Moritz Hoesch
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View article: Fermi surface and pseudogap in highly doped Sr2IrO4
Fermi surface and pseudogap in highly doped Sr2IrO4 Open
The fate of the Fermi surface in bulk electron-doped Sr 2 IrO 4 remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate the ele…
View article: Spin polarization of the two-dimensional electron gas at the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi mathvariant="normal">EuO/SrTiO</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub></mml:math> (001) interface
Spin polarization of the two-dimensional electron gas at the (001) interface Open
Spin-polarized two-dimensional electron gases (2DEGs) are of particular interest for functional oxide electronics applications. The redox-created 2DEG residing on the strontium titanate, SrTiO3 (STO), side of a europium monoxide (EuO)/SrTi…
View article: Percival soft X-ray CMOS Imager for Photon Science – Status and Prospects
Percival soft X-ray CMOS Imager for Photon Science – Status and Prospects Open
Percival is a CMOS-based imager with 2 megapixels, also called P2M, designed for photon science experiments. The first generation of the P2M sensor showed some performance issues. Specifically, ADCs in full-speed operation mode are affecte…
View article: Unlocking Exceptional Negative Valency and Spin Reconstruction in Non‐Collinear Anti‐Ferromagnetic Antiperovskite Mn<sub>3</sub>NiN Film
Unlocking Exceptional Negative Valency and Spin Reconstruction in Non‐Collinear Anti‐Ferromagnetic Antiperovskite Mn<sub>3</sub>NiN Film Open
Antiperovskite manganese nitrides have intriguing magnetic and electronic properties that are not well understood. Just as their perovskite oxide counterparts, they are expected to display properties tunable through epitaxial strain engine…
View article: Magnetic x-ray spectroscopy of Gd-doped EuO thin films
Magnetic x-ray spectroscopy of Gd-doped EuO thin films Open
We present a detailed x-ray magnetic circular dichroism (XMCD) study of the magnetic properties of Gd-doped EuO thin films, synthesized via molecular-beam epitaxy with Gd doping levels up to over 12%. The impact of Gd doping on the electro…
View article: Imaging Orbital Vortex Lines in Three-Dimensional Momentum Space
Imaging Orbital Vortex Lines in Three-Dimensional Momentum Space Open
We report the experimental discovery of orbital vortex lines in the three-dimensional (3D) band structure of a topological semimetal. Combining linear and circular dichroism in soft x-ray angle-resolved photoemission (SX-ARPES) with first-…
View article: Strain tuning of oxygen vacancy channels in SrCoO2.5 thin films
Strain tuning of oxygen vacancy channels in SrCoO2.5 thin films Open
Tuning of the oxygen vacancy channels (OVCs) ordering is crucial to control ionic conduction, which has much promise in energy materials and memory devices. Brownmillerite (BM) oxides have been proven to be an ideal playground for explorin…
View article: Fermi surface and pseudogap in highly doped Sr$_{2}$IrO$_{4}$
Fermi surface and pseudogap in highly doped Sr$_{2}$IrO$_{4}$ Open
The fate of the Fermi surface in bulk electron-doped Sr$_{2}$IrO$_{4}$ remains elusive, as does the origin and extension of its pseudogap phase. Here, we use high-resolution angle-resolved photoelectron spectroscopy (ARPES) to investigate …
View article: Spin polarization of the two-dimensional electron gas at the EuO/SrTiO$_3$ interface
Spin polarization of the two-dimensional electron gas at the EuO/SrTiO$_3$ interface Open
Spin-polarized two-dimensional electron gases (2DEGs) are of particular interest for functional oxide electronics applications. The redox-created 2DEG residing on the strontium titanate, SrTiO$_3$ (STO), side of a europium monoxide (EuO)/S…
View article: High-accuracy measurements of core-excited transitions in light Li-like ions
High-accuracy measurements of core-excited transitions in light Li-like ions Open
The transition energies of the two 1s core-excited soft x-ray lines (dubbed q and r) from 1s22s1S1/2 to the respective upper levels 1s(2S)2s2p(3P)2P3/2 and 2P1/2 of Li-like oxygen, fluorine, and neon were measured and calibrated u…
View article: High-accuracy Measurements of Core-excited Transitions in Light Li-like Ions
High-accuracy Measurements of Core-excited Transitions in Light Li-like Ions Open
The transition energies of the two $1s$-core-excited soft X-ray lines (dubbed q and r) from $1s^2 2s ^1S_{1/2}$ to the respective upper levels $1s(^{2}S)2s2p(^{3}P) ^{2}P_{3/2}$ and $^{2}P_{1/2}$ of Li-like oxygen, fluorine and neon were m…
View article: Chirality in the Kagome Metal CsV$_3$Sb$_5$
Chirality in the Kagome Metal CsV$_3$Sb$_5$ Open
Using x-ray photoelectron diffraction (XPD) and angle-resolved photoemission spectroscopy, we study photoemission intensity changes related to changes in the geometric and electronic structure in the kagome metal CsV$_3$Sb$_5$ upon transit…
View article: High-precision Transition Energy Measurements of Neon-like Fe xvii Ions
High-precision Transition Energy Measurements of Neon-like Fe xvii Ions Open
We improve by a factor of 4–20 the energy accuracy of the strongest soft X-ray transitions of Fe xvii ions by resonantly exciting them in an electron beam ion trap with a monochromatic beam at the P04 beamline of the PETRA III synchrotron …
View article: Natural-linewidth measurements of the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mn>3</mml:mn><mml:mi>C</mml:mi></mml:math> and <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mn>3</mml:mn><mml:mi>D</mml:mi></mml:math> soft-x-ray transitions in Ni xix
Natural-linewidth measurements of the and soft-x-ray transitions in Ni xix Open
We used the monochromatic soft-x-ray beamline P04 at the synchrotron-radiation facility PETRA III to resonantly excite the strongest 2p−3d transitions in neonlike Ni ions, [2p6]J=0→[(2p5)1/23d3/2]J=1 and [2p6]J=0→[(2p5)3/23d5/2]J=1, respec…
View article: Chirality-Driven Orbital Angular Momentum and Circular Dichroism in CoSi
Chirality-Driven Orbital Angular Momentum and Circular Dichroism in CoSi Open
Chiral crystals and molecules were recently predicted to form an intriguing platform for unconventional orbital physics. Here, we report the observation of chirality-driven orbital textures in the bulk electronic structure of CoSi, a proto…
View article: A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons
A compact approach to higher-resolution resonant inelastic x-ray scattering detection using photoelectrons Open
The detection of inelastically scattered soft x-rays with high energy resolution usually requires large grating spectrometers. Recently, photoelectron spectrometry for analysis of x-rays (PAX) has been rediscovered for modern spectroscopy …
View article: Chirality-Driven Orbital Angular Momentum and Circular Dichroism in CoSi
Chirality-Driven Orbital Angular Momentum and Circular Dichroism in CoSi Open
Chiral crystals and molecules were recently predicted to form an intriguing platform for unconventional orbital physics. Here, we report the observation of chirality-driven orbital textures in the bulk electronic structure of CoSi, a proto…
View article: A new pathway to correlate the octahedral tilt coupling and spin-orbit reconstruction at oxide interfaces
A new pathway to correlate the octahedral tilt coupling and spin-orbit reconstruction at oxide interfaces Open
The direct experimental probing and detailed imaging of octahedral tilt, along with the control of magnetic ground state and spin-orbit occupancies in an artificially engineered heterointerface through the manipulation of strain via interf…
View article: Tomographic Imaging of Orbital Vortex Lines in Three-Dimensional Momentum Space
Tomographic Imaging of Orbital Vortex Lines in Three-Dimensional Momentum Space Open
We report the experimental discovery of orbital vortex lines in the three-dimensional (3D) band structure of a topological semimetal. Combining linear and circular dichroism in soft x-ray angle-resolved photoemission (SX-ARPES) with first-…
View article: Observation of time-reversal symmetry breaking in the band structure of altermagnetic RuO <sub>2</sub>
Observation of time-reversal symmetry breaking in the band structure of altermagnetic RuO <sub>2</sub> Open
