Kunpeng Cui
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View article: Flaw Sensitivity of Tough and Self-Healing Hydrogels with Hierarchical Structure
Flaw Sensitivity of Tough and Self-Healing Hydrogels with Hierarchical Structure Open
View article: Synchrotron Radiation X-ray Scattering Approaching Real Industrial Processing of Polymer
Synchrotron Radiation X-ray Scattering Approaching Real Industrial Processing of Polymer Open
View article: Second-Order Regularity for Degenerate Parabolic Quasi-Linear Equations in the Heisenberg Group
Second-Order Regularity for Degenerate Parabolic Quasi-Linear Equations in the Heisenberg Group Open
In the Heisenberg group Hn, we obtain the local second-order HWloc2,2-regularity for the weak solution u to a class of degenerate parabolic quasi-linear equations ∂tu=∑i=12nXiAi(Xu) modeled on the parabolic p-Laplacian equation. Specifical…
View article: Mechanisms Governing Crack Speed in Peridynamic Model
Mechanisms Governing Crack Speed in Peridynamic Model Open
View article: Role of hierarchy structure on the mechanical adaptation of self-healing hydrogels under cyclic stretching
Role of hierarchy structure on the mechanical adaptation of self-healing hydrogels under cyclic stretching Open
Soft materials with mechanical adaptability have substantial potential for various applications in tissue engineering. Gaining a deep understanding of the structural evolution and adaptation dynamics of soft materials subjected to cyclic s…
View article: Effect of Salt on Dynamic Mechanical Behaviors of Polyampholyte Hydrogels
Effect of Salt on Dynamic Mechanical Behaviors of Polyampholyte Hydrogels Open
Understanding the dynamic mechanical behaviors of tough hydrogels with ionic dynamic bonds in saline solution is crucial for applications, particularly in the biomedical field. In this work, using polyampholyte hydrogels, dually crosslinke…
View article: Load transfer between permanent and dynamic networks due to stress gradients in nonlinear viscoelastic hydrogels
Load transfer between permanent and dynamic networks due to stress gradients in nonlinear viscoelastic hydrogels Open
View article: Force-triggered rapid microstructure growth on hydrogel surface for on-demand functions
Force-triggered rapid microstructure growth on hydrogel surface for on-demand functions Open
View article: Mechanism of temperature-induced asymmetric swelling and shrinking kinetics in self-healing hydrogels
Mechanism of temperature-induced asymmetric swelling and shrinking kinetics in self-healing hydrogels Open
Understanding the physical principle that governs the stimuli-induced swelling and shrinking kinetics of hydrogels is indispensable for their applications. Here, we show that the shrinking and swelling kinetics of self-healing hydrogels co…
View article: Instantaneous micropatterning of a double-network hydrogel surface triggered by mechanical force
Instantaneous micropatterning of a double-network hydrogel surface triggered by mechanical force Open
Instantaneous patterning on soft material surfaces, such as hydrogels, is important in various research fields; however, it is extremely challenging. Existing strategies for soft material surface patterning are time-consuming and have poor…
View article: Structure Frustration Enables Thermal History-Dependent Responsive Behavior in Self-Healing Hydrogels
Structure Frustration Enables Thermal History-Dependent Responsive Behavior in Self-Healing Hydrogels Open
Biological soft tissues usually execute their functions via nonequilibrium and dynamic structural transformations. By contrast, functional hydrogels are mainly constructed by implementing static and equilibrium structures in the polymer ne…
View article: Facile preparation of cellulose hydrogel with Achilles tendon-like super strength through aligning hierarchical fibrous structure
Facile preparation of cellulose hydrogel with Achilles tendon-like super strength through aligning hierarchical fibrous structure Open
The extreme mechanical strength of fibrous connective tissues in the human body, such as ligaments and ten-dons, has always been challenging for hydrogel scientists. Here, we created extremely strong, purely cellulose -based hydrogels (DCC…
View article: Effect of mesoscale phase contrast on fatigue-delaying behavior of self-healing hydrogels
Effect of mesoscale phase contrast on fatigue-delaying behavior of self-healing hydrogels Open
The multilevel fatigue resistance mechanism of tough and self-healing hydrogels with a hierarchical structure was revealed.
