Daniel Langford
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View article: High-pressure pump–probe experiments reveal the mechanism of excited-state proton-coupled electron transfer and a shift from stepwise to concerted pathways
High-pressure pump–probe experiments reveal the mechanism of excited-state proton-coupled electron transfer and a shift from stepwise to concerted pathways Open
Chemical energy conversion and storage in natural and artificial systems rely on proton-coupled electron transfer (PCET) processes. Concerted proton-electron transfer (CPET) can provide kinetic advantages over stepwise processes (electron …
View article: Multi-material filaments for 3D printing of photoelectrocatalytic carbon nitride composites
Multi-material filaments for 3D printing of photoelectrocatalytic carbon nitride composites Open
3D printing of conductive structures via fused deposition modelling has emerged as a mainstream manufacturing technique for electrochemical devices owing to the affordability and availability of thermoplastic-carbon-based filaments. On the…
View article: Improving Photocatalytic Hydrogen Generation via Polycitric Acid‐based Carbon Nanodots
Improving Photocatalytic Hydrogen Generation via Polycitric Acid‐based Carbon Nanodots Open
Bottom‐up syntheses of carbon nanodots (CND) using solvothermal treatment of citric acid are known to afford nanometer‐sized, amorphous polycitric acid‐based materials. The addition of suitable co‐reactants in the form of in situ synthesiz…
View article: Improving Photocatalytic Hydrogen Generation via Polycitric Acid‐based Carbon Nanodots
Improving Photocatalytic Hydrogen Generation via Polycitric Acid‐based Carbon Nanodots Open
Bottom‐up syntheses of carbon nanodots (CND) using solvothermal treatment of citric acid are known to afford nanometer‐sized, amorphous polycitric acid‐based materials. The addition of suitable co‐reactants in the form of in situ synthesiz…
View article: Understanding the Visible Absorption of Electron Accepting and Donating CNDs (Small 31/2023)
Understanding the Visible Absorption of Electron Accepting and Donating CNDs (Small 31/2023) Open
Carbon Nanodots Carbon nanodots solvothermally synthesized from citric acid and formamide result in electron-rich properties upon in situ addition of NaOH, whereas otherwise electron-poor nanomaterial is obtained with reduced or oxidized c…
View article: Understanding the Visible Absorption of Electron Accepting and Donating CNDs
Understanding the Visible Absorption of Electron Accepting and Donating CNDs Open
Carbon nanodots (CNDs) synthesized from citric acid and formyl derivatives, that is, formamide, urea, or N‐ methylformamide, stand out through their broad‐range visible‐light absorbance and extraordinary photostability. Despite their poten…
View article: Spectroscopic Evidence for Ligand Substitution Reactions at the Solid–Liquid Interface of a Sub‐micrometer Gold(I) Carbene Complex
Spectroscopic Evidence for Ligand Substitution Reactions at the Solid–Liquid Interface of a Sub‐micrometer Gold(I) Carbene Complex Open
Colloidal coordination compounds in the sub‐micrometer range were synthesized from a chloro gold(I) carbene complex via the anti‐solvent procedure and stabilized by a surfactant shell of Tween 20. This compound was successfully applied as …