Alfred Q. R. Baron
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View article: First-order phase transition driven by competing charge-order fluctuations in 1T'-TaTe$_{2}$
First-order phase transition driven by competing charge-order fluctuations in 1T'-TaTe$_{2}$ Open
First-order phase transitions, characterized by a discontinuous change in the order parameter, are intriguing phenomena in condensed matter physics. However, the underlying, material-specific, microscopic mechanisms often remain unclear. H…
View article: Incipient Ionic Conductors: Ion‐Constrained Lattices Achieving Superionic‐Like Thermal Conductivity Through Extreme Anharmonicity
Incipient Ionic Conductors: Ion‐Constrained Lattices Achieving Superionic‐Like Thermal Conductivity Through Extreme Anharmonicity Open
Phonon liquid‐like thermal conduction in the solid state enables superionic conductors to serve as efficient thermoelectric device candidates. While liquid‐like motion of ions effectively suppresses thermal conductivity ( κ ), their high m…
View article: Hybridization of lattice and charge order excitations in a superconducting cuprate
Hybridization of lattice and charge order excitations in a superconducting cuprate Open
The ubiquitous tendency of superconducting cuprates to form charge density waves (CDWs) has reignited interest in the nature of their electron-phonon interaction and its role in shaping their phase diagrams. While pronounced dispersion ano…
View article: Phonon anomaly and local distortion in iron-manganese-based Elinvar alloys
Phonon anomaly and local distortion in iron-manganese-based Elinvar alloys Open
This paper examines the phonon dispersion and static local atomic distortion of iron-manganese-based Elinvar alloys using high-resolution inelastic X-ray scattering, magnetization, neutron diffraction, and neutron total scattering. In this…
View article: First-order preemptive Ising-nematic transition in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi mathvariant="normal">K</mml:mi><mml:mn>5</mml:mn></mml:msub><mml:msub><mml:mi>Fe</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:msub><mml:mi>Ag</mml:mi><mml:mn>6</mml:mn></mml:msub><mml:msub><mml:mi>Te</mml:mi><mml:mn>10</mml:mn></mml:msub></mml:mrow></mml:math>
First-order preemptive Ising-nematic transition in Open
Employing inelastic x-ray scattering and neutron scattering techniques, we observed nematic and magnetic phase transitions with distinct characters in K5Fe4Ag6Te10. Upon cooling, the nematic order undergoes a strongly first-order phase tra…
View article: OCD -Machine learning based metrology for copper pad surface for hybrid bonding integration
OCD -Machine learning based metrology for copper pad surface for hybrid bonding integration Open
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View article: Efficient storage of sparse image data in a human-readable format
Efficient storage of sparse image data in a human-readable format Open
The modern image formats used in recent position sensitive X-ray detectors are not suited to handling sparse image data, with only a few photons per frame, and then often must store vast amounts of data (~ terabyte), even if the meaningful…
View article: Space Charge Doping Induced Band Modulation in Mono- and Bi-layer Graphene: a nano-ARPES study
Space Charge Doping Induced Band Modulation in Mono- and Bi-layer Graphene: a nano-ARPES study Open
Controlled modulation of electronic band structure in two-dimensional (2D) materials via doping is crucial for devices fabrication. For instance doped graphene has been envisaged for various applications like sensors, super-capacitors, tra…
View article: Sound Velocities of the Hydrous Iron‐Rich HH1‐Phase: Implications for Lower Mantle Seismic Heterogeneities
Sound Velocities of the Hydrous Iron‐Rich HH1‐Phase: Implications for Lower Mantle Seismic Heterogeneities Open
We investigated the compressional and shear velocities, V P and V S , of the HH1‐phase by combining the inelastic x‐ray scattering and x‐ray diffraction experiments. In the pressure range of 64.7–79.6 GPa and at room temperature, the V P a…
View article: Phonons reveal coupled cholesterol-lipid dynamics in ternary membranes
Phonons reveal coupled cholesterol-lipid dynamics in ternary membranes Open
View article: Absence of Acoustic Phonon Anomaly in a Kagome Metal with Short-ranged Structural Modulation
Absence of Acoustic Phonon Anomaly in a Kagome Metal with Short-ranged Structural Modulation Open
Kagome lattice $A$V$_3$Sb$_5$ ($A$ = K, Rb, and Cs) superconductors without magnetism from vanadium $d$-electrons are intriguing because they have a novel charge density wave (CDW) order around 90 K and display superconductivity at $\sim$3…
View article: Charge Density Fluctuations with Enhanced Superconductivity at the Proposed Nematic Quantum Critical Point
Charge Density Fluctuations with Enhanced Superconductivity at the Proposed Nematic Quantum Critical Point Open
A quantum critical point (QCP) represents a continuous phase transition at absolute zero. At the QCP of an unconventional superconductor, enhanced superconducting transition temperature and magnetic fluctuations strength are often observed…
View article: Enhanced Cryogenic Thermoelectricity in Semimetal Ta<sub>2</sub>PdSe<sub>6</sub> through Non‐Fermi Liquid‐Like Charge and Heat Transport
Enhanced Cryogenic Thermoelectricity in Semimetal Ta<sub>2</sub>PdSe<sub>6</sub> through Non‐Fermi Liquid‐Like Charge and Heat Transport Open
The thermal properties of semimetal Ta 2 PdSe 6 are studied, which exhibits a large thermoelectric power factor at low temperatures, by combining chemical substitution, transport measurements, and inelastic X‐ray scattering. A serious viol…
View article: Phonon excitations in Eu<sub>2</sub>Ir<sub>2</sub>O<sub>7</sub> probed by inelastic x-ray scattering
Phonon excitations in Eu<sub>2</sub>Ir<sub>2</sub>O<sub>7</sub> probed by inelastic x-ray scattering Open
The study of phonon dynamics and its interplay with magnetic ordering is crucial for understanding the unique quantum phases in the pyrochlore iridates. Here, through inelastic x-ray scattering on a single crystal sample of the pyrochlore …
View article: Investigating meV-scale Equilibrium Atomic Dynamics with X-Rays: focus on disordered materials
Investigating meV-scale Equilibrium Atomic Dynamics with X-Rays: focus on disordered materials Open
This paper reviews non-resonant meV-resolved inelastic x-ray scattering (IXS) as a complementary method to inelastic neutron scattering (INS). Two aspects of IXS that are notable in this context are (1) that IXS allows straightforward meas…
View article: Real-space local self-motion of protonated and deuterated water
Real-space local self-motion of protonated and deuterated water Open
We report on the self-part of the Van Hove correlation function, the correlation function describing the dynamics of a single molecule, of water and deuterated water. The correlation function is determined by transforming inelastic scatter…
View article: Collective dynamics of liquid sulphur across the polymerisation transition temperature probed by inelastic x-ray scattering
Collective dynamics of liquid sulphur across the polymerisation transition temperature probed by inelastic x-ray scattering Open
Inelastic x-ray scattering (IXS) experiments on liquid sulphur were carried out below (140 ∘ C) and above (180 ∘ C) the polymerisation temperature T λ of about 159 ∘ C to investigate changes in the collective dynamics of this unique liquid…
View article: Investigating meV-scale Equilibrium Atomic Dynamics with X-Rays
Investigating meV-scale Equilibrium Atomic Dynamics with X-Rays Open
View article: Structural and Dynamical Changes in a Gd-Co Metallic Glass by Cryogenic Rejuvenation
Structural and Dynamical Changes in a Gd-Co Metallic Glass by Cryogenic Rejuvenation Open
View article: Structural and Dynamical Changes in a Gd-Co Metallic Glass by Cryogenic Rejuvenation
Structural and Dynamical Changes in a Gd-Co Metallic Glass by Cryogenic Rejuvenation Open
To experimentally clarify the changes in structural and dynamic heterogeneities in a metallic glass (MG), Gd65Co35, by rejuvenation with a temperature cycling (cryogenic rejuvenation), high-energy x-ray diffraction (HEXRD), anomalous x-ray…
View article: PyCSFex: an extensible Python three package for calculating x-ray structure factors in complex crystals
PyCSFex: an extensible Python three package for calculating x-ray structure factors in complex crystals Open
Near-perfect diffracting crystals have many uses in x-ray optics including as monochromators, energy analyzers, and phase retarders. The usefulness of a particular Bragg reflection is often related to its angular acceptance and efficiency,…
View article: The false beat signal of a high-speed X-ray imaging detector for synchrotron radiation experiments and its elimination with a synchronized CITIUS detector
The false beat signal of a high-speed X-ray imaging detector for synchrotron radiation experiments and its elimination with a synchronized CITIUS detector Open
Recent advances in high-speed X-ray imaging detectors for synchrotron radiation experiments have enabled frame rates to exceed 10 kframes/s. The frame rates are getting closer to the revolution frequencies of the large-scale storage rings,…
View article: Anomalous Shubnikov-de Haas effect and observation of the Bloch-Grüneisen temperature in the Dirac semimetal ZrTe5
Anomalous Shubnikov-de Haas effect and observation of the Bloch-Grüneisen temperature in the Dirac semimetal ZrTe5 Open
Appearance of quantum oscillations (QO) in both thermodynamic and transport properties of metals at low temperatures is the most striking experimental consequence of the existence of a Fermi surface (FS). The frequency of these oscillation…
View article: Density deficit of Earth’s core revealed by a multimegabar primary pressure scale
Density deficit of Earth’s core revealed by a multimegabar primary pressure scale Open
An accurate pressure scale is a fundamental requirement to understand planetary interiors. Here, we establish a primary pressure scale extending to the multimegabar pressures of Earth’s core, by combined measurement of the acoustic velocit…
View article: Observation of long-range anisotropy in a vapor-deposited metallic glass
Observation of long-range anisotropy in a vapor-deposited metallic glass Open
View article: Collective excitations in a melt of fast phase change material GeCu<sub>2</sub>Te<sub>3</sub>
Collective excitations in a melt of fast phase change material GeCu<sub>2</sub>Te<sub>3</sub> Open
Inelastic x-ray scattering measurements have been carried out to investigate atomic dynamics in a melt of fast phase change material GeCu 2 Te 3 . The dynamic structure factor was analysed using the model function with three damped harmoni…
View article: Experimental observation of mesoscopic fluctuations to identify origin of thermodynamic anomalies of ambient liquid water
Experimental observation of mesoscopic fluctuations to identify origin of thermodynamic anomalies of ambient liquid water Open
We report an experimental observation of mesoscopic fluctuations underlying the thermodynamic anomalies of ambient liquid water. The combination of two sound-velocity-measurement methods with largely different frequencies, namely inelastic…
View article: Dynamic Lone Pair Expression as Chemical Bonding Origin of Giant Phonon Anharmonicity in Thermoelectric InTe
Dynamic Lone Pair Expression as Chemical Bonding Origin of Giant Phonon Anharmonicity in Thermoelectric InTe Open
Loosely bonded (“rattling”) atoms with s 2 lone pair electrons are usually associated with strong anharmonicity and unexpectedly low thermal conductivity, yet their detailed correlation remains largely unknown. Here we resolve this correla…
View article: Sound velocity of hexagonal close-packed iron to the Earth’s inner core pressure
Sound velocity of hexagonal close-packed iron to the Earth’s inner core pressure Open
View article: Data for "Sound velocity of hexagonal close-packed iron to the Earth's inner core pressure"
Data for "Sound velocity of hexagonal close-packed iron to the Earth's inner core pressure" Open
This file is the dataset used in the article "Sound velocity of hexagonal close-packed iron to the Earth's inner core pressure", Nat. Commun. 13, 7211 (2022). https://doi.org/10.1038/s41467-022-34789-2