Claire Wilson
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View article: Observing Transient Breathing States of MIL‐53 Homologues Using In Situ Single Crystal 3D Electron Diffraction
Observing Transient Breathing States of MIL‐53 Homologues Using In Situ Single Crystal 3D Electron Diffraction Open
The MIL‐53 series of metal–organic frameworks (MOFs) is considered archetypal for flexible MOFs, with desolvated materials rapidly transitioning between open and closed phases in a stepwise breathing process in response to changes in tempe…
View article: Inhibition of Metal–Support Interactions by Rare-Earth Doping in Palladium/Ceria Zirconia Three-Way Catalysts
Inhibition of Metal–Support Interactions by Rare-Earth Doping in Palladium/Ceria Zirconia Three-Way Catalysts Open
The impact of rare-earth (RE) doping in ceria-zirconiacritical for enhancing thermal stability and optimizing redox propertieson surface palladium (Pd) behavior has been investigated. RE doping was found to weaken metal-support interacti…
View article: Observing Transient Breathing States of MIL-53 Homologues using in situ Single Crystal 3D Electron Diffraction
Observing Transient Breathing States of MIL-53 Homologues using in situ Single Crystal 3D Electron Diffraction Open
The MIL-53 series of metal-organic frameworks (MOFs) are considered archetypal flexible MOFs, with desolvated materials rapidly transitioning between open and closed phases in a stepwise breathing process in response to changes in temperat…
View article: Enhanced barocaloric performance in neopentyl plastic crystal solid solutions
Enhanced barocaloric performance in neopentyl plastic crystal solid solutions Open
The discovery of colossal barocaloric effects in neopentyl glycol (NPG) makes plastic crystals promising candidates for solid-state refrigerants that have lower environmental impact than traditional vapour compression fluids. However, opti…
View article: COVID-19 symptom severity and duration among outpatients, July 2021-May 2023: The PROTECT observational study
COVID-19 symptom severity and duration among outpatients, July 2021-May 2023: The PROTECT observational study Open
Introduction With the emergence of new SARS-CoV-2 variants has come significant variations in disease manifestation, severity, and duration in non-hospitalized infected patients. To characterize symptom patterns and risk factors associated…
View article: Synthesis of radical-bridged lanthanide heterobimetallic complexes
Synthesis of radical-bridged lanthanide heterobimetallic complexes Open
Heteromultimetallic lanthanide (Ln) molecules are used in sensing and imaging, and have recently demonstrated Ln to-Ln energy transfer and potential as quantum logic processors. However, the selective synthesis of molecular Ln heteromultim…
View article: P-705. Non-Clinicians Effectively Perform Lung Ultrasound in Patients with Influenza-like Illness
P-705. Non-Clinicians Effectively Perform Lung Ultrasound in Patients with Influenza-like Illness Open
Background Point-of-care ultrasound (POCUS) is a low-cost, portable imaging modality with greater sensitivity than chest x-ray to evaluate acute respiratory infections including influenza-like illness (ILI). However, clinical scale has bee…
View article: P-1266. Understanding Factors that Influence Patients’ Decision to Seek Care for Flu-Like Symptoms in Emergency Departments During Seasonal Respiratory Viral Surges
P-1266. Understanding Factors that Influence Patients’ Decision to Seek Care for Flu-Like Symptoms in Emergency Departments During Seasonal Respiratory Viral Surges Open
Background Emergency departments (EDs) are directly impacted by seasonal surges in rates of respiratory viral infection and transmission with increased rates of ED visits for flu-like symptoms. It remains unclear as to why patients assigne…
View article: Clinical trials in the emergency department: Concierge coordinators to reduce attrition
Clinical trials in the emergency department: Concierge coordinators to reduce attrition Open
View article: Formation of an anthropogenic rock: mechanisms and microstructures of lithification of a legacy deposit of cementitious material
Formation of an anthropogenic rock: mechanisms and microstructures of lithification of a legacy deposit of cementitious material Open
Billions of tonnes of anthropogenic geomaterials, such as slags, ashes and cementitious materials, are deposited on the Earth's surface globally every year. These materials have the potential to become rock but little is known about how th…
View article: 1,2,5,6-Tetrathiocin as a scaffold for improved charge transport in double-cable oligothiophene systems
1,2,5,6-Tetrathiocin as a scaffold for improved charge transport in double-cable oligothiophene systems Open
Four small molecules featuring central 1,2,5,6-tetrathiocin (TTC) units fusing two oligothiophene chains have been prepared, their structures elucidated through X-ray crystallography and their charge transport properties studied in OFETs.
