Adam M. Boyce
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View article: A Bilayer Cathode Design Procedure for Li ion Batteries Using the Multilayer Doyle-Fuller-Newman Model (M-DFN)
A Bilayer Cathode Design Procedure for Li ion Batteries Using the Multilayer Doyle-Fuller-Newman Model (M-DFN) Open
Heterogeneities in lithium ion batteries can be significant factors in electrode under utilisation and degradation while charging. Bilayer electrodes have been proposed as a convenient and scalable way to homogenise the electrode response.…
View article: Understanding energy-power trade-off in the structure of Li-Ion battery cathodes by localized operando XRD
Understanding energy-power trade-off in the structure of Li-Ion battery cathodes by localized operando XRD Open
Power and energy density represent a trade-off in design of lithium-ion batteries. This is because for high energy density thick electrodes are required, and for high power density thin electrodes are required. A strategy to break this tra…
View article: Flow Battery Manifold Design With Heterogeneous Inputs Through Generative Adversarial Neural Networks
Flow Battery Manifold Design With Heterogeneous Inputs Through Generative Adversarial Neural Networks Open
Generative machine learning has emerged as a powerful tool for design representation and exploration. However, its application is often constrained by the need for large datasets of existing designs and the lack of interpretability about w…
View article: Flow Battery Manifold Design with Heterogeneous Inputs Through Generative Adversarial Neural Networks
Flow Battery Manifold Design with Heterogeneous Inputs Through Generative Adversarial Neural Networks Open
Generative machine learning has emerged as a powerful tool for design representation and exploration. However, its application is often constrained by the need for large datasets of existing designs and the lack of interpretability about w…
View article: Bridging the Gap between Microstructurally Resolved Computed Tomography-Based and Homogenised Doyle-Fuller-Newman Models for Lithium-Ion Batteries
Bridging the Gap between Microstructurally Resolved Computed Tomography-Based and Homogenised Doyle-Fuller-Newman Models for Lithium-Ion Batteries Open
Lithium-ion batteries (LIB) are synonymous with the modern age of electrification, yet advances in battery design, manufacturing, and chemistry are still urgently needed. Mathematical modelling plays an important role in understanding LIB …
View article: Editorial: Lithium-ion batteries: manufacturing, modelling and advanced experimental techniques
Editorial: Lithium-ion batteries: manufacturing, modelling and advanced experimental techniques Open
View article: The Effect of Mud Cracking on the Performance of Thick Li‐Ion Electrodes
The Effect of Mud Cracking on the Performance of Thick Li‐Ion Electrodes Open
Electrode‐level fracture, or mud cracking, occurs during the drying process of Li‐ion electrodes and is known to be particularly prevalent in thick electrodes. Whilst these cracks are generally viewed as an obstruction to the production of…
View article: A groovy laser processing route to achieving high power and energy lithium-ion batteries
A groovy laser processing route to achieving high power and energy lithium-ion batteries Open
3D-structured NMC622 with precisely controlled electrolyte channels were manufactured by incorporating femtosecond laser processing with conventional slurry casting. Demonstrated in a full cell for the first time, the 3D electrode structur…
View article: The role of chemo-mechanical modelling in the development of battery technology—a perspective
The role of chemo-mechanical modelling in the development of battery technology—a perspective Open
In the race to reduce global CO 2 emissions and achieve net-zero, chemomechanics must play a critical role in the technological development of current and next-generation batteries to improve their energy storage capabilities and their lif…
View article: A Groovy Laser Processing Route to Achieving High Power and Energy Lithium-Ion Batteries
A Groovy Laser Processing Route to Achieving High Power and Energy Lithium-Ion Batteries Open
View article: Bridging the Gap Between Microstructurally ResolvedComputed Tomography-Based and HomogenisedDoyle-Fuller-Newman Models for Lithium-Ion Batteries
Bridging the Gap Between Microstructurally ResolvedComputed Tomography-Based and HomogenisedDoyle-Fuller-Newman Models for Lithium-Ion Batteries Open
Lithium-ion batteries (LIB) are synonymous with the modern age of electrification, yet advances in battery design, manufacturing, and chemistry are still urgently needed. Mathematical modelling plays an important role in understanding LIB …
View article: Silicon-Based Solid-State Batteries: Electrochemistry and Mechanics to Guide Design and Operation
Silicon-Based Solid-State Batteries: Electrochemistry and Mechanics to Guide Design and Operation Open
Solid-state batteries (SSBs) are promising alternatives to the incumbent lithium-ion technology; however, they face a unique set of challenges that must be overcome to enable their widespread adoption. These challenges include solid-solid …
View article: Numerical Design of Microporous Carbon Binder Domains Phase in Composite Cathodes for Lithium-Ion Batteries
Numerical Design of Microporous Carbon Binder Domains Phase in Composite Cathodes for Lithium-Ion Batteries Open
Lithium-ion battery (LIB) performance can be significantly affected by the nature of the complex electrode microstructure. The carbon binder domain (CBD) present in almost all LIB electrodes is used to enhance mechanical stability and faci…
View article: Silicon-based Solid-State Batteries: Electrochemistry and Mechanics to Guide Design and Operation
