Unlocking Li superionic conductivity in face-centred cubic oxides via face-sharing configurations Article Swipe
Yu Chen
,
Zhengyan Lun
,
Xinye Zhao
,
Krishna Prasad Koirala
,
Linze Li
,
Yingzhi Sun
,
Christopher A. O’Keefe
,
Xiaochen Yang
,
Zijian Cai
,
Chongmin Wang
,
Huiwen Ji
,
Clare P. Grey
,
Bin Ouyang
,
Gerbrand Ceder
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41563-024-01800-8
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1038/s41563-024-01800-8
Oxides with a face-centred cubic (fcc) anion sublattice are generally not considered as solid-state electrolytes as the structural framework is thought to be unfavourable for lithium (Li) superionic conduction. Here we demonstrate Li superionic conductivity in fcc-type oxides in which face-sharing Li configurations have been created through cation over-stoichiometry in rocksalt-type lattices via excess Li. We find that the face-sharing Li configurations create a novel spinel with unconventional stoichiometry and raise the energy of Li, thereby promoting fast Li-ion conduction. The over-stoichiometric Li–In–Sn–O compound exhibits a total Li superionic conductivity of 3.38 × 10 −4 S cm −1 at room temperature with a low migration barrier of 255 meV. Our work unlocks the potential of designing Li superionic conductors in a prototypical structural framework with vast chemical flexibility, providing fertile ground for discovering new solid-state electrolytes.
Related Topics
Concepts
Fast ion conductor
Stoichiometry
Materials science
Conductivity
Lithium (medication)
Ion
Electrolyte
Spinel
Ionic conductivity
Chemical physics
Thermal conduction
Condensed matter physics
Physical chemistry
Chemistry
Physics
Electrode
Metallurgy
Composite material
Medicine
Endocrinology
Organic chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41563-024-01800-8
- https://www.nature.com/articles/s41563-024-01800-8.pdf
- OA Status
- hybrid
- Cited By
- 39
- References
- 47
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4391474836
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4391474836Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41563-024-01800-8Digital Object Identifier
- Title
-
Unlocking Li superionic conductivity in face-centred cubic oxides via face-sharing configurationsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2024Year of publication
- Publication date
-
2024-02-02Full publication date if available
- Authors
-
Yu Chen, Zhengyan Lun, Xinye Zhao, Krishna Prasad Koirala, Linze Li, Yingzhi Sun, Christopher A. O’Keefe, Xiaochen Yang, Zijian Cai, Chongmin Wang, Huiwen Ji, Clare P. Grey, Bin Ouyang, Gerbrand CederList of authors in order
- Landing page
-
https://doi.org/10.1038/s41563-024-01800-8Publisher landing page
- PDF URL
-
https://www.nature.com/articles/s41563-024-01800-8.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
hybridOpen access status per OpenAlex
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-
https://www.nature.com/articles/s41563-024-01800-8.pdfDirect OA link when available
- Concepts
-
Fast ion conductor, Stoichiometry, Materials science, Conductivity, Lithium (medication), Ion, Electrolyte, Spinel, Ionic conductivity, Chemical physics, Thermal conduction, Condensed matter physics, Physical chemistry, Chemistry, Physics, Electrode, Metallurgy, Composite material, Medicine, Endocrinology, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
39Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 25, 2024: 14Per-year citation counts (last 5 years)
- References (count)
-
47Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.Li | 33, 42, 61, 88, 117 |
| abstract_inverted_index.We | 56 |
| abstract_inverted_index.as | 13, 16 |
| abstract_inverted_index.at | 99 |
| abstract_inverted_index.be | 23 |
| abstract_inverted_index.cm | 97 |
| abstract_inverted_index.in | 36, 39, 50, 120 |
| abstract_inverted_index.is | 20 |
| abstract_inverted_index.of | 74, 91, 107, 115 |
| abstract_inverted_index.to | 22 |
| abstract_inverted_index.we | 31 |
| abstract_inverted_index.× | 93 |
| abstract_inverted_index.255 | 108 |
| abstract_inverted_index.Li, | 75 |
| abstract_inverted_index.Li. | 55 |
