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View article: Interfacial Co‐Operativity Enables Ultrafast Charge Transfer Within the Co‐Fe Prussian Blue Analogue|Zno Heterostructure
Interfacial Co‐Operativity Enables Ultrafast Charge Transfer Within the Co‐Fe Prussian Blue Analogue|Zno Heterostructure Open
Heterostructures of Cobalt‐Iron (Co‐Fe) Prussian blue analogues (PBA) and inorganic semiconductors are attractive materials for photocatalytic and photoelectrochemical water oxidation. Their efficiency is rooted in the charge transfer (CT)…
View article: Photocatalytic Oxygen Evolution with Prussian Blue Coated ZnO Origami Core‐Shell Nanostructures
Photocatalytic Oxygen Evolution with Prussian Blue Coated ZnO Origami Core‐Shell Nanostructures Open
The design and development of particulate photocatalysts have been an attractive strategy to incorporate earth‐abundant metal ions to water splitting devices. Herein, we synthesized CoFe‐Prussian blue (PB) coated ZnO origami core‐shell nan…
View article: Probing the Interfacial Molecular Structure of a Co‐Prussian Blue In Situ (Adv. Mater. Interfaces 20/2024)
Probing the Interfacial Molecular Structure of a Co‐Prussian Blue In Situ (Adv. Mater. Interfaces 20/2024) Open
Charge Transfer Process Surface-specific in situ VSFG spectroscopy elucidated the compositional and electronic evolution of a Co-PBA interfaces during electrochemical oxidation of the material. This is a happy pairing of nonlinear VSFG spe…
View article: Probing the Interfacial Molecular Structure of a Co‐Prussian Blue In Situ
Probing the Interfacial Molecular Structure of a Co‐Prussian Blue In Situ Open
Molecular‐level insight into the interfacial composition of electrodes at the solid‐electrolyte and the solid‐electrode interface is essential to understanding the charge transfer processes, which are vital for electrochemical (EC) and pho…
View article: Charge Transfer Dynamics in Organic–Inorganic Hybrid Heterostructures—Insights by Vibrational‐Sum Frequency Generation Spectroscopy
Charge Transfer Dynamics in Organic–Inorganic Hybrid Heterostructures—Insights by Vibrational‐Sum Frequency Generation Spectroscopy Open
Organic‐inorganic heterostructures play a pivotal role in modern electronic and optoelectronic applications including photodetectors and field effect transistors, as well as in solar energy conversion such as photoelectrodes of dye‐sensiti…
View article: Cover Feature: Studying Molecular Rearrangement of P1 Dye at a Passivating Alumina Surface Using Vibrational Sum‐Frequency Generation Spectroscopy: Effect of Atomic‐Level Roughness (ChemPhysChem 18/2023)
Cover Feature: Studying Molecular Rearrangement of P1 Dye at a Passivating Alumina Surface Using Vibrational Sum‐Frequency Generation Spectroscopy: Effect of Atomic‐Level Roughness (ChemPhysChem 18/2023) Open
The Cover Feature illustrates surface-sensitive probing of a molecularly functionalized model photoelectrode with vibrational sum frequency generation (VSFG) spectroscopy. VSFG spectroscopy unravels the effect of the surface roughness on t…
View article: Studying Molecular Rearrangement of P1 Dye at a Passivating Alumina Surface Using Vibrational Sum‐Frequency Generation Spectroscopy: Effect of Atomic‐Level Roughness
Studying Molecular Rearrangement of P1 Dye at a Passivating Alumina Surface Using Vibrational Sum‐Frequency Generation Spectroscopy: Effect of Atomic‐Level Roughness Open
The effect of roughness and thickness of alumina layers, mimicking the passivation layer commonly used in dye‐sensitized photoelectrodes, on the molecular adsorption of P1 dye, 4‐(bi(4‐(2,2‐dicyano‐vinyl)‐thiophene‐2‐yl]‐phenyl]‐aminobenzo…
View article: Frontispiece: A Happy Get‐Together – Probing Electrochemical Interfaces by Non‐Linear Vibrational Spectroscopy
Frontispiece: A Happy Get‐Together – Probing Electrochemical Interfaces by Non‐Linear Vibrational Spectroscopy Open
Electrochemical interfaces are key structures in energy storage and catalysis. Hence, a molecular understanding of the active sites at these interfaces, their solvation, the structure of adsorbates, and the formation of solid-electrolyte i…
View article: A Happy Get‐Together – Probing Electrochemical Interfaces by Non‐Linear Vibrational Spectroscopy
A Happy Get‐Together – Probing Electrochemical Interfaces by Non‐Linear Vibrational Spectroscopy Open
Electrochemical interfaces are key structures in energy storage and catalysis. Hence, a molecular understanding of the active sites at these interfaces, their solvation, the structure of adsorbates, and the formation of solid‐electrolyte i…
View article: Not that innocent – ammonium ions boost homogeneous light-driven hydrogen evolution
Not that innocent – ammonium ions boost homogeneous light-driven hydrogen evolution Open
We report that the homogeneous light-driven hydrogen evolution reaction (HER) can be significantly enhanced by the presence of seemingly innocent ammonium (NH4+) cations. Expermiental studies with different catalysts, photosensitizers and …
View article: Frontispiece: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex
Frontispiece: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex Open
CO2 Valorization In their Research Article on page 10527 ff., S. Roy,W. Schöfberger et al. demonstrate the electrocatalytic reduction of CO2 to acetic acid by a molecular manganese corrole complex, and propose the formation and reduction o…
View article: Frontispiz: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex
Frontispiz: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex Open
CO2-Verwertung Im Forschungsartikel auf S. 10614 ff. beschreiben S. Roy, W. Schöfberger et al. die elektrokatalytische Reduktion von CO2 zu Essigsäure durch einen molekulare Mangan-Corrolkomplex. Die Bildung und Reduktion einer Oxalat-Zwis…
View article: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex
Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex Open
The controlled electrochemical reduction of carbon dioxide to value added chemicals is an important strategy in terms of renewable energy technologies. Therefore, the development of efficient and stable catalysts in an aqueous environment …
View article: Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex
Electrocatalytic Reduction of CO<sub>2</sub> to Acetic Acid by a Molecular Manganese Corrole Complex Open
The controlled electrochemical reduction of carbon dioxide to value added chemicals is an important strategy in terms of renewable energy technologies. Therefore, the development of efficient and stable catalysts in an aqueous environment …