Tyler J. Slade
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View article: Hidden symmetry-breaking in a kagome Ising ferromagnet
Hidden symmetry-breaking in a kagome Ising ferromagnet Open
Kagome metals can host unconventional electronic phenomena that emerge from their frustrated lattice geometry and associated band topology. Correlated electronic orders, such as charge-density waves and superconductivity, are observed to i…
View article: Nature of quantum criticality in the Ising ferromagnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mrow> <mml:msub> <mml:mi>TbV</mml:mi> <mml:mn>6</mml:mn> </mml:msub> <mml:msub> <mml:mi>Sn</mml:mi> <mml:mn>6</mml:mn> </mml:msub> </mml:mrow> </mml:math>
Nature of quantum criticality in the Ising ferromagnet Open
TbV 6 Sn 6 is a topological metal where ferromagnetic Tb ions with strong uniaxial magnetic anisotropy interact with V kagome layers. Inelastic neutron scattering (INS) measurements show that the Tb ions adopt an Ising doublet grou…
View article: Suppression of the valence transition in solution-grown single crystals of Eu$_2$Pt$_6$Al$_{15}$
Suppression of the valence transition in solution-grown single crystals of Eu$_2$Pt$_6$Al$_{15}$ Open
The study of Eu intermetallic compounds has allowed the exploration of valence fluctuations and transitions in 4f electron systems. Recently, a Eu$_2$Pt$_6$Al$_{15}$ phase synthesized by arc-melting followed by a thermal treatment was repo…
View article: Superconducting dome and structural changes in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>LaRu</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mi>Si</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> under pressure
Superconducting dome and structural changes in under pressure Open
LaRu$_3$Si$_2$ is of current research interest as a kagome metal with a superconducting transition temperature, $T_c\sim$7 K and higher temperature charge density wave (CDW) orders. Here we report electrical transport and X-ray diffraction…
View article: Use of Frit‐Disc Crucible Sets to Make Solution Growth More Quantitative and Versatile
Use of Frit‐Disc Crucible Sets to Make Solution Growth More Quantitative and Versatile Open
The recent availability of step‐edge, frit‐disc crucible sets (generally sold as Canfield Crucible Sets or CCS) has led to multiple innovations associated with the group's use of solution growth. The use of CCS allows for the clean separat…
View article: Use of frit-disc crucible sets to make solution growth more quantitative and versatile
Use of frit-disc crucible sets to make solution growth more quantitative and versatile Open
The recent availability of step-edge, frit-disc crucible sets (generally sold as Canfield Crucible Sets or CCS) has led to multiple innovations associated with our group's use of solution growth. Use of CCS allows for the clean separation …
View article: Design and predict tetragonal van der Waals layered quantum materials of MPd5I2 (M=Ga, In and 3d transition metals)
Design and predict tetragonal van der Waals layered quantum materials of MPd5I2 (M=Ga, In and 3d transition metals) Open
Quantum materials with stacked van der Waals (vdW) layers hosting non-trivial band structure topology and magnetism have shown many interesting properties. Using high throughput density functional theory calculations, we design and predict…
View article: Tuning the structure and superconductivity of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>SrNi</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">P</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math> by Rh substitution
Tuning the structure and superconductivity of by Rh substitution Open
The compound SrNi2P2 is unique among the ThCr2Si2 class since it exhibits a temperature-induced transition upon cooling from an uncollapsed tetragonal (ucT) state to a one-third-collapsed ortho…
View article: Tuning the structure and superconductivity of SrNi$_2$P$_2$ by Rh substitution
Tuning the structure and superconductivity of SrNi$_2$P$_2$ by Rh substitution Open
SrNi$_2$P$_2$ is unique among the ThCr$_2$Si$_2$ class since it exhibits a temperature induced transition upon cooling from an uncollapsed tetragonal (ucT) state to a one-third-collapsed orthorhombic (tcO) state where one out of every thre…
View article: Nature of quantum criticality in the Ising ferromagnet TbV$_6$Sn$_6$
Nature of quantum criticality in the Ising ferromagnet TbV$_6$Sn$_6$ Open
