Tim Liedl
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View article: DNA Glass: Encasing Diffraction‐Quality, Mesoporous DNA Crystals in Architected Silica
DNA Glass: Encasing Diffraction‐Quality, Mesoporous DNA Crystals in Architected Silica Open
Self‐assembling DNA crystals have emerged over the last two decades as an efficient and effective means of organizing matter at the nanoscale, but functionalization of these lattices has proved challenging as physiological buffer condition…
View article: Bringing Attomolar Detection to the Point‐of‐Care with Nanopatterned DNA Origami Nanoantennas
Bringing Attomolar Detection to the Point‐of‐Care with Nanopatterned DNA Origami Nanoantennas Open
Creating increasingly sensitive and cost‐effective nucleic acid detection methods is critical for enhancing point‐of‐care (POC) applications. This requires highly specific capture of biomarkers and efficient transduction of capture events.…
View article: DNA Glass: Encasing Diffraction-Quality, Mesoporous DNA Crystals in Silica
DNA Glass: Encasing Diffraction-Quality, Mesoporous DNA Crystals in Silica Open
Self-assembling DNA crystals have emerged over the last two decades as an efficient and effective means of organizing matter at the nanoscale, but functionalization of these lattices has proved challenging as physiological buffer condition…
View article: High-endurance mechanical switching in a DNA origami snap-through mechanism
High-endurance mechanical switching in a DNA origami snap-through mechanism Open
Switchable elements are key components of dynamic technological and biological systems, enabling reversible transitions between well-defined states. Here, we present a DNA origami-based, mechanically bistable snap-through mechanism that ca…
View article: DNA origami signal amplification in lateral flow immunoassays
DNA origami signal amplification in lateral flow immunoassays Open
Lateral flow immunoassays (LFIAs) enable a rapid detection of analytes in a simple, paper-based test format. Despite their multiple advantages, such as low cost and ease of use, their low sensitivity compared to laboratory-based testing li…
View article: Self‐Assembled Physical Unclonable Function Labels Based on Plasmonic Coupling
Self‐Assembled Physical Unclonable Function Labels Based on Plasmonic Coupling Open
Counterfeiting of goods and pharmaceuticals impacts economies around the globe and threatens human health. Hardware‐based cryptography exploiting physical unclonable functions (PUFs) provides the means to securely identify and authenticate…
View article: Fabrication of Functional 3D Nanoarchitectures via Atomic Layer Deposition on DNA Origami Crystals
Fabrication of Functional 3D Nanoarchitectures via Atomic Layer Deposition on DNA Origami Crystals Open
While DNA origami is a powerful bottom-up fabrication technique, the physical and chemical stability of DNA nanostructures is generally limited to aqueous buffer conditions. Wet chemical silicification can stabilize these structures but do…
View article: Scattering-based super-resolution optical fluctuation imaging
Scattering-based super-resolution optical fluctuation imaging Open
Super-resolution optical imaging has become a prominent tool in life and material sciences, allowing one to decipher structures at increasingly greater spatial detail. Among the utilized techniques in this field, super-resolution optical f…
View article: Deterministic and Scalable Quantum Light Generation in DNA Origami-Programmed Organic Molecule-MoS$_2$ Monolayer Hybrids
Deterministic and Scalable Quantum Light Generation in DNA Origami-Programmed Organic Molecule-MoS$_2$ Monolayer Hybrids Open
The functionalization of atomically-thin transition metal dichalcogenides (TMDs) with organic molecules is a promising approach for realizing nanoscale optoelectronic devices with tailored functionalities, such as quantum light generation …
View article: Tunable dynamics of flexible magnetic microcrosses: synchronous rotation, breathing and out-of-plane arm overtaking
Tunable dynamics of flexible magnetic microcrosses: synchronous rotation, breathing and out-of-plane arm overtaking Open
We investigate the rotational dynamics of magnetically driven microcrosses. Using slender body theory, we explain the dynamical regimes observed including a breathing mode and an overtaking displaying a three-dimensional rotations.
View article: Bringing Attomolar Detection to the Point-of-Care with Nanopatterned DNA Origami Nanoantennas
Bringing Attomolar Detection to the Point-of-Care with Nanopatterned DNA Origami Nanoantennas Open
Creating increasingly sensitive and cost-effective nucleic acid detection methods is critical for enhancing point-of-care (POC) applications. This involves capturing all desired biomarkers in a sample with high specificity and transducing …
View article: Fabrication of functional 3D nanoarchitectures via atomic layer deposition on DNA origami crystals
Fabrication of functional 3D nanoarchitectures via atomic layer deposition on DNA origami crystals Open
While DNA origami is a powerful bottom-up fabrication technique, the physical and chemical stability of DNA nanostructures is generally limited to aqueous buffer conditions. Wet chemical silicification can stabilise these structures but do…
View article: Scattering-Based Super-Resolution Optical Fluctuation Imaging
Scattering-Based Super-Resolution Optical Fluctuation Imaging Open
Super-resolution optical imaging has become a prominent tool in life and material sciences, allowing one to decipher structures at increasingly greater spatial detail. Among the utilized techniques in this field, super-resolution optical f…
View article: Diamond-lattice photonic crystals assembled from DNA origami
Diamond-lattice photonic crystals assembled from DNA origami Open
Colloidal self-assembly allows rational design of structures on the micrometer and submicrometer scale. One architecture that can generate complete three-dimensional photonic bandgaps is the diamond cubic lattice, which has remained diffic…
View article: Unraveling the Chirality Transfer from Circularly Polarized Light to Single Plasmonic Nanoparticles
