Ultrafast pump-probe phase-randomized tomography Article Swipe
Filippo Glerean
,
Enrico Maria Rigoni
,
Giacomo Jarc
,
Shahla Yasmin Mathengattil
,
Angela Montanaro
,
Francesca Giusti
,
Matteo Mitrano
,
Fabio Benatti
,
Daniele Fausti
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41377-025-01789-y
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1038/s41377-025-01789-y
Measuring fluctuations in matter’s low-energy excitations is the key to unveiling the nature of the non-equilibrium response of materials. A promising outlook in this respect is offered by spectroscopic methods that address matter fluctuations by exploiting the statistical nature of light-matter interactions with weak few-photon probes. Here we report the first implementation of ultrafast phase randomized tomography, combining pump-probe experiments with quantum optical state tomography, to measure the ultrafast non-equilibrium dynamics in complex materials. Our approach utilizes a time-resolved multimode heterodyne detection scheme with phase-randomized coherent ultrashort laser pulses, overcoming the limitations of phase-stable configurations and enabling a robust reconstruction of the statistical distribution of phase-averaged optical observables. This methodology is validated by measuring the coherent phonon response in α-quartz. By tracking the dynamics of the shot-noise limited photon number distribution of few-photon probes with ultrafast resolution, our results set an upper limit to the non-classical features of phononic state in α-quartz and provide a pathway to access non-equilibrium quantum fluctuations in more complex quantum materials.
Related Topics
Concepts
Ultrashort pulse
Physics
Photon
Quantum tomography
Quantum optics
Optics
Phase (matter)
Quantum
Laser
Quantum state
Quantum mechanics
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41377-025-01789-y
- https://www.nature.com/articles/s41377-025-01789-y.pdf
- OA Status
- gold
- Cited By
- 4
- References
- 61
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4408209924
All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4408209924Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1038/s41377-025-01789-yDigital Object Identifier
- Title
-
Ultrafast pump-probe phase-randomized tomographyWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-03-06Full publication date if available
- Authors
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Filippo Glerean, Enrico Maria Rigoni, Giacomo Jarc, Shahla Yasmin Mathengattil, Angela Montanaro, Francesca Giusti, Matteo Mitrano, Fabio Benatti, Daniele FaustiList of authors in order
- Landing page
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https://doi.org/10.1038/s41377-025-01789-yPublisher landing page
- PDF URL
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https://www.nature.com/articles/s41377-025-01789-y.pdfDirect link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://www.nature.com/articles/s41377-025-01789-y.pdfDirect OA link when available
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Ultrashort pulse, Physics, Photon, Quantum tomography, Quantum optics, Optics, Phase (matter), Quantum, Laser, Quantum state, Quantum mechanicsTop concepts (fields/topics) attached by OpenAlex
- Cited by
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4Total citation count in OpenAlex
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2025: 4Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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