Jyh‐Pin Chou
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View article: Engineering surface defects on layered PtTe <sub>2</sub> and PdTe <sub>2</sub> with reacting methanol
Engineering surface defects on layered PtTe <sub>2</sub> and PdTe <sub>2</sub> with reacting methanol Open
Transition metal dichalcogenides (TMDs), owing to their two-dimensional (2D) structures, could provide the largest active surface for reactions but consume minimal materials, so become potentially ideal catalysts. Structurally perfect basa…
View article: Direct and Sustainable Ammonia Synthesis from Air and Water with Sulfur-Deficient MoS<sub>2</sub> Piezocatalysts
Direct and Sustainable Ammonia Synthesis from Air and Water with Sulfur-Deficient MoS<sub>2</sub> Piezocatalysts Open
Eco-friendly ammonia (NH3) production is critical for advancing sustainable agriculture and industry. This study introduces a sustainable, cleaner approach using MoS2 nanoflowers (NFs) to synthesize NH3 dir…
View article: Enhanced Photocatalytic Performance of Halogenated Phenylacetylene-Decorated Cu<sub>2</sub>O Surfaces via Electronic Structure Modulation: A DFT and Experimental Study
Enhanced Photocatalytic Performance of Halogenated Phenylacetylene-Decorated Cu<sub>2</sub>O Surfaces via Electronic Structure Modulation: A DFT and Experimental Study Open
This study investigates the photocatalytic performance of Cu2O surfaces modified with halogen-substituted phenylacetylenes (4-XA), including 1-ethynyl-4-fluorobenzene (4-FA), 1-chloro-4-ethynylbenzene (4-CA), and 1-bromo-4-ethyn…
View article: Direct evidence of coupling between charge density wave and Kondo lattice in ferromagnet Fe5GeTe2
Direct evidence of coupling between charge density wave and Kondo lattice in ferromagnet Fe5GeTe2 Open
d-electronic heavy fermion systems have sparked interest in exploring the connection between electronic and spin degrees of freedom in Kondo systems. Nevertheless, the coexistence of charge order on a Kondo lattice has yet to be discovered…
View article: Unveiling the Flexocatalytic Potential of Wide‐Bandgap Spinel Oxides: Light‐Free Hydrogen Evolution via Strain‐Induced Polarization and Oxygen Vacancy Engineering
Unveiling the Flexocatalytic Potential of Wide‐Bandgap Spinel Oxides: Light‐Free Hydrogen Evolution via Strain‐Induced Polarization and Oxygen Vacancy Engineering Open
Wide‐bandgap spinel oxides, such as ZnAl 2 O 4 (ZAO) and ZnCr 2 O 4 (ZCO), are traditionally limited by poor electron activation under light irradiation, resulting in suboptimal photocatalytic performance. This study investigates a novel a…
View article: Surface Functionalization of Cu<sub>2</sub>O Polyhedra with Different Halide-Substituted Phenylacetylenes for Photocatalytic Activity Comparison
Surface Functionalization of Cu<sub>2</sub>O Polyhedra with Different Halide-Substituted Phenylacetylenes for Photocatalytic Activity Comparison Open
View article: Specific Cu<sub>2</sub>O surfaces for electrocatalytic oxygen reduction reaction
Specific Cu<sub>2</sub>O surfaces for electrocatalytic oxygen reduction reaction Open
Cu 2 O rhombic dodecahedra are more active towards electrochemical oxygen reduction reaction than octahedra and cubes on a carbon nanotube matrix. Density functional theory calculations provide mechanistic insights to understand this facet…
View article: One-Pot Synthesis of Tannic Acid-Au Nanoparticles for the Colorimetric Determination of Hydrogen Peroxide and Glucose
One-Pot Synthesis of Tannic Acid-Au Nanoparticles for the Colorimetric Determination of Hydrogen Peroxide and Glucose Open
This study introduces a novel one-pot method employing tannic acid (TA) to synthesize stable gold nanoparticles (TA-AuNPs), which are characterized using transmission electron microscopy, X-ray powder diffraction, and Fourier transform inf…
View article: Double‐Hollow Au@CdS Yolk@Shell Nanostructures as Superior Plasmonic Photocatalysts for Solar Hydrogen Production
Double‐Hollow Au@CdS Yolk@Shell Nanostructures as Superior Plasmonic Photocatalysts for Solar Hydrogen Production Open
