Unveiling the Influence of Linkers on Conformations of Oligomeric Acceptors for High‐Performance Polymer Solar Cells Article Swipe
Jingnan Wu
,
Fengbo Sun
,
Xunchang Wang
,
Qiaonan Chen
,
Leandro R. Franco
,
Xufan Zheng
,
C. Moysés Araújo
,
Renqiang Yang
,
Donghong Yu
,
Ergang Wang
·
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202406772
YOU?
·
· 2024
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202406772
Conformational isomerism of organic photovoltaic materials has a profound impact on their molecular packing and therefore performance of polymer solar cells (PSCs). However, the conformations of oligomeric acceptors (OAs) are mostly predicted by simulations rather than experimental determinations. Herein, the stereochemical S ‐shaped structure of two dimeric‐type acceptor molecules, V‐DYIC and V‐DYIC‐4F, is first confirmed with different end groups (IC for V‐DYIC and IC‐2F for V‐DYIC‐4F), incorporating vinylene linkage for connecting the distinct state‐of‐the‐art small molecule acceptor Y ‐segments. Through the synthetic control of fluorination sites adjacent to the vinyl‐linker, S ‐shaped the conformation by NMR experiments is validated. Compared to the O ‐shaped dimer, S ‐shaped conformation results in enhanced lamellar order and reduced nonradiative recombination losses. The optimal acceptor, V‐DYIC‐4F, achieved a champion efficiency of 18.10% with the lowest energy loss of 0.556 eV in its devices paired with PM6 due to their efficient carrier transport, and suppressed recombination compared to other devices, being attributed to the synergistic effect of conformation and end group fluorination. The insights gained in this work contribute valuable knowledge of both synthetic control and structural determination of OAs, providing strategic design guidelines for the future development of dimeric acceptors toward high‐efficiency PSCs.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/advs.202406772
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202406772
- OA Status
- gold
- Cited By
- 9
- References
- 45
- Related Works
- 10
- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
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https://openalex.org/W4402005423Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/advs.202406772Digital Object Identifier
- Title
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Unveiling the Influence of Linkers on Conformations of Oligomeric Acceptors for High‐Performance Polymer Solar CellsWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2024Year of publication
- Publication date
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2024-08-29Full publication date if available
- Authors
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Jingnan Wu, Fengbo Sun, Xunchang Wang, Qiaonan Chen, Leandro R. Franco, Xufan Zheng, C. Moysés Araújo, Renqiang Yang, Donghong Yu, Ergang WangList of authors in order
- Landing page
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https://doi.org/10.1002/advs.202406772Publisher landing page
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202406772Direct link to full text PDF
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202406772Direct OA link when available
- Concepts
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Polymer, Materials science, Nanotechnology, Polymer chemistry, Chemical engineering, Chemistry, Engineering, Composite materialTop concepts (fields/topics) attached by OpenAlex
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9Total citation count in OpenAlex
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2025: 6, 2024: 3Per-year citation counts (last 5 years)
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45Number of works referenced by this work
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10Other works algorithmically related by OpenAlex
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