Understanding and Engineering Interfacial Adhesion in Solid‐State Batteries with Metallic Anodes Article Swipe
Ieuan D. Seymour
,
Edouard Quérel
,
Rowena H. Brugge
,
Federico M. Pesci
,
Ainara Aguadero
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/cssc.202202215
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1002/cssc.202202215
High performance alkali metal anode solid‐state batteries require solid/solid interfaces with fast ion transfer that are morphologically and chemically stable upon electrochemical cycling. Void formation at the alkali metal/solid‐state electrolyte interface during alkali metal stripping is responsible for constriction resistances and hotspots that can facilitate dendrite propagation and failure. Both externally applied pressures (35–400 MPa) and temperatures above the melting point of the alkali metal have been shown to improve the interfacial contact with the solid electrolyte, preventing the formation of voids. However, the extreme pressure and temperature conditions required can be difficult to meet for commercial solid‐state battery applications. In this review, we highlight the importance of interfacial adhesion or ‘wetting’ at alkali metal/solid electrolyte interfaces for achieving solid‐state batteries that can withstand high current densities without cell failure. The intrinsically poor adhesion at metal/ceramic interfaces poses fundamental limitations on many inorganics solid‐state electrolyte systems in the absence of applied pressure. Suppression of alkali metal voids can only be achieved for systems with high interfacial adhesion (i. e. ‘perfect wetting’) where the contact angle between the alkali metal and the solid‐state electrolyte surface goes to θ =0°. We identify key strategies to improve interfacial adhesion and suppress void formation including the adoption of interlayers, alloy anodes and 3D scaffolds. Computational modeling techniques have been invaluable for understanding the structure, stability and adhesion of solid‐state battery interfaces and we provide an overview of key techniques. Although focused on alkali metal solid‐state batteries, the fundamental understanding of interfacial adhesion discussed in this review has broader applications across the field of chemistry and material science from corrosion to biomaterials development.
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Metadata
- Type
- review
- Language
- en
- Landing Page
- https://doi.org/10.1002/cssc.202202215
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cssc.202202215
- OA Status
- hybrid
- Cited By
- 26
- References
- 306
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4323652807
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4323652807Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/cssc.202202215Digital Object Identifier
- Title
-
Understanding and Engineering Interfacial Adhesion in Solid‐State Batteries with Metallic AnodesWork title
- Type
-
reviewOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-03-09Full publication date if available
- Authors
-
Ieuan D. Seymour, Edouard Quérel, Rowena H. Brugge, Federico M. Pesci, Ainara AguaderoList of authors in order
- Landing page
-
https://doi.org/10.1002/cssc.202202215Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cssc.202202215Direct link to full text PDF
- Open access
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YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/cssc.202202215Direct OA link when available
- Concepts
-
Materials science, Anode, Electrolyte, Wetting, Alkali metal, Fast ion conductor, Ceramic, Adhesion, Nanotechnology, Alloy, Chemical engineering, Composite material, Electrode, Chemistry, Organic chemistry, Physical chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
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26Total citation count in OpenAlex
- Citations by year (recent)
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2025: 12, 2024: 7, 2023: 7Per-year citation counts (last 5 years)
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306Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.batteries | 7, 121 |
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| abstract_inverted_index.batteries, | 242 |
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| abstract_inverted_index.strategies | 192 |
| abstract_inverted_index.structure, | 220 |
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| abstract_inverted_index.morphologically | 17 |
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| cited_by_percentile_year.min | 98 |
| corresponding_author_ids | https://openalex.org/A5071720185, https://openalex.org/A5004733589 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 5 |
| corresponding_institution_ids | https://openalex.org/I4210118429, https://openalex.org/I47508984 |
| citation_normalized_percentile.value | 0.94382124 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |