider, Luca ArgentiList of authors in order
- Landing page
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https://doi.org/10.1103/physreva.108.013114Publisher landing page
- Open access
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YesWhether a free full text is available
- OA status
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greenOpen access status per OpenAlex
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https://www.osti.gov/biblio/1991274Direct OA link when available
- Concepts
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Atomic physics, Photoionization, Ionization, Physics, Double ionization, Ab initio, Helium, Helium atom, Photon, Electron, Quantum mechanics, IonTop concepts (fields/topics) attached by OpenAlex
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6Total citation count in OpenAlex
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2025: 3, 2024: 3Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W4245312620, https://openalex.org/W4211101250, https://openalex.org/W2561223232, https://openalex.org/W2991077692, https://openalex.org/W2995159779, https://openalex.org/W4221137116, https://openalex.org/W2132577564, https://openalex.org/W2097421518, https://openalex.org/W2043021112, https://openalex.org/W2006246239, https://openalex.org/W1972200722, https://openalex.org/W2091169571, https://openalex.org/W1621473306, https://openalex.org/W2024930129, https://openalex.org/W2020820782, https://openalex.org/W1985139192, https://openalex.org/W2075463149, https://openalex.org/W2035868004, https://openalex.org/W1894623165, https://openalex.org/W2152406212, https://openalex.org/W2023052957, https://openalex.org/W2057218928, https://openalex.org/W2443127368, https://openalex.org/W1556692390, https://openalex.org/W2073719624, https://openalex.org/W2093181719, https://openalex.org/W1995719458, https://openalex.org/W1971718622, https://openalex.org/W2078288421, https://openalex.org/W2030960272, https://openalex.org/W2557597438, https://openalex.org/W2769039341, https://openalex.org/W2757707227, https://openalex.org/W2901868145, https://openalex.org/W3003515723, https://openalex.org/W2000871067, https://openalex.org/W2114267968, https://openalex.org/W2262352627, https://openalex.org/W4213223317, https://openalex.org/W4238772618, https://openalex.org/W2750585098, https://openalex.org/W1986840969, https://openalex.org/W2046021365, https://openalex.org/W2075950706, https://openalex.org/W2077663506, https://openalex.org/W2039881386, https://openalex.org/W2069096237, https://openalex.org/W2089169191, https://openalex.org/W2049939570, https://openalex.org/W2052979335, https://openalex.org/W4242131536, https://openalex.org/W3101525718 |
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| sustainable_development_goals[0].display_name | Affordable and clean energy |
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