Jinlu He
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View article: Strategically Constructing Alkali‐Metal Interfacial Bridges to Boost Photocatalytic CO <sub>2</sub> Methanation on Supported Ni─Ru Bimetallic Catalysts
Strategically Constructing Alkali‐Metal Interfacial Bridges to Boost Photocatalytic CO <sub>2</sub> Methanation on Supported Ni─Ru Bimetallic Catalysts Open
Efficient photocatalytic conversion of CO 2 into CH 4 is crucial yet challenging due to the complex multi‐electron transfer processes and sluggish intermediate transformation. Herein, an innovative strategy is introduced to dramatically en…
View article: Autonomous Materials Synthesis Laboratories: Integrating Artificial Intelligence with Advanced Robotics for Accelerated Discovery
Autonomous Materials Synthesis Laboratories: Integrating Artificial Intelligence with Advanced Robotics for Accelerated Discovery Open
This comprehensive review examines the evolution of autonomous materials synthesis laboratories that integrate artificial intelligence with advanced robotics to accelerate discovery. Traditional materials development pipelines typically re…
View article: Disaster Exposure and Insomnia Severity During 7⋅20 Flood in Henan: The Moderated Mediation Model
Disaster Exposure and Insomnia Severity During 7⋅20 Flood in Henan: The Moderated Mediation Model Open
Natural disaster exposure is considered to be one of the risk factors for mental health. We investigated whether natural disaster exposure was associated with insomnia severity and the roles of catastrophizing and dark personalities in the…
View article: Mechanistic Insights into the Atomic-Level Synergy of NiRu Single-Atom Alloy on ZrO2 for Efficient Photocatalytic CO2 Methanation and Biogas Upgrading
Mechanistic Insights into the Atomic-Level Synergy of NiRu Single-Atom Alloy on ZrO2 for Efficient Photocatalytic CO2 Methanation and Biogas Upgrading Open
Atomic-level modulation of transition metal nanoparticles through single-atom hetero-doping provides a promising strategy for optimizing catalytic reaction. However, a fundamental understanding of the underlying reaction mechanism remains …
View article: Inhibiting Dissolution of Platinum with Atomic Rare Earth Bridged by Nitrogen to Boost Alkaline Hydrogen Evolution
Inhibiting Dissolution of Platinum with Atomic Rare Earth Bridged by Nitrogen to Boost Alkaline Hydrogen Evolution Open
The unfavorable water dissociation and continuous dissolution of Pt single‐atom catalysts significantly impede their practical application in alkaline anion exchange membrane water electrolyzers (AEMWEs). Herein, by integrating the electro…
View article: Non‐Radical Mediated Photocatalytic H<sub>2</sub>O<sub>2</sub> Synthesis in Conjugate‐Enhanced Phenolic Resins with Ultrafast Charge Separation
Non‐Radical Mediated Photocatalytic H<sub>2</sub>O<sub>2</sub> Synthesis in Conjugate‐Enhanced Phenolic Resins with Ultrafast Charge Separation Open
It is essential for the development of highly efficient polymeric photocatalysts for hydrogen peroxide (H 2 O 2 ) production. Nevertheless, the non‐uniform molecular structures and sluggish reaction pathway of polymeric photocatalysts lead…
View article: Non‐Radical Mediated Photocatalytic H<sub>2</sub>O<sub>2</sub> Synthesis in Conjugate‐Enhanced Phenolic Resins with Ultrafast Charge Separation
Non‐Radical Mediated Photocatalytic H<sub>2</sub>O<sub>2</sub> Synthesis in Conjugate‐Enhanced Phenolic Resins with Ultrafast Charge Separation Open
It is essential for the development of highly efficient polymeric photocatalysts for hydrogen peroxide (H 2 O 2 ) production. Nevertheless, the non‐uniform molecular structures and sluggish reaction pathway of polymeric photocatalysts lead…
View article: Triphenylamine‐Functionalized Metal Nanoclusters for Efficient and Stable Perovskite Solar Cells
Triphenylamine‐Functionalized Metal Nanoclusters for Efficient and Stable Perovskite Solar Cells Open
Reported herein is a ligand engineering strategy to develop photoelectric active metal nanoclusters (NCs) with atomic precision. Triphenylamine (TPA), a typical organic molecule in the photoelectric field, is introduced for the first time …
View article: One-pot gram-scale synthesis of robust copper nanoclusters for photocatalytic difluoroalkylarylation of alkenes
One-pot gram-scale synthesis of robust copper nanoclusters for photocatalytic difluoroalkylarylation of alkenes Open
Atomically precise copper nanoclusters have emerged as a promising class of catalysts. However, the exploration of copper nanocluster catalysts has been slow, likely because of their complicated synthesis, limited stability, and low activi…
View article: Structure Distortion Endows Copper Nanoclusters with Surface-Active Uncoordinated Sites for Boosting Catalysis
Structure Distortion Endows Copper Nanoclusters with Surface-Active Uncoordinated Sites for Boosting Catalysis Open
The utilization of structure distortion to modulate the electronic structure and alter catalytic properties of metallic nanomaterials is a well-established practice, but accurately identifying and comprehensively understanding these distor…
View article: Comprehensive and practical guidelines for reduction synthesis of atomically precise coinage–metal nanoclusters
Comprehensive and practical guidelines for reduction synthesis of atomically precise coinage–metal nanoclusters Open
As a model system for studying the structure–property relationship and surface coordination chemistry of metal nanomaterials, ligand-stabilized, atomically precise coinage–metal (Au, Ag, and Cu) nanoclusters (NCs) have attracted considerab…
