Xiaoming Cao
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View article: Fe-(μ-O)-Zn dual-atom boosting C-C coupling for direct oxidation of methane to acetic acid using O2
Fe-(μ-O)-Zn dual-atom boosting C-C coupling for direct oxidation of methane to acetic acid using O2 Open
Direct oxidation of methane (DOM) into high-value C2+ products using molecular oxygen (O2) is essential for the sustainable production of clean energy and bulk chemicals, but is still challenging due to the difficult C-H activation and unc…
View article: Minimising the Demand for High-Fidelity Training Data towards Chemically Accurate Adsorption Energy Predictions
Minimising the Demand for High-Fidelity Training Data towards Chemically Accurate Adsorption Energy Predictions Open
Adsorption energy is a critical descriptor for high-throughput screening of heterogeneous catalysts and electrode materials. However, precise experimental data are scarce due to the complexity of experiments, while high-fidelity density fu…
View article: Ternary Schottky-p-n heterojunction strategy for enhancing photothermal dry reforming of methane
Ternary Schottky-p-n heterojunction strategy for enhancing photothermal dry reforming of methane Open
Breaking the trade-off between activity and stability in catalysts for dry reforming of methane has long remained a huge challenge. Here, we demonstrate a ternary Schottky-p-n (TSPN) heterojunction strategy based on Ni-NiO-Sr 2 Nb 2 O 7 (N…
View article: Enhanced Photocatalytic Hydrogen Evolution Activity Driven by the Synergy Between Surface Vacancies and Cocatalysts: Surface Reaction Matters
Enhanced Photocatalytic Hydrogen Evolution Activity Driven by the Synergy Between Surface Vacancies and Cocatalysts: Surface Reaction Matters Open
The incorporation of defects and cocatalysts is known to be effective in improving photocatalytic activity, yet their coupled contribution to the photocatalytic hydrogen evolution process has not been well‐explored. In this study, We demon…
View article: Adversarial Augmented Fields for Efficient Geophysical Analysis
Adversarial Augmented Fields for Efficient Geophysical Analysis Open
Accurate and comprehensive data remain critical for modeling and understanding Earth's complex systems, directly influencing weather forecasting, climate change predictions, and disaster management strategies. However, the scarcity of data…
View article: Study on the preparation of porous polyethylene glycol terephthalate film and the influencing factors of etching rate
Study on the preparation of porous polyethylene glycol terephthalate film and the influencing factors of etching rate Open
Porous polyethylene glycol terephthalate (PET) film is a kind of mesopore structure template with pore size ranging from nanometer to micrometer by chemical etching after irradiation of heavy ions. The etching rate is an important factor a…
View article: Effects of Cu, Sn, and Ti doping on the interfacial properties of Ag-based filler metal/WC: First-principles study and experimental characterization
Effects of Cu, Sn, and Ti doping on the interfacial properties of Ag-based filler metal/WC: First-principles study and experimental characterization Open
First-principles calculations were used to determine the formation energy, work of adhesion, and electronic structure of the interface of Ag-doped (Cu, Sn, and Ti)/WC, revealing the effect of doping atoms on the interfacial bonding behavio…
View article: Silver and Copper Dual Single Atoms Boosting Direct Oxidation of Methane to Methanol via Synergistic Catalysis
Silver and Copper Dual Single Atoms Boosting Direct Oxidation of Methane to Methanol via Synergistic Catalysis Open
Rationally constructing atom‐precise active sites is highly important to promote their catalytic performance but still challenging. Herein, this work designs and constructs ZSM‐5 supported Cu and Ag dual single atoms as a proof‐of‐concept …
View article: Effect of Temperature on the Morphology and Corrosion Resistance of Modified Boron Nitride Nanosheets Incorporated into Steel Phosphate Coating
Effect of Temperature on the Morphology and Corrosion Resistance of Modified Boron Nitride Nanosheets Incorporated into Steel Phosphate Coating Open
In this study, the impact of various temperatures (25 °C, 45 °C, and 55 °C) on q235 steel specimens was studied to analyze the influence on the morphology and corrosion resistance of modified boron nitride nanosheets incorporated into the …
View article: Preparation and Modification of Polydopamine Boron Nitride—Titanium Dioxide Nanohybrid Particles Incorporated into Zinc Phosphating Bath to Enhance Corrosion Performance of Zinc Phosphate-Silane Coated Q235 Steel
Preparation and Modification of Polydopamine Boron Nitride—Titanium Dioxide Nanohybrid Particles Incorporated into Zinc Phosphating Bath to Enhance Corrosion Performance of Zinc Phosphate-Silane Coated Q235 Steel Open
In this work, PDA@BN-TiO2 nanohybrid particles were incorporated chemically into a zinc-phosphating solution to form a robust, low-temperature phosphate-silane coating on Q235 steel specimens. The morphology and surface modification of the…
View article: Investigation of coordinated behavior of deformation at the interface of Cu–Al laminated composite
Investigation of coordinated behavior of deformation at the interface of Cu–Al laminated composite Open
To understand the differences between the microstructure and stress states owing to uncoordinated deformation in different regions of a Cu–Al contact interface, the normal stress distribution at the contact interface of the Cu–Al composite…
View article: Advantages and Limitations of Hydrogen Peroxide for Direct Oxidation of Methane to Methanol at Mono-Copper Active Sites in Cu-Exchanged Zeolites
Advantages and Limitations of Hydrogen Peroxide for Direct Oxidation of Methane to Methanol at Mono-Copper Active Sites in Cu-Exchanged Zeolites Open
The performance of the direct oxidation of methane to methanol (DMTM) is significantly influenced by the oxidant. It is still incredibly challenging to realize one-pot DMTM using dioxygen. So far, hydrogen peroxide is still the most freque…
View article: Data from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma
