2025-10-07
Tailoring nanoscale interfaces for perovskite–perovskite–silicon triple-junction solar cells
2025-10-07 • Jianghui Zheng, Guoliang Wang, Leiping Duan, Weiyuan Duan, Yang Jiang, Phoebe Pearce, Yijun Gao, M. A. Parvez Mahmud, Chwenhaw Liao, Tik Lun Leung,...
Abstract Triple‐junction solar cells theoretically outperform their double-junction and single‐junction counterparts in power conversion efficiency, yet practical perovskite–perovskite–silicon devices have fallen short of both theoretical limits and commercial targets. To address surface defects in the top perovskite junction, we introduce a piperazine-1,4-diium chloride treatment, which replaces less stable lithium fluoride. For interfacing the top and middle perovskite junctions, we optimize the size of gold nan…