TbV$_6$Sn$_6$ is a topological metal where ferromagnetic Tb ions with strong uniaxial magnetic anisotropy interact with V kagome layers. Inelastic neutron scattering (INS) measurements show that the Tb ions adopt an Ising doublet ground st…
View article: Design and Predict Tetragonal van der Waals Layered Quantum Materials of MPd5I2 (M=Ga, In and 3d Transition Metals)
Design and Predict Tetragonal van der Waals Layered Quantum Materials of MPd5I2 (M=Ga, In and 3d Transition Metals) Open
Quantum materials with stacking van der Waals (vdW) layers that can host non-trivial band structure topology and magnetism have shown many interesting properties. Here using high-throughput density functional theory calculations, we design…
View article: Effect of Ni substitution on the fragile magnetic system <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>La</mml:mi><mml:mn>5</mml:mn></mml:msub><mml:msub><mml:mi>Co</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>Ge</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:math>
Effect of Ni substitution on the fragile magnetic system Open
La5Co2Ge3 is an itinerant ferromagnet with a Curie temperature TC of ~3.8K and a remarkably small saturated moment of 0.1µB/Co. Here we present the growth and characterization of sin…
View article: Design and Predict Tetragonal van der Waals Layered Quantum Materials of MPd$_5$I$_2$ (M=Ga, In and 3$d$ Transition Metals)
Design and Predict Tetragonal van der Waals Layered Quantum Materials of MPd$_5$I$_2$ (M=Ga, In and 3$d$ Transition Metals) Open
Quantum materials with stacked van der Waals (vdW) layers hosting non-trivial band structure topology and magnetism have shown many interesting properties. Using high throughput density functional theory calculations, we design and predict…
View article: <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>La</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:msub><mml:mi>Co</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:mi>X</mml:mi></mml:mrow></mml:math> <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mo>(</mml:mo><mml:mi>X</mml:mi><mml:mo>=</mml:mo><mml:mi>Pb</mml:mi><mml:mo>,</mml:mo><mml:mo> </mml:mo><mml:mi>Bi</mml:mi><mml:mo>,</mml:mo><mml:mo> </mml:mo><mml:mi>Sb</mml:mi><mml:mo>)</mml:mo></mml:math>: A demonstration of antagonistic pairs as a route to quasi-low-dimensional ternary compounds
: A demonstration of antagonistic pairs as a route to quasi-low-dimensional ternary compounds Open
We outline how pairs of strongly immiscible elements, referred to here as antagonistic pairs, can be used to synthesize ternary compounds with low or quasi-reduced-dimensional motifs intrinsically built into their crystal structures. By id…
View article: Effect of Ni substitution on the fragile magnetic system ${\text{La}_{5}\text{Co}_{2}\text {Ge}_{3}}$
Effect of Ni substitution on the fragile magnetic system ${\text{La}_{5}\text{Co}_{2}\text {Ge}_{3}}$ Open
$\text{La}_{5}\text{Co}_{2}\text{Ge}_{3}$ is an itinerant ferromagnet with a Curie temperature, $T_C$, of $\sim$ 3.8 K and a remarkably small saturated moment of 0.1 $μ_{B}/\text{Co}$. Here we present the growth and characterization of sin…
View article: New insight into tuning magnetic phases of RMn6Sn6 kagome metals
New insight into tuning magnetic phases of RMn6Sn6 kagome metals Open
View article: La$_4$Co$_4$X (X = Pb, Bi, Sb): a demonstration of antagonistic pairs as a route to quasi-low dimensional ternary compounds
La$_4$Co$_4$X (X = Pb, Bi, Sb): a demonstration of antagonistic pairs as a route to quasi-low dimensional ternary compounds Open
We outline how pairs of strongly immiscible elements, referred to here as antagonistic pairs, can be used to synthesize ternary compounds with quasi-reduced dimensional motifs. By identifying third elements that are compatible with a given…
View article: Chiral and flat-band magnetic quasiparticles in ferromagnetic and metallic kagome layers
Chiral and flat-band magnetic quasiparticles in ferromagnetic and metallic kagome layers Open
View article: Strong enhancement of magnetic ordering temperature and structural/valence transitions in EuPd <sub>3</sub> S <sub>4</sub> under high pressure
Strong enhancement of magnetic ordering temperature and structural/valence transitions in EuPd <sub>3</sub> S <sub>4</sub> under high pressure Open
We present a comprehensive study of the inhomogeneous mixed-valence compound, EuPd 3 S 4 , by electrical transport, X-ray diffraction, time-domain 151 Eu synchrotron Mössbauer spectroscopy, and X-ray absorption spectroscopy measurements un…
View article: Strong Anharmonicity at the Origin of Anomalous Thermal Conductivity in Double Perovskite Cs<sub>2</sub>NaYbCl<sub>6</sub>
