Philip M. Stanley
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View article: Photochargeable Mn‐Based Metal–Organic Framework and Decoupled Photocatalysis
Photochargeable Mn‐Based Metal–Organic Framework and Decoupled Photocatalysis Open
Designing multifunctional materials that mimic the light‐dark decoupling of natural photosynthesis is a key challenge in the field of energy conversion. Herein, we introduce MnBr‐253 , a precious metal‐free metal–organic framework (MOF) bu…
View article: Durch Licht Aufladbare Mn‐Basierte Metall‐Organische Gerüstverbindungen und Davon Entkoppelte Photokatalyse
Durch Licht Aufladbare Mn‐Basierte Metall‐Organische Gerüstverbindungen und Davon Entkoppelte Photokatalyse Open
Die Entwicklung von multifunktionalen Materialien, die die Hell‐Dunkel‐Entkopplung der natürlichen Photosynthese nachahmen, ist eine zentrale Herausforderung im Bereich der Energieumwandlung. In diesem Artikel stellen wir MnBr‐253 vor, ein…
View article: Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In)
Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In) Open
Recently, several ternary phosphidotrielates and ‐tetrelates have been investigated with respect to their very good ionic conductivity, while less focus was pointed towards their electronic structures. Here, we report on a novel series of …
View article: Photocatalytic CO<sub>2</sub>‐to‐Syngas Evolution with Molecular Catalyst Metal‐organic Framework Nanozymes (Adv. Mater. 6/2023)
Photocatalytic CO<sub>2</sub>‐to‐Syngas Evolution with Molecular Catalyst Metal‐organic Framework Nanozymes (Adv. Mater. 6/2023) Open
Photocatalytic Nanozymes Highly active, efficient, and durable catalysts for light-driven carbon dioxide and water conversion to fuels are pivotal for a sustainable energy cycle. In article number 2207380, Philip M. Stanley, Julien Warnan,…
View article: Decoupled Solar Energy Storage and Dark Photocatalysis in a 3D Metal–Organic Framework (Adv. Mater. 1/2023)
Decoupled Solar Energy Storage and Dark Photocatalysis in a 3D Metal–Organic Framework (Adv. Mater. 1/2023) Open
Charge Storage Long live the electron! Solar-energy conversion and long-term storage for on-demand electrical and chemical energy are crucial toward decentralized energy distribution. In article number 2207280, Julien Warnan and co-workers…
View article: Photocatalytic CO<sub>2</sub>‐to‐Syngas Evolution with Molecular Catalyst Metal‐Organic Framework Nanozymes
Photocatalytic CO<sub>2</sub>‐to‐Syngas Evolution with Molecular Catalyst Metal‐Organic Framework Nanozymes Open
Syngas, a mixture of CO and H 2 , is a high‐priority intermediate for producing several commodity chemicals, e.g., ammonia, methanol, and synthetic hydrocarbon fuels. Accordingly, parallel sunlight‐driven catalytic conversion of CO 2 and p…
View article: Decoupled Solar Energy Storage and Dark Photocatalysis in a 3D Metal–Organic Framework
Decoupled Solar Energy Storage and Dark Photocatalysis in a 3D Metal–Organic Framework Open
Materials enabling solar energy conversion and long‐term storage for readily available electrical and chemical energy are key for off‐grid energy distribution. Herein, the specific confinement of a rhenium coordination complex in a metal–o…
View article: Topology- and wavelength-governed CO<sub>2</sub> reduction photocatalysis in molecular catalyst-metal–organic framework assemblies
Topology- and wavelength-governed CO<sub>2</sub> reduction photocatalysis in molecular catalyst-metal–organic framework assemblies Open
Two MOF molecular catalyst hybrids with differing topologies show mass and light transport governed photocatalysis. MOF-specific, irradiation wavelength-dependent product control is unlocked by switching between two energy/electron transfe…
View article: Vectorial Catalysis in Surface‐Anchored Nanometer‐Sized Metal–Organic Frameworks‐Based Microfluidic Devices
Vectorial Catalysis in Surface‐Anchored Nanometer‐Sized Metal–Organic Frameworks‐Based Microfluidic Devices Open
Vectorial catalysis—controlling multi‐step reactions in a programmed sequence and by defined spatial localization in a microscale device—is an enticing goal in bio‐inspired catalysis research. However, translating concepts from natural cas…
View article: Vektorielle Katalyse mit oberflächenverankerten nano‐metallorganischen Gerüsten in mikrofluidischen Reaktoren
Vektorielle Katalyse mit oberflächenverankerten nano‐metallorganischen Gerüsten in mikrofluidischen Reaktoren Open
Vektorielle Katalyse – die Steuerung von mehrstufigen Reaktionen in einer programmierten Abfolge und durch definierte räumliche Lokalisierung in einem mikroskaligen Reaktor – ist ein grundlegendes Ziel in der bioinspirierten Katalyseforsch…
View article: Frontispiece: Host–Guest Interactions in a Metal–Organic Framework Isoreticular Series for Molecular Photocatalytic CO<sub>2</sub> Reduction
Frontispiece: Host–Guest Interactions in a Metal–Organic Framework Isoreticular Series for Molecular Photocatalytic CO<sub>2</sub> Reduction Open
Metal–Organic Frameworks In their Communication on page 17854, Julien Warnan, Roland A. Fischer et al. report the rational engineering of a series of metal–organic frameworks for photocatalytic solar fuel production.
View article: Molecular Dye-Sensitized Photocatalysis with Metal-Organic Framework and Metal Oxide Colloids for Fuel Production
Molecular Dye-Sensitized Photocatalysis with Metal-Organic Framework and Metal Oxide Colloids for Fuel Production Open
Colloidal dye-sensitized photocatalysis is a promising route toward efficient solar fuel production by merging properties of catalysis, support, light absorption, and electron mediation in one. Metal-organic frameworks (MOFs) are host mate…
View article: Wirt‐Gast‐Wechselwirkungen in einer Serie isoretikulärer Metall‐organischer Gerüststrukturen für molekulare photokatalytische CO<sub>2</sub>‐Reduktion
Wirt‐Gast‐Wechselwirkungen in einer Serie isoretikulärer Metall‐organischer Gerüststrukturen für molekulare photokatalytische CO<sub>2</sub>‐Reduktion Open
Eine Strategie zur Verbesserung der Stabilität, Effizienz und Selektivität von homogenen molekularen Katalysatoren ist die Immobilisierung auf Trägeroberflächen oder innerhalb von Matrizes. Hier untersuchen wir die Immobilisierung des CO 2…
View article: Host–Guest Interactions in a Metal–Organic Framework Isoreticular Series for Molecular Photocatalytic CO<sub>2</sub> Reduction
Host–Guest Interactions in a Metal–Organic Framework Isoreticular Series for Molecular Photocatalytic CO<sub>2</sub> Reduction Open
A strategy to improve homogeneous molecular catalyst stability, efficiency, and selectivity is the immobilization on supporting surfaces or within host matrices. Herein, we examine the co‐immobilization of a CO 2 reduction catalyst [ReBr(C…
View article: Decoding DNA data storage for investment
Decoding DNA data storage for investment Open