| abstract_inverted_index.Our | 110 |
| abstract_inverted_index.The | 81 |
| abstract_inverted_index.and | 70 |
| abstract_inverted_index.are | 9 |
| abstract_inverted_index.for | 25, 132 |
| abstract_inverted_index.low | 104 |
| abstract_inverted_index.new | 134 |
| abstract_inverted_index.not | 11 |
| abstract_inverted_index.the | 17, 59, 72, 113 |
| abstract_inverted_index.via | 53 |
| abstract_inverted_index.(Li) | 27 |
| abstract_inverted_index.3.38 | 92 |
| abstract_inverted_index.Here | 30 |
| abstract_inverted_index.been | 45 |
| abstract_inverted_index.fast | 78 |
| abstract_inverted_index.find | 57 |
| abstract_inverted_index.have | 44 |
| abstract_inverted_index.meV. | 109 |
| abstract_inverted_index.room | 100 |
| abstract_inverted_index.that | 58 |
| abstract_inverted_index.vast | 126 |
| abstract_inverted_index.with | 2, 67, 102, 125 |
| abstract_inverted_index.work | 111 |
| abstract_inverted_index.−1 | 98 |
| abstract_inverted_index.−4 | 95 |
| abstract_inverted_index.(fcc) | 6 |
| abstract_inverted_index.anion | 7 |
| abstract_inverted_index.cubic | 5 |
| abstract_inverted_index.novel | 65 |
| abstract_inverted_index.raise | 71 |
| abstract_inverted_index.total | 87 |
| abstract_inverted_index.which | 40 |
| abstract_inverted_index.Li-ion | 79 |
| abstract_inverted_index.Oxides | 1 |
| abstract_inverted_index.cation | 48 |
| abstract_inverted_index.create | 63 |
| abstract_inverted_index.energy | 73 |
| abstract_inverted_index.excess | 54 |
| abstract_inverted_index.ground | 131 |
| abstract_inverted_index.oxides | 38 |
| abstract_inverted_index.spinel | 66 |
| abstract_inverted_index.barrier | 106 |
| abstract_inverted_index.created | 46 |
| abstract_inverted_index.fertile | 130 |
| abstract_inverted_index.lithium | 26 |
| abstract_inverted_index.thereby | 76 |
| abstract_inverted_index.thought | 21 |
| abstract_inverted_index.through | 47 |
| abstract_inverted_index.unlocks | 112 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.chemical | 127 |
| abstract_inverted_index.compound | 84 |
| abstract_inverted_index.exhibits | 85 |
| abstract_inverted_index.fcc-type | 37 |
| abstract_inverted_index.lattices | 52 |
| abstract_inverted_index.designing | 116 |
| abstract_inverted_index.framework | 19, 124 |
| abstract_inverted_index.generally | 10 |
| abstract_inverted_index.migration | 105 |
| abstract_inverted_index.potential | 114 |
| abstract_inverted_index.promoting | 77 |
| abstract_inverted_index.providing | 129 |
| abstract_inverted_index.conductors | 119 |
| abstract_inverted_index.considered | 12 |
| abstract_inverted_index.structural | 18, 123 |
| abstract_inverted_index.sublattice | 8 |
| abstract_inverted_index.superionic | 28, 34, 89, 118 |
| abstract_inverted_index.conduction. | 29, 80 |
| abstract_inverted_index.demonstrate | 32 |
| abstract_inverted_index.discovering | 133 |
| abstract_inverted_index.solid-state | 14, 135 |
| abstract_inverted_index.temperature | 101 |
| abstract_inverted_index.conductivity | 35, 90 |
| abstract_inverted_index.electrolytes | 15 |
| abstract_inverted_index.face-centred | 4 |
| abstract_inverted_index.face-sharing | 41, 60 |
| abstract_inverted_index.flexibility, | 128 |
| abstract_inverted_index.prototypical | 122 |
| abstract_inverted_index.unfavourable | 24 |
| abstract_inverted_index.electrolytes. | 136 |
| abstract_inverted_index.rocksalt-type | 51 |
| abstract_inverted_index.stoichiometry | 69 |
| abstract_inverted_index.configurations | 43, 62 |
| abstract_inverted_index.unconventional | 68 |
| abstract_inverted_index.Li–In–Sn–O | 83 |
| abstract_inverted_index.over-stoichiometry | 49 |
| abstract_inverted_index.over-stoichiometric | 82 |
| cited_by_percentile_year.max | 100 |
| cited_by_percentile_year.min | 99 |
| corresponding_author_ids | https://openalex.org/A5070260665, https://openalex.org/A5032840004 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 14 |
| corresponding_institution_ids | https://openalex.org/I103163165, https://openalex.org/I223532165 |
| citation_normalized_percentile.value | 0.98833729 |
| citation_normalized_percentile.is_in_top_1_percent | True |
| citation_normalized_percentile.is_in_top_10_percent | True |