Altermagnets are an emerging elementary class of collinear magnets. Unlike ferromagnets, their distinct crystal symmetries inhibit magnetization while, unlike antiferromagnets, they promote strong spin polarization in the band structure. T…
View article: Multi-Mode Front Lens for Momentum Microscopy: Part II Experiments
Multi-Mode Front Lens for Momentum Microscopy: Part II Experiments Open
We have experimentally demonstrated different operating modes for the front lenses of the momentum microscopes described in Part I. Measurements at energies from vacuum UV at a high-harmonic generation (HHG)-based source to the soft and ha…
View article: High-Precision Transition Energy Measurements of Neon-like Fe XVII Ions
High-Precision Transition Energy Measurements of Neon-like Fe XVII Ions Open
We improve by a factor of 4-20 the energy accuracy of the strongest soft X-ray transitions of Fe XVII ions by resonantly exciting them in an electron beam ion trap with a monochromatic beam at the P04 beamline of the PETRA III synchrotron …
View article: Orbital-selective metal skin induced by alkali-metal-dosing Mott-insulating Ca2RuO4
Orbital-selective metal skin induced by alkali-metal-dosing Mott-insulating Ca2RuO4 Open
View article: Doping-Induced Electronic and Structural Phase Transition in the Bulk Weyl Semimetal Mo1-xWxTe2
Doping-Induced Electronic and Structural Phase Transition in the Bulk Weyl Semimetal Mo1-xWxTe2 Open
A comprehensive study of the electronic and structural phase transition from 1T` to Td in the bulk Weyl semimetal Mo1-xWxTe2 at different doping concentrations has been carried out using time-of-flight momentum microscopy (including circul…
View article: Fluctuation, insulation and superconductivity: the pressure-dependent phase-diagram of Rb$_2$Mo$_6$Se$_6$
Fluctuation, insulation and superconductivity: the pressure-dependent phase-diagram of Rb$_2$Mo$_6$Se$_6$ Open
The quasi-one-dimensional (q1D) material Rb$_2$Mo$_6$Se$_6$ has been proposed to display a nontrivial combination of low-dimensional fluctuations and a dynamical charge density wave (CDW) at ambient pressure. This may lead to a progressive…
View article: Active sites of Te-hyperdoped silicon by hard x-ray photoelectron spectroscopy
Active sites of Te-hyperdoped silicon by hard x-ray photoelectron spectroscopy Open
Multiple dopant configurations of Te impurities in close vicinity in silicon are investigated using photoelectron spectroscopy, photoelectron diffraction, and Bloch wave calculations. The samples are prepared by ion implantation followed b…
View article: Circular dichroism in hard X-ray photoelectron diffraction observed by time-of-flight momentum microscopy
Circular dichroism in hard X-ray photoelectron diffraction observed by time-of-flight momentum microscopy Open
View article: Active Sites of Te-hyperdoped Silicon by Hard X-ray Photoelectron Spectroscopy
Active Sites of Te-hyperdoped Silicon by Hard X-ray Photoelectron Spectroscopy Open
Multiple dopant configurations of Te impurities in close vicinity in silicon are investigated using photoelectron spectroscopy, photoelectron diffraction, and Bloch wave calculations. The samples are prepared by ion implantation followed b…
View article: New Measurement Resolves Key Astrophysical Fe XVII Oscillator Strength Problem
New Measurement Resolves Key Astrophysical Fe XVII Oscillator Strength Problem Open
One of the most enduring and intensively studied problems of x-ray astronomy is the disagreement of state-of-the art theory and observations for the intensity ratio of two Fe XVII transitions of crucial value for plasma diagnostics, dubbed…
View article: X-Ray Photoabsorption of Density-sensitive Metastable States in Ne vii, Fe xxii, and Fe xxiii
X-Ray Photoabsorption of Density-sensitive Metastable States in Ne vii, Fe xxii, and Fe xxiii Open
Metastable states of ions can be sufficiently populated in absorbing and emitting astrophysical media, enabling spectroscopic plasma-density diagnostics. Long-lived states appear in many isoelectronic sequences with an even number of elect…