Understanding Optical Properties and Electronic Structures of High‐Entropy Alloyed Perovskite Nanocrystals Article Swipe
Y. Chiang
,
Sunil B. Shivarudraiah
,
Alexander Wieczorek
,
Khoong Hong Khoo
,
Zhidong Leong
,
Jia Wei Melvin Lim
,
Zengshan Xing
,
Sudhir Kumar
,
Simon F. Solari
,
Yen‐Ting Li
,
Yu‐Cheng Chiu
,
Tze Chien Sum
,
Yun Liu
,
Sebastian Siol
,
Chih‐Jen Shih
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202505890
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/ange.202505890
High‐entropy alloying (HEA) has emerged as a prominent strategy to modulate physiochemical properties of nanomaterials. Nevertheless, this approach is underexplored in luminescent semiconductor nanocrystals (NCs) due to the lack of understanding into the HEA‐induced electronic effect and photophysical behaviors. Herein, harnessing the defect tolerance of metal halide perovskite NCs, we systematically synthesized and characterized high‐entropy halide perovskite (HEP) NCs containing multiple B‐site elements (Pb 2+ , Sr 2 ⁺, Ca 2 ⁺, Cd 2 ⁺, and Mg 2 ⁺). High‐resolution transmission electron microscopy, transient photoluminescence and absorption spectroscopy, X‐ray photoemission spectroscopy, and density functional theory simulations are employed to unravel the evolution of electronic structures with respect to the alloying degree and link them to the spectral signatures and photostability. Counterintuitively, although the HEP NCs exhibit lateral sizes smaller than the Bohr diameter of CsPbBr 3 NCs (∼7 nm), HEA reduces the band dispersion and broadens the conduction band, thereby vanishing the excitonic feature by forming near band‐edge shallow states. We show that these HEA‐induced shallow states foster rapid radiative recombination and improve photostability, accompanied by a significantly reduced lead content by up to 70%. These findings pioneer the understanding of the correlation between HEA‐induced electronic effect and photophysical properties, highlighting the versatility of HEA for band structure engineering and stabilization of metal halide perovskites NCs.
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- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/ange.202505890
- OA Status
- hybrid
- References
- 97
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4412922578
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https://openalex.org/W4412922578Canonical identifier for this work in OpenAlex
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https://doi.org/10.1002/ange.202505890Digital Object Identifier
- Title
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Understanding Optical Properties and Electronic Structures of High‐Entropy Alloyed Perovskite NanocrystalsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2025Year of publication
- Publication date
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2025-07-24Full publication date if available
- Authors
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Y. Chiang, Sunil B. Shivarudraiah, Alexander Wieczorek, Khoong Hong Khoo, Zhidong Leong, Jia Wei Melvin Lim, Zengshan Xing, Sudhir Kumar, Simon F. Solari, Yen‐Ting Li, Yu‐Cheng Chiu, Tze Chien Sum, Yun Liu, Sebastian Siol, Chih‐Jen ShihList of authors in order
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https://doi.org/10.1002/ange.202505890Publisher landing page
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YesWhether a free full text is available
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hybridOpen access status per OpenAlex
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https://doi.org/10.1002/ange.202505890Direct OA link when available
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Nanocrystal, Perovskite (structure), Materials science, Electronic structure, Nanotechnology, Crystallography, Chemistry, Computational chemistryTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.to | 10, 27, 99, 108, 115, 184 |
| abstract_inverted_index.up | 183 |
| abstract_inverted_index.we | 50 |
| abstract_inverted_index.(Pb | 64 |
| abstract_inverted_index.HEA | 140, 205 |
| abstract_inverted_index.HEP | 124 |
| abstract_inverted_index.NCs | 59, 125, 137 |
| abstract_inverted_index.and | 37, 53, 76, 86, 92, 112, 119, 145, 172, 198, 210 |
| abstract_inverted_index.are | 97 |
| abstract_inverted_index.due | 26 |
| abstract_inverted_index.for | 206 |
| abstract_inverted_index.has | 4 |
| abstract_inverted_index.the | 28, 33, 42, 101, 109, 116, 123, 131, 142, 147, 152, 189, 192, 202 |
| abstract_inverted_index.70%. | 185 |
| abstract_inverted_index.Bohr | 132 |
| abstract_inverted_index.NCs, | 49 |
| abstract_inverted_index.NCs. | 216 |
| abstract_inverted_index.band | 143, 207 |
| abstract_inverted_index.into | 32 |
| abstract_inverted_index.lack | 29 |
| abstract_inverted_index.lead | 180 |
| abstract_inverted_index.link | 113 |
| abstract_inverted_index.near | 157 |
| abstract_inverted_index.nm), | 139 |
| abstract_inverted_index.show | 162 |
| abstract_inverted_index.than | 130 |
| abstract_inverted_index.that | 163 |
| abstract_inverted_index.them | 114 |
| abstract_inverted_index.this | 17 |
| abstract_inverted_index.with | 106 |
| abstract_inverted_index.⁺, | 69, 72, 75 |
| abstract_inverted_index.(HEA) | 3 |
| abstract_inverted_index.(HEP) | 58 |
| abstract_inverted_index.(NCs) | 25 |
| abstract_inverted_index.(∼7 | 138 |
