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View article: Triple Radical Sorting: Aryl-Alkylation of Alkenes
Triple Radical Sorting: Aryl-Alkylation of Alkenes Open
The cross-coupling of aryl bromides with alkenes can provide access to diverse combinatorial chemical space. Two-component couplings between these partners are well-known, but three-component aryl-functionalizations of unactivated alkenes …
View article: Selective coupling in hybrid organization: Institutional logic contradiction in the context of ERP post-implementation
Selective coupling in hybrid organization: Institutional logic contradiction in the context of ERP post-implementation Open
Drawing a qualitative case study over two years during, this paper provides a detailed sociological account of the local practices and institutional logic and found out that local teams used selective coupling, which led to hybrid practice…
View article: Elevated Serum IgA at Onset of Type 1 Diabetes in Children
Elevated Serum IgA at Onset of Type 1 Diabetes in Children Open
Background. Elevated serum IgA levels have been observed in various autoimmune conditions, including type 1 diabetes (T1D). However, whether children with T1D and elevated serum IgA have unique features has not been studied. We aimed to ev…
View article: Use of a Self-Contained Mechanically Powered Negative Pressure Dressing Reduces Surgical Site Infection After Intestinal Stoma Reversal
Use of a Self-Contained Mechanically Powered Negative Pressure Dressing Reduces Surgical Site Infection After Intestinal Stoma Reversal Open
Background The use of closed-incision negative pressure wound therapy (ci-NPWT) has been shown to reduce postoperative wound complications and surgical site infections after stoma closures. However, use of this approach has not been widely…
View article: Alkene Dialkylation via Triple Radical Sorting
Alkene Dialkylation via Triple Radical Sorting Open
The development of bimolecular homolytic substitution (SH2) catalysis has expanded cross-coupling logic by enabling the selective merger of any primary radical with any secondary or tertiary radical via a radical sorting mechanism. SH2 cat…
View article: Copper-Catalyzed Coupling of Alkyl Vicinal Bis(boronic Esters) to an Array of Electrophiles
Copper-Catalyzed Coupling of Alkyl Vicinal Bis(boronic Esters) to an Array of Electrophiles Open
A neighboring boronate group in the substrate provides a dramatic rate acceleration in transmetalation to copper and thereby enables organoboronic esters to participate in unprecedented site-selective cross-couplings. This cross-coupling o…
View article: Alcohols as Alkylating Agents: Photoredox‐Catalyzed Conjugate Alkylation via In Situ Deoxygenation
Alcohols as Alkylating Agents: Photoredox‐Catalyzed Conjugate Alkylation via In Situ Deoxygenation Open
The rapid exploration of sp 3 ‐enriched chemical space is facilitated by fragment‐coupling technologies that utilize simple and abundant alkyl precursors, among which alcohols are a highly desirable, commercially accessible, and synthetica…
View article: Diastereo‐ and Enantioselective 1,4‐Difunctionalization of Borylenynes by Catalytic Conjunctive Cross‐Coupling
Diastereo‐ and Enantioselective 1,4‐Difunctionalization of Borylenynes by Catalytic Conjunctive Cross‐Coupling Open
Enantioselective conjunctive cross‐coupling of enyne‐derived boronate complexes occurs with 1,4 addition of the electrophile and migrating group across the π system. This reaction pathway furnishes α‐boryl allenes as the reaction product. …
View article: Gray Matter Age Prediction as a Biomarker for Risk of Dementia
Gray Matter Age Prediction as a Biomarker for Risk of Dementia Open
Significance The difference between brain age estimated from MRI and chronological age is thought to serve as an important biomarker reflecting pathological processes in the brain. Several recent studies showed the relation between acceler…
View article: O2‐02‐05: PREDICTING BRAIN AGE AS A BIOMARKER FOR RISK OF DEMENTIA
O2‐02‐05: PREDICTING BRAIN AGE AS A BIOMARKER FOR RISK OF DEMENTIA Open
The gap between predicted brain age using magnetic resonance imaging (MRI) and chronological age may serve as biomarker for dementia. We aimed to investigate the utility of such a gap as a risk biomarker for incident dementia in a general …
View article: HIERARCHICAL TASK NETWORK APPROACH FOR TIME AND BUDGET CONSTRAINED CONSTRUCTION PROJECT PLANNING
HIERARCHICAL TASK NETWORK APPROACH FOR TIME AND BUDGET CONSTRAINED CONSTRUCTION PROJECT PLANNING Open
Completing a construction project on time and within budget is of great importance in the construction industry. To achieve this goal, a construction plan satisfying the time and cost constraints is crucial. While a rich amount of literatu…
View article: Grey Matter Age Prediction as a Biomarker for Risk of Dementia: A Population-based Study
Grey Matter Age Prediction as a Biomarker for Risk of Dementia: A Population-based Study Open
Key Points Question Is the gap between brain age predicted from MRI and chronological age associated with incident dementia in a general population of Dutch adults? Findings Brain age was predicted using a deep learning model, using MRI-de…