Aditya Prajapati
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View article: Best practices for in-situ and operando techniques within electrocatalytic systems
Best practices for in-situ and operando techniques within electrocatalytic systems Open
In-situ and operando techniques in heterogeneous electrocatalysis are a powerful tool used to elucidate reaction mechanisms. Ultimately, they are key in determining concrete links between a catalyst's physical/electronic structure and its …
View article: Decarbonizing nitrogen fertilizer production via the electrochemical nitrogen oxidation reaction
Decarbonizing nitrogen fertilizer production via the electrochemical nitrogen oxidation reaction Open
View article: Insights into the Electrochemical Oxidation and Reduction of Nickel Oxide Surfaces
Insights into the Electrochemical Oxidation and Reduction of Nickel Oxide Surfaces Open
Surface oxidation/reduction processes, driven by varying electrochemical potentials, can substantially impact catalyst effectiveness and, consequently, electrolyzer performance. This study combines theoretical and experimental approaches t…
View article: Assessing the Sensitivity of Pourbaix Diagrams to Computational Protocols: Electrochemical Stability of Ni Oxides as a Case Study
Assessing the Sensitivity of Pourbaix Diagrams to Computational Protocols: Electrochemical Stability of Ni Oxides as a Case Study Open
Pourbaix diagrams stand as a useful tool in assessing and visualizing materials’ electrochemical stability and are widely used for electrocatalyst design. However, their reliability hinges on the accuracy of the chemical potentials of invo…
View article: Mechanistic Insights into the Electrochemical Oxidation of 5-Hydroxymethylfurfural on a Thin Film Ni Anode
Mechanistic Insights into the Electrochemical Oxidation of 5-Hydroxymethylfurfural on a Thin Film Ni Anode Open
Oxygen evolution reaction (OER) in ambient electrolyzers consumes a significant amount of energy and yields oxygen, an inherently low-value product. Therefore, it is imperative to choose anodic reactions that can make efficient use of the …
View article: Mechanistic Insights into the Electrochemical Oxidation of 5-Hydroxymethylfurfural on a Thin-Film Ni Anode
Mechanistic Insights into the Electrochemical Oxidation of 5-Hydroxymethylfurfural on a Thin-Film Ni Anode Open
The electrochemical oxidation of alcohols is being explored as a favorable substitute for the oxygen evolution reaction owing to its capability to generate high-value products and lower overpotentials. Herein, we present a systematic inves…
View article: A Perspective on Solar-Driven Electrochemical Routes for Sustainable Methanol Production
A Perspective on Solar-Driven Electrochemical Routes for Sustainable Methanol Production Open
The transition towards sustainable and renewable energy sources is imperative in mitigating the environmental impacts of escalating global energy consumption. Methanol, with its versatile applications and potential as a clean energy carrie…
View article: Atomic Layer Deposition of Cu Electrocatalysts on Gas Diffusion Electrodes for CO<sub>2</sub> Reduction
Atomic Layer Deposition of Cu Electrocatalysts on Gas Diffusion Electrodes for CO<sub>2</sub> Reduction Open
Electrochemical reduction of CO2 using Cu catalysts enables the synthesis of C2+ products including C2H4 and C2H5OH. In this study, Cu catalysts were fabricated using plasma…
View article: Bridging fundamental science and applied science to accelerate CO2 electrolyzer scale-up
Bridging fundamental science and applied science to accelerate CO2 electrolyzer scale-up Open
View article: CO2-free high-purity ethylene from electroreduction of CO2 with 4% solar-to-ethylene and 10% solar-to-carbon efficiencies
CO2-free high-purity ethylene from electroreduction of CO2 with 4% solar-to-ethylene and 10% solar-to-carbon efficiencies Open
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View article: Reply to the ‘Comment on “Migration-assisted, moisture gradient process for ultrafast, continuous CO<sub>2</sub> capture from dilute sources at ambient conditions”’ by J. Casado, <i>Energy Environ. Sci.</i>, 2022, 10.1039/D2EE00555G
Reply to the ‘Comment on “Migration-assisted, moisture gradient process for ultrafast, continuous CO<sub>2</sub> capture from dilute sources at ambient conditions”’ by J. Casado, <i>Energy Environ. Sci.</i>, 2022, 10.1039/D2EE00555G Open
Prajapati et al. developed a novel, robust, modular and industrially-scalable CO 2 capture process that utilizes a migration-assisted moisture gradient (MAMG) process.
View article: Migration-assisted, moisture gradient process for ultrafast, continuous CO<sub>2</sub> capture from dilute sources at ambient conditions
Migration-assisted, moisture gradient process for ultrafast, continuous CO<sub>2</sub> capture from dilute sources at ambient conditions Open
An ultrafast, continuous CO 2 capture process driven by moisture gradient and electric field with low energy consumption to capture and concentrate CO 2 from dilute sources.
View article: 2D High‐Entropy Transition Metal Dichalcogenides for Carbon Dioxide Electrocatalysis
2D High‐Entropy Transition Metal Dichalcogenides for Carbon Dioxide Electrocatalysis Open
High‐entropy alloys combine multiple principal elements at a near equal fraction to form vast compositional spaces to achieve outstanding functionalities that are absent in alloys with one or two principal elements. Here, the prediction, s…
View article: Fundamental insight into electrochemical oxidation of methane towards methanol on transition metal oxides
Fundamental insight into electrochemical oxidation of methane towards methanol on transition metal oxides Open
Significance The electrochemical conversion of CH 4 to liquid fuel such as CH 3 OH offers a sustainable and environmentally benign route to utilize shale gas. This process requires controlled oxidation by optimal splitting and formation of…