Tyler J. Quill
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View article: Electron–ion coupling breaks energy symmetry in bistable organic electrochemical transistors
Electron–ion coupling breaks energy symmetry in bistable organic electrochemical transistors Open
Organic electrochemical transistors are extensively studied for applications ranging from bioelectronics to analog and neuromorphic computing. Despite significant advances, the fundamental interactions between the polymer semiconductor cha…
View article: Revealing the Full Potential of Mixed Ionic-Electronic Semiconductors – Avoiding Homocoupling to Boost Electrochemical Transistor Performance
Revealing the Full Potential of Mixed Ionic-Electronic Semiconductors – Avoiding Homocoupling to Boost Electrochemical Transistor Performance Open
Organic electrochemical transistors (OECTs) enable the transduction of ionic signals into electronic outputs, positioning them as ideal candidates for next-generation sensing and (bio)signal processing applications. Recent years have witne…
View article: The Influence of Alkyl Spacers and Molecular Weight on the Charge Transport and Storage Properties of Oxy‐Bithiophene‐Based Conjugated Polymers
The Influence of Alkyl Spacers and Molecular Weight on the Charge Transport and Storage Properties of Oxy‐Bithiophene‐Based Conjugated Polymers Open
Conjugated polymers (CPs) with polar side chains can conduct electronic and ionic charges simultaneously, making them promising for bioelectronics, electrocatalysis and energy storage. Recent work showed that adding alkyl spacers between C…
View article: The Influence of Alkyl Spacers and Molecular Weight on the Charge Transport and Storage Properties of Oxy‐Bithiophene‐Based Conjugated Polymers
The Influence of Alkyl Spacers and Molecular Weight on the Charge Transport and Storage Properties of Oxy‐Bithiophene‐Based Conjugated Polymers Open
Conjugated polymers (CPs) with polar side chains can conduct electronic and ionic charges simultaneously, making them promising for bioelectronics, electrocatalysis and energy storage. Recent work showed that adding alkyl spacers between C…
View article: The hierarchical structure of organic mixed ionic–electronic conductors and its evolution in water
The hierarchical structure of organic mixed ionic–electronic conductors and its evolution in water Open
View article: Repurposing mebendazole against triple-negative breast cancer CNS metastasis
Repurposing mebendazole against triple-negative breast cancer CNS metastasis Open
View article: Repurposing mebendazole against triple-negative breast cancer leptomeningeal disease
Repurposing mebendazole against triple-negative breast cancer leptomeningeal disease Open
Purpose Triple-negative breast cancer (TNBC) is an aggressive subtype that often metastasizes to the brain. Leptomeningeal disease (LMD), a devastating brain metastasis common in TNBC, has limited treatment options. We sought to test wheth…
View article: Charge Carrier Induced Structural Ordering And Disordering in Organic Mixed Ionic Electronic Conductors
Charge Carrier Induced Structural Ordering And Disordering in Organic Mixed Ionic Electronic Conductors Open
Operational stability underpins the successful application of organic mixed ionic‐electronic conductors (OMIECs) in a wide range of fields, including biosensing, neuromorphic computing, and wearable electronics. In this work, both the oper…
View article: On the Importance of Chemical Precision in Organic Electronics: Fullerene Intercalation in Perfectly Alternating Conjugated Polymers
On the Importance of Chemical Precision in Organic Electronics: Fullerene Intercalation in Perfectly Alternating Conjugated Polymers Open
The true structure of alternating conjugated polymers—the state‐of‐the‐art materials for many organic electronics—often deviates from the idealized picture. Homocoupling defects are in fact inherent to the widely used cross‐coupling polyme…
View article: Role of aggregates and microstructure of mixed-ionic–electronic-conductors on charge transport in electrochemical transistors
Role of aggregates and microstructure of mixed-ionic–electronic-conductors on charge transport in electrochemical transistors Open
OMIECs undergo structural rearrangements to accommodate ions and electronic charge carriers during which percolating networks are formed for efficient electronic charge transport.
View article: A tetrathienopyrrole-based ladder-type donor polymer for high-performance organic near-infrared cavity detectors
A tetrathienopyrrole-based ladder-type donor polymer for high-performance organic near-infrared cavity detectors Open
Ladder-type extension of a push–pull donor polymer affords enhanced peak external quantum efficiencies in microcavity organic photodetectors, with detectivities ranging from 1.07 × 10 12 to 1.82 × 10 10 Jones in the 900–1400 nm regime.
