Luca Maggiulli
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View article: Influence of the Acid Reactivity of Carbenium Ions in Zeolites on the Methanol‐to‐Olefins Process
Influence of the Acid Reactivity of Carbenium Ions in Zeolites on the Methanol‐to‐Olefins Process Open
Carbocations are typical intermediates in acid catalyzed reactions in organic chemistry synthesis. Confinement within the framework of zeotype materials distinguishes the function of carbenium ions as catalytic centers in various chemical …
View article: Einfluss der Säurereaktivität von Carbeniumionen in Zeolithen auf den Methanol‐zu‐Olefinen‐Prozess
Einfluss der Säurereaktivität von Carbeniumionen in Zeolithen auf den Methanol‐zu‐Olefinen‐Prozess Open
Zusammenfassung Carbokationen sind typische Zwischenprodukte in säurekatalysierten Reaktionen der organischen Synthesechemie. Die Einbettung in das Gerüst zeotypischer Materialien kennzeichnet die Funktion von Carbeniumionen als katalytisc…
View article: Multiorigin and Topology-Dependent Product Selectivity in the Methanol-to-Olefins Process by Operando Transient CH<sub>3</sub>OH/CD<sub>3</sub>OD Switching Experiments
Multiorigin and Topology-Dependent Product Selectivity in the Methanol-to-Olefins Process by Operando Transient CH<sub>3</sub>OH/CD<sub>3</sub>OD Switching Experiments Open
The methanol-to-olefins (MTO) process using methanol from renewable feedstocks has attracted attention as an alternative industrial process to fuels and chemicals. MTO is characterized by a hydrocarbon pool mechanism within the pores of a …
View article: Correlating the Nature of Carbenium Ions in Zeolites to the Product Distribution in the Methanol-to-Olefins Process
Correlating the Nature of Carbenium Ions in Zeolites to the Product Distribution in the Methanol-to-Olefins Process Open
The methanol-to-olefins (MTO) process on zeolite-based catalysts enables the production of olefins from green methanol. Selectivity control requires an understanding of the nature and evolution of hydrocarbon species that act as catalytica…
View article: The Mechanism of Rapid and Green Metal–Organic Framework Synthesis by <i>In Situ</i> Spectroscopy and Diffraction
The Mechanism of Rapid and Green Metal–Organic Framework Synthesis by <i>In Situ</i> Spectroscopy and Diffraction Open
Room-temperature aqueous synthesis provides facile access to metal-organic frameworks (MOFs) through green routes, avoiding the use of toxic solvents at high temperatures that are typical for common solvothermal MOF synthesis routes. Never…
View article: Operando Spectroscopy of Catalysts Exploiting Multi-technique and Modulated Excitation Approaches
Operando Spectroscopy of Catalysts Exploiting Multi-technique and Modulated Excitation Approaches Open
Operando spectroscopy combines the in situ determination of material structure by spectroscopy/diffraction techniques with the measurement of material performance, which is conversion/selectivity in the field of heterogeneous catalysis. A …
View article: The formation, reactivity and transformation pathways of formaldehyde in the methanol-to-hydrocarbon conversion
The formation, reactivity and transformation pathways of formaldehyde in the methanol-to-hydrocarbon conversion Open
Formaldehyde, which is formed as the primary product from methanol, has a profound impact on product distribution and catalyst deactivation in the industrially-relevant methanol-to-hydrocarbons conversion.