View article: Converting Undesirable Defects into Activity Sites Enhances the Photoelectrochemical Performance of The ZnIn<sub>2</sub>S<sub>4</sub> Photoanode
Converting Undesirable Defects into Activity Sites Enhances the Photoelectrochemical Performance of The ZnIn<sub>2</sub>S<sub>4</sub> Photoanode Open
Heteroatom doping can tune the band structure of semiconductors and enhance their carrier transfer capacity for improving the performance of photoelectrochemical water oxidation. Nevertheless, the introduction of dopants is not always bene…
View article: Atomically precise Cu41 clusters as model catalysts: Open metal sites matter
Atomically precise Cu41 clusters as model catalysts: Open metal sites matter Open
Although the significance of open metal sites for controlling metal nanoparticle catalysis have been well-documented, the direct identification of authentic active sites remains a grand challenge. In this work, we report a new couple of “i…
View article: Ru-P pair sites boost charge transport in hematite photoanodes for exceeding 1% efficient solar water splitting
Ru-P pair sites boost charge transport in hematite photoanodes for exceeding 1% efficient solar water splitting Open
Fast transport of charge carriers in semiconductor photoelectrodes are a major determinant of the solar-to-hydrogen efficiency for photoelectrochemical (PEC) water slitting. While doping metal ions as single atoms/clusters in photoelectrod…
View article: Single-atomic-site platinum steers photogenerated charge carrier lifetime of hematite nanoflakes for photoelectrochemical water splitting
Single-atomic-site platinum steers photogenerated charge carrier lifetime of hematite nanoflakes for photoelectrochemical water splitting Open
Although much effort has been devoted to improving photoelectrochemical water splitting of hematite (α-Fe 2 O 3 ) due to its high theoretical solar-to-hydrogen conversion efficiency of 15.5%, the low applied bias photon-to-current efficien…
View article: Dynamic semiconductor-electrolyte interface for sustainable solar water splitting over 600 hours under neutral conditions
Dynamic semiconductor-electrolyte interface for sustainable solar water splitting over 600 hours under neutral conditions Open
Photoelectrochemical (PEC) water splitting that functions in pH-neutral electrolyte attracts increasing attention to energy demand sustainability. Here, we propose a strategy to in situ form a NiB layer by tuning the composition of the neu…
View article: An Assessment of Airborne Bacteria and Fungi in the Female Dormitory Environment: Level, Impact Factors and Dose Rate
An Assessment of Airborne Bacteria and Fungi in the Female Dormitory Environment: Level, Impact Factors and Dose Rate Open
In this study, the levels of airborne bacteria and fungi were tested in a female dormitory room; the effects of heating, relative humidity and number of occupants on indoor microorganisms were analyzed and the dose rate of exposure to micr…
View article: Antibacterial Capability of Triclosan Treated on Filter Fiber Materials
Antibacterial Capability of Triclosan Treated on Filter Fiber Materials Open
Antibacterial filtration material is an effectively control technique of airborne biological pollutant to purify indoor air. This study aims to assess the antibacterial capability of triclosan treated on three filter fiber materials: the g…
View article: Weak Distance Dependence of Hot-Electron-Transfer Rates at the Interface between Monolayer MoS<sub>2</sub> and Gold
Weak Distance Dependence of Hot-Electron-Transfer Rates at the Interface between Monolayer MoS<sub>2</sub> and Gold Open
Electron transport across the transition-metal dichalcogenide (TMD)/metal interface plays an important role in determining the performance of TMD-based optoelectronic devices. However, the robustness of this process against structural hete…
View article: Ultrafast charge transfer and recombination dynamics at the monolayer-multilayer WSe2 homojunction revealed by time-resolved photoemission electron microscopy
Ultrafast charge transfer and recombination dynamics at the monolayer-multilayer WSe2 homojunction revealed by time-resolved photoemission electron microscopy Open
Transition metal dichalcogenides (TMDs) have rapidly emerged as one of the most attractive families of two-dimensional materials due to their numerous outstanding electronic and optoelectronic properties. TMDs have layer-dependent band str…
View article: WhyOxygen Increases Carrier Lifetimes but AcceleratesDegradation of CH3NH3PbI3 under LightIrradiation: Time-Domain AbInitio Analysis
WhyOxygen Increases Carrier Lifetimes but AcceleratesDegradation of CH3NH3PbI3 under LightIrradiation: Time-Domain AbInitio Analysis Open
Exposure to oxygen and light undermines
chemical stability of metal
halide perovskites, while it surprisingly improves their optical properties.
Focusing on CH3NH3PbI3, we demonstrate
that material degradation and charge carrier lifetimes …
View article: Unravelling the effects of oxidation state of interstitial iodine and oxygen passivation on charge trapping and recombination in CH<sub>3</sub>NH<sub>3</sub>PbI<sub>3</sub> perovskite: a time-domain <i>ab initio</i> study
Unravelling the effects of oxidation state of interstitial iodine and oxygen passivation on charge trapping and recombination in CH<sub>3</sub>NH<sub>3</sub>PbI<sub>3</sub> perovskite: a time-domain <i>ab initio</i> study Open
The oxidation state of interstitial iodine and oxygen passivation control the electron–hole recombination in CH3NH3PbI3 perovskite.