Water‐Enhanced Multicolor Electrochromism in Nickel‐Catecholate MOFs Article Swipe
Qi Zhao
,
Jing Yang
,
Xingyang Wang
,
Wanwan Wang
,
Yulin Gao
,
Xue Chen
,
Jianguo Sun
,
Hao Yuan
,
Yu Liu
,
Jinwoo Park
,
Lewis Kien Juen Ting
,
Qing Wang
,
Pooi See Lee
,
Yanfeng Gao
,
Yong‐Wei Zhang
,
John Wang
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202500678
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1002/advs.202500678
Metal–organic frameworks (MOFs) represent a novel electrochromic material system but are limited in tunable color versatility, rapid switching speed, and long‐term cycling stability. A new multicolor electrochromic behavior is reported, with transitions from green to blue to purple, in conducting nickel‐catecholate (Ni‐CAT‐1) MOFs. The system significantly improves cycling stability to 2000 cycles and reduces switching time to 3.6 s, both of which outperform most state‐of‐the‐art MOF systems. An in‐depth understanding of the coloring mechanism, particularly the interconversion among C─O, C─O • , and C = O groups is revealed. Water molecules play diverse roles in this redox process. Specifically, water molecules induce distortions in Ni─O bonds, facilitating C = O bond formation and expediting the oxidized coloring process, while also aiding the dissociation of ions from solvation complexes to enhance the reduction process. The practical applications of these findings are demonstrated by designing flexible multicolor electrochromic devices (FMEDs) for use in camouflage, flexible displays, and augmented reality (AR).
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1002/advs.202500678
- https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202500678
- OA Status
- gold
- Cited By
- 2
- References
- 61
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4408921400
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4408921400Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1002/advs.202500678Digital Object Identifier
- Title
-
Water‐Enhanced Multicolor Electrochromism in Nickel‐Catecholate MOFsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
-
2025-03-27Full publication date if available
- Authors
-
Qi Zhao, Jing Yang, Xingyang Wang, Wanwan Wang, Yulin Gao, Xue Chen, Jianguo Sun, Hao Yuan, Yu Liu, Jinwoo Park, Lewis Kien Juen Ting, Qing Wang, Pooi See Lee, Yanfeng Gao, Yong‐Wei Zhang, John WangList of authors in order
- Landing page
-
https://doi.org/10.1002/advs.202500678Publisher landing page
- PDF URL
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https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202500678Direct link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/advs.202500678Direct OA link when available
- Concepts
-
Electrochromism, Nickel, Materials science, Chemical engineering, Nanotechnology, Chemistry, Metallurgy, Electrode, Physical chemistry, EngineeringTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
2Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 2Per-year citation counts (last 5 years)
- References (count)
-
61Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.reality | 157 |
| abstract_inverted_index.reduces | 54 |
| abstract_inverted_index.tunable | 14 |
| abstract_inverted_index.Abstract | 0 |
| abstract_inverted_index.behavior | 28 |
| abstract_inverted_index.coloring | 73, 117 |
| abstract_inverted_index.findings | 139 |
| abstract_inverted_index.flexible | 144, 153 |
| abstract_inverted_index.improves | 47 |
| abstract_inverted_index.material | 8 |
| abstract_inverted_index.oxidized | 116 |
| abstract_inverted_index.process, | 118 |
| abstract_inverted_index.process. | 98, 133 |
| abstract_inverted_index.systems. | 67 |
| abstract_inverted_index.augmented | 156 |
| abstract_inverted_index.complexes | 128 |
| abstract_inverted_index.designing | 143 |
| abstract_inverted_index.displays, | 154 |
| abstract_inverted_index.formation | 112 |
| abstract_inverted_index.molecules | 91, 101 |
| abstract_inverted_index.practical | 135 |
| abstract_inverted_index.reduction | 132 |
| abstract_inverted_index.reported, | 30 |
| abstract_inverted_index.represent | 4 |
| abstract_inverted_index.revealed. | 89 |
| abstract_inverted_index.solvation | 127 |
| abstract_inverted_index.stability | 49 |
| abstract_inverted_index.switching | 18, 55 |
| abstract_inverted_index.conducting | 40 |
| abstract_inverted_index.expediting | 114 |
| abstract_inverted_index.frameworks | 2 |
| abstract_inverted_index.in‐depth | 69 |
| abstract_inverted_index.mechanism, | 74 |
| abstract_inverted_index.multicolor | 26, 145 |
| abstract_inverted_index.outperform | 63 |
| abstract_inverted_index.stability. | 23 |
| abstract_inverted_index.camouflage, | 152 |
| abstract_inverted_index.distortions | 103 |
| abstract_inverted_index.long‐term | 21 |
| abstract_inverted_index.transitions | 32 |
| abstract_inverted_index.applications | 136 |
| abstract_inverted_index.demonstrated | 141 |
| abstract_inverted_index.dissociation | 123 |
| abstract_inverted_index.facilitating | 107 |
| abstract_inverted_index.particularly | 75 |
| abstract_inverted_index.versatility, | 16 |
| abstract_inverted_index.Specifically, | 99 |
| abstract_inverted_index.significantly | 46 |
| abstract_inverted_index.understanding | 70 |
| abstract_inverted_index.(Ni‐CAT‐1) | 42 |
| abstract_inverted_index.electrochromic | 7, 27, 146 |
| abstract_inverted_index.Metal–organic | 1 |
| abstract_inverted_index.interconversion | 77 |
| abstract_inverted_index.nickel‐catecholate | 41 |
| abstract_inverted_index.state‐of‐the‐art | 65 |
| cited_by_percentile_year.max | 97 |
| cited_by_percentile_year.min | 95 |
| countries_distinct_count | 2 |
| institutions_distinct_count | 16 |
| citation_normalized_percentile.value | 0.84077148 |
| citation_normalized_percentile.is_in_top_1_percent | False |
| citation_normalized_percentile.is_in_top_10_percent | True |