| abstract_inverted_index.These | 186 |
| abstract_inverted_index.band, | 149 |
| abstract_inverted_index.metal | 46, 213 |
| abstract_inverted_index.rapid | 169 |
| abstract_inverted_index.sizes | 128 |
| abstract_inverted_index.these | 164 |
| abstract_inverted_index.⁺). | 79 |
| abstract_inverted_index.CsPbBr | 135 |
| abstract_inverted_index.defect | 43 |
| abstract_inverted_index.degree | 111 |
| abstract_inverted_index.effect | 36, 197 |
| abstract_inverted_index.foster | 168 |
| abstract_inverted_index.halide | 47, 56, 214 |
| abstract_inverted_index.states | 167 |
| abstract_inverted_index.theory | 95 |
| abstract_inverted_index.Herein, | 40 |
| abstract_inverted_index.X‐ray | 89 |
| abstract_inverted_index.between | 194 |
| abstract_inverted_index.content | 181 |
| abstract_inverted_index.density | 93 |
| abstract_inverted_index.emerged | 5 |
| abstract_inverted_index.exhibit | 126 |
| abstract_inverted_index.feature | 154 |
| abstract_inverted_index.forming | 156 |
| abstract_inverted_index.improve | 173 |
| abstract_inverted_index.lateral | 127 |
| abstract_inverted_index.pioneer | 188 |
| abstract_inverted_index.reduced | 179 |
| abstract_inverted_index.reduces | 141 |
| abstract_inverted_index.respect | 107 |
| abstract_inverted_index.shallow | 159, 166 |
| abstract_inverted_index.smaller | 129 |
| abstract_inverted_index.states. | 160 |
| abstract_inverted_index.thereby | 150 |
| abstract_inverted_index.unravel | 100 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.B‐site | 62 |
| abstract_inverted_index.alloying | 2, 110 |
| abstract_inverted_index.although | 122 |
| abstract_inverted_index.approach | 18 |
| abstract_inverted_index.broadens | 146 |
| abstract_inverted_index.diameter | 133 |
| abstract_inverted_index.electron | 82 |
| abstract_inverted_index.elements | 63 |
| abstract_inverted_index.employed | 98 |
| abstract_inverted_index.findings | 187 |
| abstract_inverted_index.modulate | 11 |
| abstract_inverted_index.multiple | 61 |
| abstract_inverted_index.spectral | 117 |
| abstract_inverted_index.strategy | 9 |
| abstract_inverted_index.evolution | 102 |
| abstract_inverted_index.excitonic | 153 |
| abstract_inverted_index.prominent | 8 |
| abstract_inverted_index.radiative | 170 |
| abstract_inverted_index.structure | 208 |
| abstract_inverted_index.tolerance | 44 |
| abstract_inverted_index.transient | 84 |
| abstract_inverted_index.vanishing | 151 |
| abstract_inverted_index.absorption | 87 |
| abstract_inverted_index.behaviors. | 39 |
| abstract_inverted_index.conduction | 148 |
| abstract_inverted_index.containing | 60 |
| abstract_inverted_index.dispersion | 144 |
| abstract_inverted_index.electronic | 35, 104, 196 |
| abstract_inverted_index.functional | 94 |
| abstract_inverted_index.harnessing | 41 |
| abstract_inverted_index.perovskite | 48, 57 |
| abstract_inverted_index.properties | 13 |
| abstract_inverted_index.signatures | 118 |
| abstract_inverted_index.structures | 105 |
| abstract_inverted_index.accompanied | 175 |
| abstract_inverted_index.band‐edge | 158 |
| abstract_inverted_index.correlation | 193 |
| abstract_inverted_index.engineering | 209 |
| abstract_inverted_index.luminescent | 22 |
| abstract_inverted_index.microscopy, | 83 |
| abstract_inverted_index.perovskites | 215 |
| abstract_inverted_index.properties, | 200 |
| abstract_inverted_index.simulations | 96 |
| abstract_inverted_index.synthesized | 52 |
| abstract_inverted_index.versatility | 203 |
| abstract_inverted_index.highlighting | 201 |
| abstract_inverted_index.nanocrystals | 24 |
| abstract_inverted_index.transmission | 81 |
| abstract_inverted_index.HEA‐induced | 34, 165, 195 |
| abstract_inverted_index.Nevertheless, | 16 |
| abstract_inverted_index.characterized | 54 |
| abstract_inverted_index.photoemission | 90 |
| abstract_inverted_index.photophysical | 38, 199 |
| abstract_inverted_index.recombination | 171 |
| abstract_inverted_index.semiconductor | 23 |
| abstract_inverted_index.significantly | 178 |
| abstract_inverted_index.spectroscopy, | 88, 91 |
| abstract_inverted_index.stabilization | 211 |
| abstract_inverted_index.underexplored | 20 |
| abstract_inverted_index.understanding | 31, 190 |
| abstract_inverted_index.High‐entropy | 1 |
| abstract_inverted_index.high‐entropy | 55 |
| abstract_inverted_index.nanomaterials. | 15 |
| abstract_inverted_index.physiochemical | 12 |
| abstract_inverted_index.systematically | 51 |
| abstract_inverted_index.photostability, | 174 |
| abstract_inverted_index.photostability. | 120 |
| abstract_inverted_index.High‐resolution | 80 |
| abstract_inverted_index.photoluminescence | 85 |
| abstract_inverted_index.Counterintuitively, | 121 |
| cited_by_percentile_year | |
| corresponding_author_ids | https://openalex.org/A5084655324, https://openalex.org/A5111926744, https://openalex.org/A5001213992, https://openalex.org/A5050359948, https://openalex.org/A5100321991 |
| countries_distinct_count | 4 |
| institutions_distinct_count | 15 |
| corresponding_institution_ids | https://openalex.org/I115228651, https://openalex.org/I172675005, https://openalex.org/I3004594783, https://openalex.org/I35440088, https://openalex.org/I4210090941, https://openalex.org/I4210092485, https://openalex.org/I4210119046, https://openalex.org/I71824836 |
| citation_normalized_percentile.value | 0.3440778 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | False |