Visualization of Phase Segregation and Surface Reconstruction of Pt-Based Bi-metallic Clusters During In Situ Oxidation Article Swipe
Jane Y. Howe
,
Ya-Huei Cathy Chin
,
Weifeng Tu
,
Yifei Yang
,
Junnan Shangguan
,
Stas Dogel
,
David Hoyle
,
Matthew Reynolds
,
Hooman Hosseinkhannazer
,
D. D. Perović
·
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.1017/s1431927616004529
YOU?
·
· 2016
· Open Access
·
· DOI: https://doi.org/10.1017/s1431927616004529
Bi-metallic clusters such as Ni-Au [1], Pt-Ni [2], Pd-Au [3], Pt-Pd [4], and Pt-Au of nano-meter dimensions are effective catalysts for hydrocarbon activation (Ni-Au [1], Pt-Ni [2]), alcohol oxidation (Pd-Au) [3], aromatic hydrogenation (Pt-Pd) [4], and water-gas-shift (Pt-Au) [5] reactions.Their catalytic performance is dictated predominantly by the number and type of sites at their surfaces and thus by their size, shape, and local atomic ensembles at cluster surfaces.When exposed to reaction mixtures, these clusters may undergo dynamics reconstruction at surfaces and in the bulk phase, driven by changing chemical potentials.As an example, bi-elemental alloy with a more oxophilic metal may disintegrate and undergo bulk phase segregation during oxidation reactions, as oxygen atoms solvate into the cluster bulk and the more oxophilic metal undergoes bulk oxidation.
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- en
- Landing Page
- https://doi.org/10.1017/s1431927616004529
- https://www.cambridge.org/core/services/aop-cambridge-core/content/view/22335ADB19BD9F978819D533F35A3486/S1431927616004529a.pdf/div-class-title-span-class-bold-visualization-of-phase-segregation-and-surface-reconstruction-of-pt-based-bi-metallic-clusters-during-span-span-class-italic-span-class-bold-in-situ-span-span-span-class-bold-oxidation-span-div.pdf
- OA Status
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- Cited By
- 1
- References
- 7
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W2559796380
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https://openalex.org/W2559796380Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1017/s1431927616004529Digital Object Identifier
- Title
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Visualization of Phase Segregation and Surface Reconstruction of Pt-Based Bi-metallic Clusters During In Situ OxidationWork title
- Type
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articleOpenAlex work type
- Language
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enPrimary language
- Publication year
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2016Year of publication
- Publication date
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2016-07-01Full publication date if available
- Authors
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Jane Y. Howe, Ya-Huei Cathy Chin, Weifeng Tu, Yifei Yang, Junnan Shangguan, Stas Dogel, David Hoyle, Matthew Reynolds, Hooman Hosseinkhannazer, D. D. PerovićList of authors in order
- Landing page
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https://doi.org/10.1017/s1431927616004529Publisher landing page
- PDF URL
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https://www.cambridge.org/core/services/aop-cambridge-core/content/view/22335ADB19BD9F978819D533F35A3486/S1431927616004529a.pdf/div-class-title-span-class-bold-visualization-of-phase-segregation-and-surface-reconstruction-of-pt-based-bi-metallic-clusters-during-span-span-class-italic-span-class-bold-in-situ-span-span-span-class-bold-oxidation-span-div.pdfDirect link to full text PDF
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YesWhether a free full text is available
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bronzeOpen access status per OpenAlex
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https://www.cambridge.org/core/services/aop-cambridge-core/content/view/22335ADB19BD9F978819D533F35A3486/S1431927616004529a.pdf/div-class-title-span-class-bold-visualization-of-phase-segregation-and-surface-reconstruction-of-pt-based-bi-metallic-clusters-during-span-span-class-italic-span-class-bold-in-situ-span-span-span-class-bold-oxidation-span-div.pdfDirect OA link when available
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In situ, Materials science, Visualization, Metal, Surface reconstruction, Phase (matter), Surface (topology), Metallurgy, Chemistry, Computer science, Geometry, Data mining, Organic chemistry, MathematicsTop concepts (fields/topics) attached by OpenAlex
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1Total citation count in OpenAlex
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2019: 1Per-year citation counts (last 5 years)
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10Other works algorithmically related by OpenAlex
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