Structural engineering has proven effective in tailoring the photocatalytic properties of semiconductor nanostructures. In this work, a sophisticated double‐hollow yolk@shell nanostructure composed of a plasmonic, mobile, hollow Au nanosph…
View article: Spatially Extended Charge Density Wave Switching by Nanoscale Local Manipulation in a VTe<sub>2</sub> Monolayer
Spatially Extended Charge Density Wave Switching by Nanoscale Local Manipulation in a VTe<sub>2</sub> Monolayer Open
Monolayer transition metal dichalcogenide VTe2 exhibits multiple charge density wave (CDW) phases, mainly (4 × 4) and (4 × 1). Here we report facile dynamic and tens-of-nanometer scale switching between these CDW phases with gen…
View article: Investigating the role of undercoordinated Pt sites at the surface of layered PtTe2 for methanol decomposition
Investigating the role of undercoordinated Pt sites at the surface of layered PtTe2 for methanol decomposition Open
View article: Unveiling the stacking-dependent electronic properties of 2D ultrathin rare-earth metalloxenes family LnX$_2$ (Ln = Eu, Gd, Dy; X = Ge, Si)
Unveiling the stacking-dependent electronic properties of 2D ultrathin rare-earth metalloxenes family LnX$_2$ (Ln = Eu, Gd, Dy; X = Ge, Si) Open
The studies of electronic effects in reduced dimensionality have become a frontier in nanoscience due to exotic and highly tunable character of quantum phenomena. Recently, a new class of 2D ultrathin Ln$X_2$ metalloxenes composed of a tri…
View article: Dual-plasmonic Au@Cu7S4 yolk@shell nanocrystals for photocatalytic hydrogen production across visible to near infrared spectral region
Dual-plasmonic Au@Cu7S4 yolk@shell nanocrystals for photocatalytic hydrogen production across visible to near infrared spectral region Open
View article: Enhancing Co2 Methanation Via Synergistic Multi-Valence Pd0−Pdδ+ Interactions on Tio2
Enhancing Co2 Methanation Via Synergistic Multi-Valence Pd0−Pdδ+ Interactions on Tio2 Open
View article: Unveiling the stacking-dependent electronic properties of the 2D ultrathin rare-earth metalloxenes family LnX<sub>2</sub> (Ln = Eu, Gd, Dy; X = Ge, Si)
Unveiling the stacking-dependent electronic properties of the 2D ultrathin rare-earth metalloxenes family LnX<sub>2</sub> (Ln = Eu, Gd, Dy; X = Ge, Si) Open
It is discovered that in 2D rare-earth metalloxenes the capping layer enables the modification of the stacking order within metalloxene film and induces changes in the electronic band-structure and magnetic ground-state.
View article: Incorporation of Atomic Fe-Oxide Triggers a Quantum Leap in the Co2 Methanation Performance of Ni-Hydroxide
Incorporation of Atomic Fe-Oxide Triggers a Quantum Leap in the Co2 Methanation Performance of Ni-Hydroxide Open
View article: Manipulating H2o2 Reactivity on Pristine Anatase Tio2 with Various Surface Features and Implications in Oxidation Reactions
Manipulating H2o2 Reactivity on Pristine Anatase Tio2 with Various Surface Features and Implications in Oxidation Reactions Open
View article: Single Atom Ag Bonding between Pf3t Nanocluster and Tio2 Leads the Ultra-Stable Visible-Light-Driven Photocatalytic H2 Production
Single Atom Ag Bonding between Pf3t Nanocluster and Tio2 Leads the Ultra-Stable Visible-Light-Driven Photocatalytic H2 Production Open
View article: Accurate harmonic vibrational frequencies for diatomic molecules via quantum computing
Accurate harmonic vibrational frequencies for diatomic molecules via quantum computing Open
During the noisy intermediate-scale quantum (NISQ) era, quantum computational\napproaches refined to overcome the challenge of limited quantum resources are\nhighly valuable. However, the accuracy of the molecular properties predicted by\n…
View article: Nafion/Silver Nanoparticles as an Electrochemically Sensitive Interface for the Detection of Ractopamine in Pork Liver
Nafion/Silver Nanoparticles as an Electrochemically Sensitive Interface for the Detection of Ractopamine in Pork Liver Open
Many countries have allowed farmers to feed β-adrenergic receptor agonists, such as ractopamine (Rac), to animals to improve the quality of their meat. However, Rac consumption can cause health problems for humans; thus, detecting Rac in m…
View article: X-ray quantification of oxygen groups on diamond surfaces for quantum applications