Strong Anharmonicity at the Origin of Anomalous Thermal Conductivity in Double Perovskite Cs<sub>2</sub>NaYbCl<sub>6</sub> Open
Anomalous thermal transport of Cs 2 NaYbCl 6 double‐halide perovskite above room temperature is reported and rationalized. Calculations of phonon dispersion relations and scattering rates up to the fourth order in lattice anharmonicity hav…
View article: Vacancy-tuned magnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>LaMn</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:msub><mml:mi>Sb</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>
Vacancy-tuned magnetism in Open
The layered AMP2 (A = alkali-earth or rare-earth atom, M = transition metal, P = Sb, Bi) compounds are widely studied for their rich magnetism and electronic structure topology. We provide a detailed characterization of the magn…
View article: Vacancy Tuned Magnetism in LaMn$_x$Sb$_2$
Vacancy Tuned Magnetism in LaMn$_x$Sb$_2$ Open
The layered ATMPn$_2$ (A = alkali earth or rare earth atom, TM = transition metal, Pn = Sb, Bi) compounds are widely studied for their rich magnetism and electronic structure topology. Here, we characterize the physical properties of LaMn$…
View article: New insight into tuning magnetic phases of $R$Mn$_6$Sn$_6$ kagome metals
New insight into tuning magnetic phases of $R$Mn$_6$Sn$_6$ kagome metals Open
Predicting magnetic ordering in kagome compounds offers the possibility of harnessing topological or flat-band physical properties through tuning of the magnetism. Here, we examine the magnetic interactions and phases of ErMn$_6$Sn$_6$ whi…
View article: Orbital character of the spin-reorientation transition in TbMn6Sn6
Orbital character of the spin-reorientation transition in TbMn6Sn6 Open
View article: <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>Mn</mml:mi><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi>Pt</mml:mi><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mi>Pd</mml:mi><mml:mi>x</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow><mml:mn>5</mml:mn></mml:msub><mml:mi mathvariant="normal">P</mml:mi></mml:mrow></mml:math>: Isovalent tuning of Mn-sublattice magnetic order
: Isovalent tuning of Mn-sublattice magnetic order Open
Here, e report the growth and characterization of MnPd5P, a rare-earth-free ferromagnet, with TC ≈ 295 K and planar anisotropy, and conduct a substitutional study with its antiferromagnetic analogue MnPt5P.…
View article: Single Crystal Growth of Synthetic Sulfide- and Phosphide-Based Minerals for Physical Measurements
Single Crystal Growth of Synthetic Sulfide- and Phosphide-Based Minerals for Physical Measurements Open
In this work, we review recent advances in the use of high-temperature solution growth that allow for the growth of single crystalline samples of synthetic minerals. We outline how low-melting binary or ternary solutions are attractive sol…
View article: Orbital character of the spin-reorientation transition in TbMn$_6$Sn$_6$
Orbital character of the spin-reorientation transition in TbMn$_6$Sn$_6$ Open
Ferromagnetic (FM) order in a two-dimensional kagome layer is predicted to generate a topological Chern insulator without an applied magnetic field. The Chern gap is largest when spin moments point perpendicular to the kagome layer, enabli…
View article: High-temperature ferromagnetism in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>Cr</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mo>+</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>Pt</mml:mi></mml:mrow><mml:mrow><mml:mn>5</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub><mml:mi mathvariant="normal">P</mml:mi></mml:math>
High-temperature ferromagnetism in Open
In this work, we present the growth and basic magnetic and transport properties of Cr1+xPt5-xP. We show that single crystals can readily be grown from a high-temperature solution created by adding dilute quantities of…
View article: Chiral and flat-band magnetic cluster excitations in a ferromagnetic kagome metal
Chiral and flat-band magnetic cluster excitations in a ferromagnetic kagome metal Open
TbMn6Sn6 is a metallic ferrimagnet that displays signatures of band topology arising from a combination of uniaxial ferromagnetism and spin-orbit coupling within its Mn kagome layers. Whereas the low energy magnetic excitations can be desc…
View article: Machine learning guided discovery of ternary compounds involving La and immiscible Co and Pb elements
Machine learning guided discovery of ternary compounds involving La and immiscible Co and Pb elements Open