View article: Highly reducible polyoxometalate–Dy(III) SMM hybrid materials with exceptional charge stability
Highly reducible polyoxometalate–Dy(III) SMM hybrid materials with exceptional charge stability Open
Lanthanide single-molecule magnets (SMMs) continue to draw attention as potential building blocks for ultra-dense data storage devices due to their bistable magnetic ground states and pronounced magnetic anisotropy. To realise...
View article: Electron rich N-heterotriangulenes as host materials for OLEDs
Electron rich N-heterotriangulenes as host materials for OLEDs Open
In this work, we present a series of N-heterotriangulenes featuring electron-rich, electronically discrete bridging moieties forming distinct 3D structures. We investigate their physical properties and performance in OLED devices.
View article: Synthesis, characterization, and density functional theory of a novel Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl) pyridine)Cu(II) and polymeric Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl)pyridine)Cd(II) complexes
Synthesis, characterization, and density functional theory of a novel Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl) pyridine)Cu(II) and polymeric Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl)pyridine)Cd(II) complexes Open
View article: Synthesis, characterization and density functional theory of a novel Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl) pyridine)Cu(II) and polymeric Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3
Synthesis, characterization and density functional theory of a novel Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3-triazole-5-yl) pyridine)Cu(II) and polymeric Dichloro (2-(1-anthracene-9-ylmethyl)-1H-1,2,3 Open
View article: Polyoxometalates as advanced-performance anions for ∼<i>D</i><sub>5h</sub> Dy(<scp>iii</scp>) single-ion magnets
Polyoxometalates as advanced-performance anions for ∼<i>D</i><sub>5h</sub> Dy(<span>iii</span>) single-ion magnets Open
Enhancing single-ion magnet (SIM) magnetisation reversal barriers using a bulky polyoxometalate (POM) trianion to engineer the second coordination sphere.
View article: The charge transport properties of dicyanomethylene-functionalised violanthrone derivatives
The charge transport properties of dicyanomethylene-functionalised violanthrone derivatives Open
The study of organic small molecule semiconductor materials as active components of organic electronic devices continues to attract considerable attention due to the range of advantages these molecules can offer. Here, we report the synthe…
View article: Temperature-Dependent Structural and Optoelectronic Properties of the Layered Perovskite 2-Thiophenemethylammonium Lead Iodide
Temperature-Dependent Structural and Optoelectronic Properties of the Layered Perovskite 2-Thiophenemethylammonium Lead Iodide Open
Improved knowledge of the influence of temperature upon layered perovskites is essential to enable perovskite-based devices to operate over a broad temperature range and to elucidate the impact of structural changes upon the optoelectronic…
View article: Synthesis and Reactivity of Bis-tris(pyrazolyl)borate Lanthanide/Aluminum Heterobimetallic Trihydride Complexes
Synthesis and Reactivity of Bis-tris(pyrazolyl)borate Lanthanide/Aluminum Heterobimetallic Trihydride Complexes Open
Molecular heterobimetallic hydride complexes of lanthanide (Ln) and main-group (MG) metals exhibit chemical properties unique from their monometallic counterparts and are highly reactive species, making their synthesis and isolation challe…
View article: Table of Contents
Table of Contents Open
View article: Synthesis and reactivity of bis-tris(pyrazolyl)borate lanthanide-aluminium heterobimetallic trihydride complexes
