Wearable electrochemical sensor for real-time sweat monitoring powered by Li–S battery: Rapid ion-electron transduction driven by high-entropy Prussian blue analogues Article Swipe
Zhonghui Sun
,
Qiuling Huang
,
Zhanchao Li
,
Weitao Zheng
,
Yan Mao
,
Dongxue Han
,
Gang Huang
·
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.asems.2025.100150
YOU?
·
· 2025
· Open Access
·
· DOI: https://doi.org/10.1016/j.asems.2025.100150
The portable electrochemical sensors couple with high-energy density batteries lay the foundation for intelligent electronic devices capable of real-time and long-term monitoring of signals at the molecular level. Currently, high-entropy materials play a crucial role in advanced energy storage system and electroanalytical chemistry due to their powerful multi active centers and lattice strain fields. Herein, we propose high-entropy Prussian blue analogues (HE-PBA) as a bidirectional catalyst to reduce the activation energy of sulfur redox reaction, alleviate polysulfides shuttle, and inhibit lithium dendritic growth in Li–S battery. Furthermore, benefited from hierarchical HE-PBA with multiple redox active sites, superior ion-selective effect, high ionic/electrical conductivity and hydrophobicity, thus contributing to splendid ion-electron transducer capability as solid contact layer in wearable potentiometric electrochemical sensors. As a result, an advanced wearable electronic device integrates LSB as a power source with potentiometric electrochemical sensor unit equipped with ion selective electrode, enabling real-time monitoring of K+ concentration in sweat metabolite during outdoor exercise. In a word, this work demonstrates a tremendous potential of designing multifunctional electrode materials for advanced energy storage and electrochemical sensing applications through high entropy strategies.
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Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1016/j.asems.2025.100150
- OA Status
- gold
- Cited By
- 2
- References
- 51
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- OpenAlex ID
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All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
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https://openalex.org/W4408541402Canonical identifier for this work in OpenAlex
- DOI
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https://doi.org/10.1016/j.asems.2025.100150Digital Object Identifier
- Title
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Wearable electrochemical sensor for real-time sweat monitoring powered by Li–S battery: Rapid ion-electron transduction driven by high-entropy Prussian blue analoguesWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2025Year of publication
- Publication date
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2025-03-18Full publication date if available
- Authors
-
Zhonghui Sun, Qiuling Huang, Zhanchao Li, Weitao Zheng, Yan Mao, Dongxue Han, Gang HuangList of authors in order
- Landing page
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https://doi.org/10.1016/j.asems.2025.100150Publisher landing page
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YesWhether a free full text is available
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goldOpen access status per OpenAlex
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https://doi.org/10.1016/j.asems.2025.100150Direct OA link when available
- Concepts
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Prussian blue, Wearable computer, Electrochemistry, Ion, Battery (electricity), Electron, Wearable technology, Materials science, Nanotechnology, Chemistry, Electrode, Computer science, Physics, Embedded system, Organic chemistry, Power (physics), Quantum mechanics, Physical chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
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2Total citation count in OpenAlex
- Citations by year (recent)
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2025: 2Per-year citation counts (last 5 years)
- References (count)
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51Number of works referenced by this work
- Related works (count)
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10Other works algorithmically related by OpenAlex
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| abstract_inverted_index.In | 156 |
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| abstract_inverted_index.as | 62, 111, 130 |
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| abstract_inverted_index.we | 55 |
| abstract_inverted_index.LSB | 129 |
| abstract_inverted_index.The | 0 |
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| abstract_inverted_index.their | 45 |
| abstract_inverted_index.word, | 158 |
| abstract_inverted_index.HE-PBA | 90 |
| abstract_inverted_index.Li–S | 84 |
| abstract_inverted_index.active | 48, 94 |
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| abstract_inverted_index.device | 127 |
| abstract_inverted_index.during | 153 |
| abstract_inverted_index.energy | 37, 70, 172 |
| abstract_inverted_index.growth | 82 |
| abstract_inverted_index.level. | 27 |
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| abstract_inverted_index.sensor | 137 |
| abstract_inverted_index.sites, | 95 |
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| abstract_inverted_index.sulfur | 72 |
| abstract_inverted_index.system | 39 |
| abstract_inverted_index.Herein, | 54 |
| abstract_inverted_index.capable | 16 |
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| abstract_inverted_index.devices | 15 |
| abstract_inverted_index.effect, | 98 |
| abstract_inverted_index.entropy | 180 |
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| abstract_inverted_index.propose | 56 |
| abstract_inverted_index.result, | 122 |
| abstract_inverted_index.sensing | 176 |
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| abstract_inverted_index.through | 178 |
| abstract_inverted_index.(HE-PBA) | 61 |
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| abstract_inverted_index.battery. | 85 |
| abstract_inverted_index.catalyst | 65 |
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| countries_distinct_count | 0 |
| institutions_distinct_count | 7 |
| sustainable_development_goals[0].id | https://metadata.un.org/sdg/7 |
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| sustainable_development_goals[0].display_name | Affordable and clean energy |
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| citation_normalized_percentile.is_in_top_10_percent | True |