Well-defined double hysteresis loop in NaNbO3 antiferroelectrics Article Swipe
Nengneng Luo
,
Li Ma
,
Gengguang Luo
,
Chao Xu
,
Lixiang Rao
,
Zhengu Chen
,
Zhenyong Cen
,
Qin Feng
,
Xiyong Chen
,
Toyohisa Fujita
,
Ye Zhu
,
Jiawang Hong
,
Jing‐Feng Li
,
Shujun Zhang
·
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-023-37469-x
YOU?
·
· 2023
· Open Access
·
· DOI: https://doi.org/10.1038/s41467-023-37469-x
Antiferroelectrics (AFEs) are promising candidates in energy-storage capacitors, electrocaloric solid-cooling, and displacement transducers. As an actively studied lead-free antiferroelectric (AFE) material, NaNbO 3 has long suffered from its ferroelectric (FE)-like polarization-electric field ( P - E ) hysteresis loops with high remnant polarization and large hysteresis. Guided by theoretical calculations, a new strategy of reducing the oxygen octahedral tilting angle is proposed to stabilize the AFE P phase (Space group Pbma) of NaNbO 3 . To validate this, we judiciously introduced CaHfO 3 with a low Goldschmidt tolerance factor and AgNbO 3 with a low electronegativity difference into NaNbO 3 , the decreased cation displacements and [BO 6 ] octahedral tilting angles were confirmed by Synchrotron X-ray powder diffraction and aberration-corrected scanning transmission electron microscopy. Of particular importance is that the 0.75NaNbO 3 −0.20AgNbO 3 −0.05CaHfO 3 ceramic exhibits highly reversible phase transition between the AFE and FE states, showing well-defined double P - E loops and sprout-shaped strain-electric field curves with reduced hysteresis, low remnant polarization, high AFE-FE phase transition field, and zero negative strain. Our work provides a new strategy for designing NaNbO 3 -based AFE material with well-defined double P - E loops, which can also be extended to discover a variety of new lead-free AFEs.
Related Topics
Concepts
Materials science
Antiferroelectricity
Ferroelectricity
Polarization (electrochemistry)
Hysteresis
Phase transition
Octahedron
Electronegativity
Condensed matter physics
Synchrotron
Dielectric
Scanning transmission electron microscopy
Crystallography
Transmission electron microscopy
Nanotechnology
Optics
Crystal structure
Optoelectronics
Chemistry
Physics
Physical chemistry
Organic chemistry
Metadata
- Type
- article
- Language
- en
- Landing Page
- https://doi.org/10.1038/s41467-023-37469-x
- https://www.nature.com/articles/s41467-023-37469-x.pdf
- OA Status
- gold
- Cited By
- 82
- References
- 61
- Related Works
- 10
- OpenAlex ID
- https://openalex.org/W4361272062
All OpenAlex metadata
Raw OpenAlex JSON
- OpenAlex ID
-
https://openalex.org/W4361272062Canonical identifier for this work in OpenAlex
- DOI
-
https://doi.org/10.1038/s41467-023-37469-xDigital Object Identifier
- Title
-
Well-defined double hysteresis loop in NaNbO3 antiferroelectricsWork title
- Type
-
articleOpenAlex work type
- Language
-
enPrimary language
- Publication year
-
2023Year of publication
- Publication date
-
2023-03-30Full publication date if available
- Authors
-
Nengneng Luo, Li Ma, Gengguang Luo, Chao Xu, Lixiang Rao, Zhengu Chen, Zhenyong Cen, Qin Feng, Xiyong Chen, Toyohisa Fujita, Ye Zhu, Jiawang Hong, Jing‐Feng Li, Shujun ZhangList of authors in order
- Landing page
-
https://doi.org/10.1038/s41467-023-37469-xPublisher landing page
- PDF URL
-
https://www.nature.com/articles/s41467-023-37469-x.pdfDirect link to full text PDF
- Open access
-
YesWhether a free full text is available
- OA status
-
goldOpen access status per OpenAlex
- OA URL
-
https://www.nature.com/articles/s41467-023-37469-x.pdfDirect OA link when available
- Concepts
-
Materials science, Antiferroelectricity, Ferroelectricity, Polarization (electrochemistry), Hysteresis, Phase transition, Octahedron, Electronegativity, Condensed matter physics, Synchrotron, Dielectric, Scanning transmission electron microscopy, Crystallography, Transmission electron microscopy, Nanotechnology, Optics, Crystal structure, Optoelectronics, Chemistry, Physics, Physical chemistry, Organic chemistryTop concepts (fields/topics) attached by OpenAlex
- Cited by
-
82Total citation count in OpenAlex
- Citations by year (recent)
-
2025: 34, 2024: 31, 2023: 17Per-year citation counts (last 5 years)
- References (count)
-
61Number of works referenced by this work
- Related works (count)
-
10Other works algorithmically related by OpenAlex
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| referenced_works | https://openalex.org/W2026331531, https://openalex.org/W3148912309, https://openalex.org/W2617785911, https://openalex.org/W2906326900, https://openalex.org/W3088638723, https://openalex.org/W2100274435, https://openalex.org/W1965502119, https://openalex.org/W1998495409, https://openalex.org/W2074423697, https://openalex.org/W2626263688, https://openalex.org/W2926972455, https://openalex.org/W1679720057, https://openalex.org/W3126879168, https://openalex.org/W2562666392, https://openalex.org/W2011484781, https://openalex.org/W1994160141, https://openalex.org/W2776432833, https://openalex.org/W2016842299, https://openalex.org/W4281997795, https://openalex.org/W4300981688, https://openalex.org/W2321982418, https://openalex.org/W1976221107, https://openalex.org/W2239931029, https://openalex.org/W1970014398, https://openalex.org/W3046613922, https://openalex.org/W2007358238, https://openalex.org/W4214704576, https://openalex.org/W1981015924, https://openalex.org/W2167590372, https://openalex.org/W3015367655, https://openalex.org/W3082997021, https://openalex.org/W1618239098, https://openalex.org/W2150543342, https://openalex.org/W2074559848, https://openalex.org/W3043932307, https://openalex.org/W2731015871, https://openalex.org/W4212948062, https://openalex.org/W2083222334, https://openalex.org/W1979544533, https://openalex.org/W1981368803, https://openalex.org/W1970127494, https://openalex.org/W2078086786, https://openalex.org/W2036113194, https://openalex.org/W4220904707, https://openalex.org/W2558338015, https://openalex.org/W3199898427, https://openalex.org/W3114216596, https://openalex.org/W3038827654, https://openalex.org/W2945141644, https://openalex.org/W3049026449, https://openalex.org/W2913878696, https://openalex.org/W3088636284, https://openalex.org/W2990623947, https://openalex.org/W3090870059, https://openalex.org/W2892708765, https://openalex.org/W3024087733, https://openalex.org/W1536768010, https://openalex.org/W2576011151, https://openalex.org/W2030673416, https://openalex.org/W3100776993, https://openalex.org/W4226466494 |
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| corresponding_author_ids | https://openalex.org/A5084854060, https://openalex.org/A5100658008, https://openalex.org/A5100747643 |
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