X-ray quantification of oxygen groups on diamond surfaces for quantum applications Open
Identifying the surface chemistry of diamond materials is increasingly important for device applications, especially quantum sensors. Oxygen-related termination species are widely used because they are naturally abundant, chemically stable…
View article: Dependence on Under-Coordinated Pt at the Surface of Layered PtTe2 in the Decomposition of Methanol
Dependence on Under-Coordinated Pt at the Surface of Layered PtTe2 in the Decomposition of Methanol Open
Decomposition of adsorbed methanol (CH 3 OH) was activated on under-coordinated Pt (denoted as Pt uc ), produced by removing Te, at layered PtTe 2 surface. Both dehydrogenation and C-O bond scission occurred, resulting in the formation of …
View article: Large-scale thallene film with emergent spin-polarized states mediated by tin intercalation for spintronics applications
Large-scale thallene film with emergent spin-polarized states mediated by tin intercalation for spintronics applications Open
The quantum effects confined in the ultimate two-dimensional limit are able to address the challenges and provide advances in high-performance spintronic devices. In the paper we show a successful strategy to enrich the electronic properti…
View article: Atomic Scaled Depth Correlation to the Oxygen Reduction Reaction Performance of Single Atom Ni Alloy to the NiO<sub>2</sub> Supported Pd Nanocrystal
Atomic Scaled Depth Correlation to the Oxygen Reduction Reaction Performance of Single Atom Ni Alloy to the NiO<sub>2</sub> Supported Pd Nanocrystal Open
This study demonstrates the intercalation of single‐atom Ni (Ni SA ) substantially reduces the reaction activity of Ni oxide supported Pd nanoparticle (NiO 2 /Pd) in the oxygen reduction reaction (ORR). The results indicate the transition …
View article: Enhancing Zinc Electrode Stability Through Pre-Desolvation and Accelerated Charge Transfer Via a Polyimide Interface
Enhancing Zinc Electrode Stability Through Pre-Desolvation and Accelerated Charge Transfer Via a Polyimide Interface Open
View article: Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor
Probing Spin Dynamics on Diamond Surfaces Using a Single Quantum Sensor Open
Understanding the dynamics of a quantum bit's environment is essential for the realization of practical systems for quantum information processing and metrology. We use single nitrogen-vacancy (NV) centers in diamond to study the dynamics …
View article: Ultrafast spintronics with geometric effects in non-adiabatic wave-packet dynamics
Ultrafast spintronics with geometric effects in non-adiabatic wave-packet dynamics Open
Motivated by the intriguing possibilities of steering ultrafast non-adiabatic processes through the geometric properties of bands in quantum materials by laser pulses, we extend a wave-packet transport theory, previously well-established i…
View article: Accurate and Efficient Quantum Computations of Molecular Properties Using Daubechies Wavelet Molecular Orbitals: A Benchmark Study against Experimental Data
Accurate and Efficient Quantum Computations of Molecular Properties Using Daubechies Wavelet Molecular Orbitals: A Benchmark Study against Experimental Data Open
Although quantum computation is regarded as a promising numerical method for computational quantum chemistry, current applications of quantum-chemistry calculations on quantum computers are limited to small molecules. This limitation can b…
View article: Rubbing-free liquid crystal electro-optic device based on organic single-crystal rubrene
Rubbing-free liquid crystal electro-optic device based on organic single-crystal rubrene Open
Liquid crystals (LCs) have been a vital component of modern communication and photonic technologies. However, traditional LC alignment on polyimide (PI) requires mechanically rubbing treatment to control LC orientation, suffering from dust…
View article: Surface Silicide Facilitates the Co2 Reduction Performance of Ni Oxide Supported Pd Nano-Islands
Surface Silicide Facilitates the Co2 Reduction Performance of Ni Oxide Supported Pd Nano-Islands Open