View article: Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel
Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel Open
Significance Tough soft materials usually show strain softening. Avoiding strain softening, although important for practical application, had not been a focus of research. Recently, a series of tough hydrogels made from hyperconnective phy…
View article: High-Fidelity Hydrogel Thin Films Processed from Deep Eutectic Solvents
High-Fidelity Hydrogel Thin Films Processed from Deep Eutectic Solvents Open
Polyampholyte (PA) hydrogels are a fascinating class of soft materials that can exhibit high toughness while retaining self-healing characteristics. This behavior results from the random distribution of oppositely charged monomers along th…
View article: Hydrogels as dynamic memory with forgetting ability
Hydrogels as dynamic memory with forgetting ability Open
Significance Life provides the best demonstration of complex and adaptive nonequilibrium system, which executes biological functions through nonequilibrium structure transformation. Creating lifelike materials to achieve part of or full bi…
View article: Lamellar Bilayer to Fibril Structure Transformation of Tough Photonic Hydrogel under Elongation
Lamellar Bilayer to Fibril Structure Transformation of Tough Photonic Hydrogel under Elongation Open
Synthetic hydrogels possessing both macroscopic anisotropic structure and toughness, which are analogous to the load-bearing bio-tissues such as muscles and tendons, are rarely available. Studying the molecular mechanism of tough and aniso…
View article: Mesoscale bicontinuous networks in self-healing hydrogels delay fatigue fracture
Mesoscale bicontinuous networks in self-healing hydrogels delay fatigue fracture Open
Significance Muscles, composed of exquisite hierarchical structures, exhibit high fatigue resistance and can resist crack propagation even after injury. The mechanism of the hierarchical structures on suppressing crack advance under recipr…
View article: Relaxation Dynamics and Underlying Mechanism of a Thermally Reversible Gel from Symmetric Triblock Copolymer
Relaxation Dynamics and Underlying Mechanism of a Thermally Reversible Gel from Symmetric Triblock Copolymer Open
We report a novel thermally responsive system from poly(butyl methacrylate)-b-poly(methacrylic acid)-b-poly(butyl methacrylate) (PBMA-b-PMAA-b-PBMA) triblock copolymer in dimethylformamide (DMF) solvent. This system shows a sol–gel transit…
View article: Effect of Structure Heterogeneity on Mechanical Performance of Physical Polyampholytes Hydrogels
Effect of Structure Heterogeneity on Mechanical Performance of Physical Polyampholytes Hydrogels Open
Recent studies reported a multiscale structure in tough and self-healing hydrogels containing physical associations. For example, a type of tough and self-healing hydrogel from charge-balanced polyampholytes (PA) has a mesoscale bicontinuo…
View article: Hydrogel Membranes: Tough and Self‐Recoverable Thin Hydrogel Membranes for Biological Applications (Adv. Funct. Mater. 31/2018)
Hydrogel Membranes: Tough and Self‐Recoverable Thin Hydrogel Membranes for Biological Applications (Adv. Funct. Mater. 31/2018) Open
In article number 1801489, triblock copolymers are utilized in a non-covalent double network strategy by Tasuku Nakajima, Jian Ping Gong, and co-workers to yield 5–100 μm thin hydrogel membranes with ≈75% water content. Those semi-permeabl…
View article: Bulk Energy Dissipation Mechanism for the Fracture of Tough and Self-Healing Hydrogels
Bulk Energy Dissipation Mechanism for the Fracture of Tough and Self-Healing Hydrogels Open
Recently, many tough and self-healing hydrogels have been developed based on physical bonds as reversible sacrificial bonds. As breaking and re-forming of physical bonds are time-dependent, these hydrogels are viscoelastic and the deformat…
View article: The non-equilibrium phase diagrams of flow-induced crystallization and melting of polyethylene
The non-equilibrium phase diagrams of flow-induced crystallization and melting of polyethylene Open
Combining extensional rheology with in-situ synchrotron ultrafast x-ray scattering, we studied flow-induced phase behaviors of polyethylene (PE) in a wide temperature range up to 240 °C. Non-equilibrium phase diagrams of crystallization an…