Silicon-based Solid-State Batteries: Electrochemistry and Mechanics to Guide Design and Operation Open
Solid-state batteries are promising alternatives to the incumbent lithium-ion technology however, they face a unique set of challenges that must be overcome to enable their widespread adoption. These challenges include solid-solid interfac…
View article: Direct 4D Observations of Electrochemically Induced Intergranular Cracking in NMC811 Particles
Direct 4D Observations of Electrochemically Induced Intergranular Cracking in NMC811 Particles Open
Establishing the nature of crack formation is paramount to understanding the degradation modes that govern decline in battery performance. Cracking has several possible origins; however, it can be classified in two general cases: mechanica…
View article: Direct 4D Observations of Electrochemically Induced Intergranular Cracking in NMC811 Particles
Direct 4D Observations of Electrochemically Induced Intergranular Cracking in NMC811 Particles Open
Establishing the nature of crack formation is paramount to understanding the degradation modes that govern decline in battery performance. Cracking has several possible origins; however, it can be classified in two general cases: mechanica…
View article: Direct observations of electrochemically induced intergranular cracking in polycrystalline NMC811 particles
Direct observations of electrochemically induced intergranular cracking in polycrystalline NMC811 particles Open
Establishing the nature of crack generation, formation, and propagation is paramount to understanding the degradation modes that govern decline in battery performance.
View article: Quantitative assessment of machine-learning segmentation of battery electrode materials for active material quantification
Quantitative assessment of machine-learning segmentation of battery electrode materials for active material quantification Open
Funding Information: This work was made possible by the facilities and support provided by the Research Complex at Harwell. The research was funded by The Faraday Institution [grant numbers: EP/S003053/1, FIRG015, FIRG025]. PRS and DJLB ac…
View article: Towards Optimised Cell Design of Thin Film Silicon-Based Solid-State Batteries via Modelling and Experimental Characterisation
Towards Optimised Cell Design of Thin Film Silicon-Based Solid-State Batteries via Modelling and Experimental Characterisation Open
To realise the promise of solid-state batteries, negative electrode materials exhibiting large volumetric expansions, such as Li and Si, must be used. These volume changes can cause significant mechanical stresses and strains that affect c…
View article: Roadmap on Li-ion battery manufacturing research
Roadmap on Li-ion battery manufacturing research Open
Growth in the Li-ion battery market continues to accelerate, driven primarily by the increasing need for economic energy storage for electric vehicles. Electrode manufacture by slurry casting is the first main step in cell production but m…
View article: A continuum of physics-based lithium-ion battery models reviewed
A continuum of physics-based lithium-ion battery models reviewed Open
Physics-based electrochemical battery models derived from porous electrode theory are a very powerful tool for understanding lithium-ion batteries, as well as for improving their design and management. Different model fidelity, and thus mo…
View article: A Continuum of Physics-Based Lithium-Ion Battery Models Reviewed
A Continuum of Physics-Based Lithium-Ion Battery Models Reviewed Open
Physics-based electrochemical battery models derived from porous electrode theory are a very powerful tool for understanding lithium-ion batteries, as well as for improving their design and management. Different model fidelity, and thus mo…
View article: Cracking predictions of lithium-ion battery electrodes by X-ray computed tomography and modelling
Cracking predictions of lithium-ion battery electrodes by X-ray computed tomography and modelling Open
Fracture of lithium-ion battery electrodes is found to contribute to capacity fade and reduce the lifespan of a battery. Traditional fracture models for batteries are restricted to consideration of a single, idealised particle; here, advan…
View article: Applications of advanced metrology for understanding the effects of drying temperature in the lithium-ion battery electrode manufacturing process
Applications of advanced metrology for understanding the effects of drying temperature in the lithium-ion battery electrode manufacturing process Open
The performance of lithium-ion batteries is determined by the architecture and properties of electrodes formed during manufacturing, particularly in the drying process when solvent is removed and the electrode structure is formed.
View article: Exploring the Influence of Porosity and Thickness on Lithium-Ion Battery Electrodes Using an Image-Based Model
Exploring the Influence of Porosity and Thickness on Lithium-Ion Battery Electrodes Using an Image-Based Model Open
View article: Cracking Predictions of Lithium-Ion Battery Electrodes by X-Ray Computed Tomography and Modelling
Cracking Predictions of Lithium-Ion Battery Electrodes by X-Ray Computed Tomography and Modelling Open
View article: Indentation of a layer on foam substrate
Indentation of a layer on foam substrate Open
View article: On the Indentation Resistance of a PC Layer on PVC Foam Substrate
On the Indentation Resistance of a PC Layer on PVC Foam Substrate Open
The indentation response of a polycarbonate face sheet bonded to a PVC foam substrate is investigated experimentally and numerically. The deformation mode involves foam crushing, and membrane stretching of the PC layer at large indenter di…