Insoo Ro
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Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking Open
Globally, 89% of post-consumer plastic waste is landfilled or incinerated, exacerbating environmental pollution, while less than 0.1% is chemically recycled. Polyolefin plastics, nearly half of global plastic production, can be converted i…
Tandem Catalysis for Plastic Depolymerization: <i>In Situ</i> Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis Open
Depolymerizing plastic waste through hydrogen‐based processes, such as hydrogenolysis and hydrocracking, presents a promising solution for converting plastics into liquid fuels. However, conventional hydrogen production methods rely heavil…
Unraveling the role of water in mechanism changes for economically viable catalytic plastic upcycling Open
The surge in global plastic production, reaching 400.3 million tons in 2022, has exacerbated environmental pollution, with only 11% of plastic being recycled. Catalytic recycling, particularly through hydrogenolysis and hydrocracking, offe…
Unraveling the Role of Water in Mechanism Changes for Economically Viable Catalytic Plastic Upcycling Open
The surge in global plastic production, reaching to 390.7 million tons in 2021, exacerbates environmental pollution, with only 11% of plastic being recycled. Catalytic recycling, particularly through hydrogenolysis and hydrocracking, offer…
Optimization of Low-Temperature Catalytic Cracking of Polyolefin Waste in Open-Batch Reactors Using Zeolite Beta with Controlled Intrinsic Properties Open
Environmental problems are worsening due to the complexity in managing plastic waste. Chemical recycling emerges as a pivotal technology that can suppress additional carbon introduction into the carbon cycle and provide petroleum alternati…
Interpretable machine learning framework for catalyst performance prediction and validation with dry reforming of methane Open
Conventional methods for developing heterogeneous catalysts are inefficient in time and cost, often relying on trial-and-error. The integration of machine-learning (ML) in catalysis research using data can reduce computational costs and pr…
Cover Feature: Enhanced Stability of Atomically Dispersed Pd Catalysts via Ionic Liquid Layer Deposition for Selective Acetylene Hydrogenation to Ethylene in Excess Ethylene (ChemCatChem 6/2023) Open
The Cover Feature shows highly selective and coke-resistant atomically dispersed Pd catalysts via ionic liquid (IL) layer deposition for selective acetylene hydrogenation to ethylene in excess ethylene. In their Research Article, I. Ro and…
View article: One-step production of renewable adipic acid esters from mucic acid over an Ir–ReO<sub><i>x</i></sub>/C catalyst with low Ir loading
One-step production of renewable adipic acid esters from mucic acid over an Ir–ReO<sub><i>x</i></sub>/C catalyst with low Ir loading Open
The production of adipic acid, a large-volume platform chemical, from biomass represents a petroleum-free route to manufacturing nylon and other polymers more sustainably.
Catalytic Upcycling of Plastic Waste into High Value-added Chemicals Open
Plastic is widely used in almost every sector of the modern economy owing to its low cost, durability, lightweight, and versatility. The mass use of plastic started in the 1950s and has exponentially increased ever since. Today, the world …
View article: DFT/MKM dataset for Rh-WOx pair site catalyst
DFT/MKM dataset for Rh-WOx pair site catalyst Open
All data required to build the microkinetic model of the Rh-WOx pair site catalyst for hydroformylation and hydrogenation reactions are provided here. Please refer to the READ_ME.pdf for a detailed description of the folder structure and p…
View article: DFT/MKM dataset for Rh-WOx pair site catalyst
DFT/MKM dataset for Rh-WOx pair site catalyst Open
All data required to build the microkinetic model of the Rh-WOx pair site catalyst for hydroformylation and hydrogenation reactions are provided here. Please refer to the READ_ME.pdf for a detailed description of the folder structure and p…
Synthesis of Heteroatom Rh–ReOx Atomically Dispersed Species on Al<sub>2</sub>O<sub>3</sub> and Their Tunable Catalytic Reactivity in Ethylene Hydroformylation Open
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Synthesis Gas Conversion over Rh-Based Catalysts Promoted by Fe and Mn Open
Rh/SiO2 catalysts promoted with Fe and Mn are selective for synthesis gas conversion to oxygenates and light hydrocarbons at 523 K and 580 psi. Selective anchoring of Fe and Mn species on Rh nanoparticles was accomplished by controlled sur…
Role of the Cu-ZrO<sub>2</sub> Interfacial Sites for Conversion of Ethanol to Ethyl Acetate and Synthesis of Methanol from CO<sub>2</sub> and H<sub>2</sub> Open
Well-defined Cu catalysts containing different amounts of zirconia were synthesized by controlled surface reactions (CSRs) and atomic layer deposition methods and studied for the selective conversion of ethanol to ethyl acetate and for met…