View article: Conjugated Polymers for Microwave Applications: Untethered Sensing Platforms and Multifunctional Devices
Conjugated Polymers for Microwave Applications: Untethered Sensing Platforms and Multifunctional Devices Open
In the past two decades, organic electronic materials have enabled and accelerated a large and diverse set of technologies, from energy‐harvesting devices and electromechanical actuators, to flexible and printed (opto)electronic circuitry.…
View article: Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices
Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices Open
Raw data for the manuscript "Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices". In reference to the manuscript, the dataset is organized in three subsets, each related to one of the F…
View article: Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices
Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices Open
Raw data for the manuscript "Conjugated polymers for microwave applications: untethered sensing platforms and multifunctional devices". In reference to the manuscript, the dataset is organized in three subsets, each related to one of the F…
View article: Copper-based 2D Conductive Metal Organic Framework Thin Films for Ultrasensitive Detection of Perfluoroalkyls in Drinking Water
Copper-based 2D Conductive Metal Organic Framework Thin Films for Ultrasensitive Detection of Perfluoroalkyls in Drinking Water Open
Perfluoroalkyls (PFAS) continue to emerge as a global health threat making their effective detection and capture extremely important. Though metal organic frameworks (MOF) have stood out as a promising class of porous materials for sensing…
View article: Efficient Electronic Tunneling Governs Transport in Conducting Polymer-Insulator Blends
Efficient Electronic Tunneling Governs Transport in Conducting Polymer-Insulator Blends Open
Electronic transport models for conducting polymers (CPs) and blends focus on the arrangement of conjugated chains, while the contributions of the nominally insulating components to transport are largely ignored. In this work, an archetypa…
View article: High‐Speed Ionic Synaptic Memory Based on 2D Titanium Carbide MXene (Adv. Funct. Mater. 12/2022)
High‐Speed Ionic Synaptic Memory Based on 2D Titanium Carbide MXene (Adv. Funct. Mater. 12/2022) Open
Analog Resistive Memories In article number 2109970, Armantas Melianas, Armin VahidMohammadi, Alberto Salleo, Mahiar Max Hamedi, and co-workers present the world's first electrochemical transistor memory based on 2D materials (MXene). Thes…
View article: Embedded Devices for Neuromorphic Time-Series Assessment
Embedded Devices for Neuromorphic Time-Series Assessment Open
Modern computation based on the von Neumann architecture is today a mature cutting-edge science. In the Von Neumann architecture, processing and memory units are implemented as separate blocks interchanging data intensively and continuousl…
View article: 2022 roadmap on neuromorphic computing and engineering
2022 roadmap on neuromorphic computing and engineering Open
Modern computation based on von Neumann architecture is now a mature cutting-edge science. In the von Neumann architecture, processing and memory units are implemented as separate blocks interchanging data intensively and continuously. Thi…
View article: <i>meso</i>-Ethynyl-extended push–pull type porphyrins for near-infrared organic photodetectors
<i>meso</i>-Ethynyl-extended push–pull type porphyrins for near-infrared organic photodetectors Open
Organic photodetectors prepared from meso -ethynyl-extended push–pull porphyrins afford specific detectivities over 10 11 Jones in the near-infrared range up to 1000 nm.
View article: High‐Speed Ionic Synaptic Memory Based on 2D Titanium Carbide MXene
High‐Speed Ionic Synaptic Memory Based on 2D Titanium Carbide MXene Open
Synaptic devices with linear high‐speed switching can accelerate learning in artificial neural networks (ANNs) embodied in hardware. Conventional resistive memories however suffer from high write noise and asymmetric conductance tuning, pr…
View article: Redox-Active Polymers Designed for the Circular Economy of Energy Storage Devices
Redox-Active Polymers Designed for the Circular Economy of Energy Storage Devices Open
Electrochemical energy storage is a keystone to support the rapid transition to a low-carbon-emission future for grid storage and transportation. While research on electrochemical energy storage devices has mostly dealt with performance im…
View article: Ion Pair Uptake in Ion Gel Devices Based on Organic Mixed Ionic–Electronic Conductors
Ion Pair Uptake in Ion Gel Devices Based on Organic Mixed Ionic–Electronic Conductors Open
In organic mixed ionic–electronic conductors (OMIECs), it is critical to understand the motion of ions in the electrolyte and OMIEC. Generally, the focus is on the movement of net charge during gating, and the motion of neutral anion–catio…
View article: 2021 Roadmap on Neuromorphic Computing and Engineering
2021 Roadmap on Neuromorphic Computing and Engineering Open
Modern computation based on the von Neumann architecture is today a mature cutting-edge science. In this architecture, processing and memory units are implemented as separate blocks interchanging data intensively and continuously. This dat…
View article: Temperature-resilient solid-state organic artificial synapses for neuromorphic computing
Temperature-resilient solid-state organic artificial synapses for neuromorphic computing Open
Ion gels enable temperature-stable and high-performance organic memories for integration into hardware artificial neural networks.