Synthesis and reactivity of bis-tris(pyrazolyl)borate lanthanide-aluminium heterobimetallic trihydride complexes Open
Molecular heterobimetallic hydride complexes of lanthanides (Ln) and main group (MG) metals exhibit chemical properties unique from their monometallic counterparts and are highly reactive species, making their synthesis and isolation chall…
View article: CCDC 2305203: Experimental Crystal Structure Determination
CCDC 2305203: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: Synthesis of the I–K Fused Polyether Array of CTX3C and Related Ciguatoxins by Use of a Gold-Catalyzed Cyclization Reaction
Synthesis of the I–K Fused Polyether Array of CTX3C and Related Ciguatoxins by Use of a Gold-Catalyzed Cyclization Reaction Open
The I-K fragment (C31-C49) of the ciguatoxin CTX3C has been synthesized from a simple chiral pool derived tetrahydropyranyl alcohol. An efficient gold-catalyzed cyclization reaction of a γ'-hydroxy ynone has been used to accomplish efficie…
View article: Lanthanide Amide Complexes Supported by the <i>Bis</i>‐tris(pyrazolyl)borate Ligand Environment
Lanthanide Amide Complexes Supported by the <i>Bis</i>‐tris(pyrazolyl)borate Ligand Environment Open
Synthesis of primary lanthanide amides in the bis ‐hydrotris(1‐pyrazolyl)borate ligand environment has been achieved. Salt metathesis of [Dy(Tp) 2 (OTf)] 1‐Dy (OTf=CF 3 SO 3 ) with K(N′′) (N′′=N(SiMe 3 ) 2 ) in toluene yielded the [ bis (s…
View article: Activation and functionalisation of carbon dioxide by bis-tris(pyrazolyl)borate-supported divalent samarium and trivalent lanthanide silylamide complexes
Activation and functionalisation of carbon dioxide by bis-tris(pyrazolyl)borate-supported divalent samarium and trivalent lanthanide silylamide complexes Open
The activation and functionalisation of carbon dioxide by bis-tris(pyrazolyl)borate-supported divalent samarium and trivalent lanthanide silylamide complexes have been reported.
View article: Overcoming the mobility penalty introduced by dipole disorder in small-molecule HTM films
Overcoming the mobility penalty introduced by dipole disorder in small-molecule HTM films Open
Strong dipoles in molecular HTMs can cause energetic disorder, leading to reduced mobility. This can be counteracted by a preferential antiparallel dipole ordering brought about by intermolecular hydrogen bond-assisted pairing.
View article: Retraction: Synthesis of a chiral dinuclear Cu(<scp>ii</scp>)-benzothiazolamine complex: evidence of cuprophilic interaction in its structure and exploration of its electrochemical properties and catalytic performance
Retraction: Synthesis of a chiral dinuclear Cu(<span>ii</span>)-benzothiazolamine complex: evidence of cuprophilic interaction in its structure and exploration of its electrochemical properties and catalytic performance Open
Retraction of ‘Synthesis of a chiral dinuclear Cu( ii )-benzothiazolamine complex: evidence of cuprophilic interaction in its structure and exploration of its electrochemical properties and catalytic performance’ by O. Stephen Ojo et al. ,…
View article: Trifluoromethylthiolation of Arenes Using Lewis Acid and Lewis Base Dual Catalysis
Trifluoromethylthiolation of Arenes Using Lewis Acid and Lewis Base Dual Catalysis Open
Incorporation of the highly lipophilic trifluoromethanesulfenyl group into bioactive molecules facilitates transport through lipid membranes, and thus, CF3S-containing compounds are important for drug discovery. Although reagent…
View article: CCDC 2305671: Experimental Crystal Structure Determination
CCDC 2305671: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: CCDC 2267652: Experimental Crystal Structure Determination
CCDC 2267652: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …