Libao Chen
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View article: Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes
Nucleophilic Oxygen‐Engineering Dual‐Gradient Cathode‐Electrolyte‐Interphase for High‐Voltage Lithium‐Rich Manganese Oxide Cathodes Open
The high‐voltage stability of lithium‐rich manganese‐based layered oxide (LRMO), particularly at voltages approaching 4.8 V, is governed by the structure of the cathode electrolyte interphase (CEI), the oxidative stability of the electroly…
View article: Niobium–Tungsten Oxides for Ultralow‐Temperature Lithium‐Ion Batteries Operation at −60 °C
Niobium–Tungsten Oxides for Ultralow‐Temperature Lithium‐Ion Batteries Operation at −60 °C Open
Lithium‐ion batteries (LIBs) experience a notable drop in capacity and cycling stability in extremely cold environments. This decline is largely due to the low intercalation potential and the sluggish kinetics of the graphite anode. Here, …
View article: Enhanced Longevity of Lithium Metal Anodes via Fluorine/Nitrogen Co‐Doped Lightweight 3D Carbon Porous Frameworks
Enhanced Longevity of Lithium Metal Anodes via Fluorine/Nitrogen Co‐Doped Lightweight 3D Carbon Porous Frameworks Open
Lithium metal anodes suffer from uncontrollable volume expansion during electrochemical cycling due to the host‐free nature of lithium deposition, leading to reduced Coulombic efficiency (CE) and shortened cycle life. In this work, a fluor…
View article: Interweaving Covalent Organic Polymer Chains Into Two‐Dimensional Networks: Synthesis, Single Crystal Structure, and Application for Stabilizing Lithium Metal Anode
Interweaving Covalent Organic Polymer Chains Into Two‐Dimensional Networks: Synthesis, Single Crystal Structure, and Application for Stabilizing Lithium Metal Anode Open
Macroscopic weaving has been proven to be the most enduring and effective method for manufacturing fabrics to meet the practical needs of humanity for thousands of years. However, the construction of molecular structures with exquisite top…
View article: A Lithiophilic Artificial Li3P Interphase with High Li-Ion Conductivity via Solid-State Friction for Lithium Metal Anodes
A Lithiophilic Artificial Li3P Interphase with High Li-Ion Conductivity via Solid-State Friction for Lithium Metal Anodes Open
Interfacial modification strategies for lithium metal anodes have emerged as a promising method to improve cycling stability, suppress lithium dendrite growth, and increase Coulombic efficiency. However, the reported chemical synthesis met…
View article: Cathodic dehalogenation polymerization of 2′,3′,5′,6′-tetrafluoro-4,4″-diiodo-1,1′:4′,1″-terphenyl on zinc metal surface for anode protection
Cathodic dehalogenation polymerization of 2′,3′,5′,6′-tetrafluoro-4,4″-diiodo-1,1′:4′,1″-terphenyl on zinc metal surface for anode protection Open
Fluorine-containing poly(p-phenylene) (CityU-42) films on zinc surfaces were directly synthesized using a cathodic dehalogenation C-C coupling strategy. The as-prepared polymers can effectively protect the zinc substrate in aqueous zinc-io…
View article: Targeted long-read sequencing enables higher diagnostic yield of ADPKD by accurate PKD1 genetic analysis
Targeted long-read sequencing enables higher diagnostic yield of ADPKD by accurate PKD1 genetic analysis Open
Genetic diagnosis of ADPKD has been challenging due to the variant heterogeneity, presence of duplicated segments, and high GC content of exon 1 in PKD1. In our reproductive center, 40 patients were still genetically undiagnosed or diagnos…
View article: Sustainable Release of Zincophilic Metal Ions from Separator Proactively Drives Interfacial Stabilization for Durable Zinc Anode
Sustainable Release of Zincophilic Metal Ions from Separator Proactively Drives Interfacial Stabilization for Durable Zinc Anode Open
One of the important challenges in advancing aqueous zinc‐ion batteries is the separator, which is crucial for promoting stable electrode‐electrolyte interface and energy density of the battery. Herein, this study introduces a metal ion‐ac…
View article: Stereoisomeric engineering mediated zinc metal electrodeposition: Critical balance of solvation and adsorption capability
Stereoisomeric engineering mediated zinc metal electrodeposition: Critical balance of solvation and adsorption capability Open
The exceptional electrochemical performance of zinc anodes is frequently impeded by inadequate deposition kinetics and interfacial chemistry. Herein, we introduce the stereoisomerism to inform the balanced selection of electrolyte additive…
View article: Soluble Covalent Organic Frameworks as Efficient Lithiophilic Modulator for High‐Performance Lithium Metal Batteries
Soluble Covalent Organic Frameworks as Efficient Lithiophilic Modulator for High‐Performance Lithium Metal Batteries Open
Lithium metal batteries (LMBs) are regarded as the potential alternative of lithium‐ion batteries due to their ultrahigh theoretical specific capacity (3860 mAh g −1 ). However, severe instability and safety problems caused by the dendrite…
View article: Soluble Covalent Organic Frameworks as Efficient Lithiophilic Modulator for High‐Performance Lithium Metal Batteries
Soluble Covalent Organic Frameworks as Efficient Lithiophilic Modulator for High‐Performance Lithium Metal Batteries Open
Lithium metal batteries (LMBs) are regarded as the potential alternative of lithium‐ion batteries due to their ultrahigh theoretical specific capacity (3860 mAh g −1 ). However, severe instability and safety problems caused by the dendrite…
View article: Three-dimensional nanostructured composite lithium soap fibers for constructing high-performance lithium metal anode interfacial layers
Three-dimensional nanostructured composite lithium soap fibers for constructing high-performance lithium metal anode interfacial layers Open
A 3D micro–nano interface was formed on the lithium metal anode by coating composite lithium soap fibers. The Li@DA anode shows prolonged cycling lifespan due to enhanced ion conductivity and suppressed volume expansion on the interface.
View article: Engineering the solid electrolyte interphase for enhancing high-rate cycling and temperature adaptability of lithium-ion batteries
Engineering the solid electrolyte interphase for enhancing high-rate cycling and temperature adaptability of lithium-ion batteries Open
The new lithium salt additive prevents the decomposition of VN and promotes the formation of a SEI film rich in RSO 3 and LiF on the graphite electrode surface.
View article: Targeted long-read sequencing enables higher diagnostic yield of ADPKD by accurate PKD1 genetic analysis in an assisted reproductive center
Targeted long-read sequencing enables higher diagnostic yield of ADPKD by accurate PKD1 genetic analysis in an assisted reproductive center Open
Autosomal dominant polycystic kidney disease (ADPKD) is mainly caused by disease-causing variants in two large multi-exon genes of PKD1 and PKD2. Genetic diagnosis of ADPKD has been challenging due to the variant heterogeneity, presence of…
View article: Ferroelectric Dipoles Tailoring Solid‐Electrolyte‐Interphase Chemistry to Enable Reversible Lithium Metal Batteries
Ferroelectric Dipoles Tailoring Solid‐Electrolyte‐Interphase Chemistry to Enable Reversible Lithium Metal Batteries Open
Solid‐electrolyte interphase (SEI) plays a decisive role in building reliable Li metal batteries. However, the scarcity of anions in Helmholtz layer (HL) caused by electrostatic repulsion usually leads to the inferior SEI derived from solv…
View article: Ferroelectric Dipoles Tailoring Solid‐Electrolyte‐Interphase Chemistry to Enable Reversible Lithium Metal Batteries
Ferroelectric Dipoles Tailoring Solid‐Electrolyte‐Interphase Chemistry to Enable Reversible Lithium Metal Batteries Open
Solid‐electrolyte interphase (SEI) plays a decisive role in building reliable Li metal batteries. However, the scarcity of anions in Helmholtz layer (HL) caused by electrostatic repulsion usually leads to the inferior SEI derived from solv…