Run‐Han Li
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View article: Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity
Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity Open
The transfer path of photogenerated charges greatly affects the final photocatalytic performance, but this important fact has not been clearly demonstrated experimentally. Here, we construct an ultrastable crystalline catalytic system incl…
View article: Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity
Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity Open
The transfer path of photogenerated charges greatly affects the final photocatalytic performance, but this important fact has not been clearly demonstrated experimentally. Here, we construct an ultrastable crystalline catalytic system incl…
View article: Conjugated phthalocyanine-based framework as artificial SEI for over 400 Wh kg−1 lithium-metal battery
Conjugated phthalocyanine-based framework as artificial SEI for over 400 Wh kg−1 lithium-metal battery Open
High-voltage lithium-metal batteries (HVLMBs) are appealing candidates for next-generation high-energy rechargeable batteries, but their practical applications are still limited by the severe capacity degradation, attributed to the poor in…
View article: Solid‐Liquid‐Gas Three‐Phase Indirect Electrolysis Enabled by Affinity Auxiliary Imparted Covalent Organic Frameworks
Solid‐Liquid‐Gas Three‐Phase Indirect Electrolysis Enabled by Affinity Auxiliary Imparted Covalent Organic Frameworks Open
The design of efficient heterogeneous redox mediators with favorable affinity to substrate and electrolyte are much desired yet still challenging for the development of indirect electrolysis system. Herein, for the first time, we have deve…
View article: In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production
In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production Open
Photocatalytic hydrogen production is one of the most valuable technologies in the future energy system. Here, we designed a metal‐covalent organic frameworks (MCOFs) with both small‐sized metal clusters and nitrogen‐rich ligands, named CO…
View article: In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production
In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production Open
Photocatalytic hydrogen production is one of the most valuable technologies in the future energy system. Here, we designed a metal‐covalent organic frameworks (MCOFs) with both small‐sized metal clusters and nitrogen‐rich ligands, named CO…
View article: Research on ballistic performance of green shear thickening functionalized fabric based on solid waste modification
Research on ballistic performance of green shear thickening functionalized fabric based on solid waste modification Open
Based on the solid waste-based modification, green shear-thickening functionalized ballistic composites were prepared. Silica aerosols were obtained from solid waste diatomaceous earth through sol–gel preparation, gel aging, and supercriti…
View article: Photochromic radical states in 3D covalent organic frameworks with zyg topology for enhanced photocatalysis
Photochromic radical states in 3D covalent organic frameworks with zyg topology for enhanced photocatalysis Open
Covalent-organic frameworks (COFs) with photoinduced donor-acceptor (D-A) radical pairs show enhanced photocatalytic activity in principle. However, achieving long-lived charge separation in COFs proves challenging due to the rapid charge …
View article: A Solvent-free Processed Low-temperature Tolerant Adhesive
A Solvent-free Processed Low-temperature Tolerant Adhesive Open
Ultra-low temperature resistant adhesive is highly desired yet scarce for material adhesion for the potential usage in Arctic/Antarctic or outer space exploration. Here we develop a solvent-free processed low-temperature tolerant adhesive …
View article: Bridging the Homogeneous and Heterogeneous Catalysis by Supramolecular Metal‐Organic Cages with Varied Packing Modes
Bridging the Homogeneous and Heterogeneous Catalysis by Supramolecular Metal‐Organic Cages with Varied Packing Modes Open
Integrating the advantages of homogeneous and heterogeneous catalysis has proved to be an optimal strategy for developing catalytic systems with high efficiency, selectivity, and recoverability. Supramolecular metal‐organic cages (MOCs), a…
View article: Photocatalytic aerobic oxidation of C(sp3)-H bonds
Photocatalytic aerobic oxidation of C(sp3)-H bonds Open
In modern industries, the aerobic oxidation of C(sp 3 )-H bonds to achieve the value-added conversion of hydrocarbons requires high temperatures and pressures, which significantly increases energy consumption and capital investment. The de…
View article: Green synthesis of bifunctional phthalocyanine-porphyrin COFs in water for efficient electrocatalytic CO2 reduction coupled with methanol oxidation
Green synthesis of bifunctional phthalocyanine-porphyrin COFs in water for efficient electrocatalytic CO2 reduction coupled with methanol oxidation Open
Electrocatalytic CO2 reduction (ECR) coupled with organic oxidation is a promising strategy to produce high value-added chemicals and improve energy efficiency. However, achieving the efficient redox coupling reaction is still challenging …
View article: CCDC 2233756: Experimental Crystal Structure Determination
CCDC 2233756: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: CCDC 2233755: Experimental Crystal Structure Determination
CCDC 2233755: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: CCDC 2233757: Experimental Crystal Structure Determination
CCDC 2233757: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: Molecular oxidation-reduction junctions for artificial photosynthetic overall reaction
Molecular oxidation-reduction junctions for artificial photosynthetic overall reaction Open
Constructing redox semiconductor heterojunction photocatalysts is the most effective and important means to complete the artificial photosynthetic overall reaction (i.e., coupling CO 2 photoreduction and water photo-oxidation reactions). H…
View article: CCDC 2130753: Experimental Crystal Structure Determination
CCDC 2130753: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: Organoborohydride-catalyzed Chichibabin-type C4-position alkylation of pyridines with alkenes assisted by organoboranes
Organoborohydride-catalyzed Chichibabin-type C4-position alkylation of pyridines with alkenes assisted by organoboranes Open
The first NaBEt3H-catalyzed intermolecular Chichibabin-type alkylation of pyridines with alkenes as the latent nucleophiles is presented in the presence of BEt3, and a series of branched C4-alkylated pyridines were obtained in a regiospeci…