Unraveling the Chirality Transfer from Circularly Polarized Light to Single Plasmonic Nanoparticles Open
Due to their broken symmetry, chiral plasmonic nanostructures have unique optical properties and numerous applications. However, there is still a lack of comprehension regarding how chirality transfer occurs between circularly polarized li…
View article: Unraveling the Chirality Transfer from Circularly Polarized Light to Single Plasmonic Nanoparticles
Unraveling the Chirality Transfer from Circularly Polarized Light to Single Plasmonic Nanoparticles Open
Due to their broken symmetry, chiral plasmonic nanostructures have unique optical properties and numerous applications. However, there is still a lack of comprehension regarding how chirality transfer occurs between circularly polarized li…
View article: Cytotoxicity of Colloidal CdSe and CdSe/ZnS Nanoparticles
Cytotoxicity of Colloidal CdSe and CdSe/ZnS Nanoparticles Open
Cytotoxicity of CdSe and CdSe/ZnS nanoparticles has been investigated for different surface modifications such as coating with mercaptopropionic\nacid, silanization, and polymer coating. For all cases, quantitative values for the onset of …
View article: Size Determination of (Bio)conjugated Water-Soluble Colloidal Nanoparticles: A Comparison of Different Techniques
Size Determination of (Bio)conjugated Water-Soluble Colloidal Nanoparticles: A Comparison of Different Techniques Open
The size of inorganic colloidal nanoparticles coated with organic layers of different thickness has been measured\nwith different techniques, including transmission electron microscopy, gel electrophoresis, size exclusion\nchromatography, …
View article: Hydrophobic Nanocrystals Coated with an Amphiphilic Polymer Shell: A General Route to Water Soluble Nanocrystals
Hydrophobic Nanocrystals Coated with an Amphiphilic Polymer Shell: A General Route to Water Soluble Nanocrystals Open
A general strategy is described which allows for transferring hydrophobically capped nanocrystals from organic to aqueous solution by\nwrapping an amphiphilic polymer around the particles. In particular, high quality CoPt3, Au, …
View article: Cooperative dynamics of DNA-grafted magnetic nanoparticles optimize magnetic biosensing and coupling to DNA origami
Cooperative dynamics of DNA-grafted magnetic nanoparticles optimize magnetic biosensing and coupling to DNA origami Open
Single-stranded DNA on MNPs shows a transition from being coiled to being brushed out at low and high grafting densities, respectively. Thereby, MNPs exhibit cooperative dynamics, which is highly relevant for magnetic biosensing and bindin…
View article: Contents list
Contents list Open
View article: Hot electrons and electromagnetic effects in the broadband Au, Ag, and Ag-Au nanocrystals: The UV, visible, and NIR plasmons
Hot electrons and electromagnetic effects in the broadband Au, Ag, and Ag-Au nanocrystals: The UV, visible, and NIR plasmons Open
Energetic and optical properties of plasmonic nanocrystals strongly depend on their sizes, shapes, and composition. Whereas using plasmonic nanoparticles in biotesting has become routine, applications of plasmonics in energy are still earl…
View article: Multilayer DNA Origami with Terminal Interfaces That Are Flat and Wide-Area
Multilayer DNA Origami with Terminal Interfaces That Are Flat and Wide-Area Open
DNA origami is a popular nanofabrication strategy that employs self-assembly of a long single scaffold strand, typically less than 10 kilobases in length, with hundreds of shorter staple strands into a desired shape. In particular, origami…
View article: Accessible hotspots for single-protein SERS in DNA-origami assembled gold nanorod dimers with tip-to-tip alignment
Accessible hotspots for single-protein SERS in DNA-origami assembled gold nanorod dimers with tip-to-tip alignment Open
The label-free identification of individual proteins from liquid samples by surface-enhanced Raman scattering (SERS) spectroscopy is a highly desirable goal in biomedical diagnostics. However, the small Raman scattering cross-section of mo…
View article: Early-Career and Emerging Researchers in Physical Chemistry Volume 2
Early-Career and Emerging Researchers in Physical Chemistry Volume 2 Open
ADVERTISEMENT RETURN TO ISSUESpecial Issue Prefac...Special Issue PrefaceNEXTEarly-Career and Emerging Researchers in Physical Chemistry Volume 2Anastassia N. AlexandrovaAnastassia N. AlexandrovaMore by Anastassia N. Alexandrovahttps://orc…
View article: Early-Career and Emerging Researchers in Physical Chemistry Volume 2
Early-Career and Emerging Researchers in Physical Chemistry Volume 2 Open
ADVERTISEMENT RETURN TO ISSUESpecial Issue Prefac...Special Issue PrefaceNEXTEarly-Career and Emerging Researchers in Physical Chemistry Volume 2Anastassia N. AlexandrovaAnastassia N. AlexandrovaMore by Anastassia N. Alexandrovahttps://orc…
View article: Self-assembled physical unclonable function labels based on plasmonic coupling
Self-assembled physical unclonable function labels based on plasmonic coupling Open
Counterfeiting threatens human health, social equity, national security and global and local economies. Hardware-based cryptography that exploits physical unclonable functions (PUFs) provides the means for secure identification and authent…
View article: Diamond-lattice photonic crystals assembled from DNA origami
Diamond-lattice photonic crystals assembled from DNA origami Open
Colloidal self-assembly allows rational design of structures on the micrometer and submicrometer scale. One architecture that can generate complete 3D photonic band gaps is the diamond cubic lattice, which has remained difficult to realize…
View article: Controlling the size and adhesion of DNA droplets using surface-active DNA molecules
Controlling the size and adhesion of DNA droplets using surface-active DNA molecules Open
Liquid droplets of biomolecules serve as organizers of the cellular interior and are of interest in biosensing and biomaterials applications. Here, we investigate means to tune the interfacial properties of a model biomolecular liquid cons…
View article: Site-directed placement of three-dimensional DNA origami
Site-directed placement of three-dimensional DNA origami Open