Understanding the Conductivity and Transference Trade-Off in Polymer Electrolytes Using a Robeson-Inspired Upper Bound Article Swipe
Zirong He
,
Nitash P. Balsara
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acsapm.5c00288
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1021/acsapm.5c00288
The development of high-performance electrolytes is crucial for advancing next-generation lithium and sodium battery technologies. Since the cation is the working ion in both technologies, electrolytes exhibiting the rapid cation transport are essential for making progress. Pathways to optimize electrolytes are unclear due to the inherent trade-off between conductivity and cation transference. While this trade-off is sometimes recognized, there are no well-accepted methodologies for quantifying it. Inspired by the Robeson upper bound for the permeability-selectivity trade-off in gas separation membranes, we propose an approach for quantifying the trade-off in electrolytes using Newman’s concentrated solution theory. We suggest calling this the Newman upper bound. By analyzing published data from 30 polymer electrolytes containing univalent lithium and sodium salts, the Newman upper bound is expressed as κ = 2.0(1/ρ+ - 1) where κ (mS/cm) is conductivity and ρ+ is the current fraction measured in a symmetric cell as first described by Bruce et al. [J. Electroanal. Chem. Interfacial Electrochem. 1987, 225 (1), 1-17]. This formulation of the upper bound introduces a critical guiding metric for designing next-generation polymer electrolytes; it highlights factors underlying the trade-off, including the salt diffusion coefficient (D), cation transference number relative to solvent velocity ((Formula presented)), and thermodynamic factor (1 + (d lnγ+-)/(d lnm)), where γ+- is the mean molar activity coefficient and m is the molality. These parameters have been measured for very few electrolytes. We posit that establishing the molecular properties that govern these parameters will lead to improved electrolytes that greatly exceed the current upper bound.
Related Topics
Concepts
Conductivity
Electrolyte
Polymer electrolytes
Materials science
Polymer
Composite material
Psychology
Chemistry
Ionic conductivity
Electrode
Physical chemistry
Metadata
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- article
- Language
- en
- Landing Page
- https://doi.org/10.1021/acsapm.5c00288
- OA Status
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- References
- 54
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- 10
- OpenAlex ID
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https://doi.org/10.1021/acsapm.5c00288Digital Object Identifier
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Understanding the Conductivity and Transference Trade-Off in Polymer Electrolytes Using a Robeson-Inspired Upper BoundWork title
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articleOpenAlex work type
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enPrimary language
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2025Year of publication
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2025-05-06Full publication date if available
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Zirong He, Nitash P. BalsaraList of authors in order
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https://doi.org/10.1021/acsapm.5c00288Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://escholarship.org/uc/item/3g6048rqDirect OA link when available
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Conductivity, Electrolyte, Polymer electrolytes, Materials science, Polymer, Composite material, Psychology, Chemistry, Ionic conductivity, Electrode, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
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0Total citation count in OpenAlex
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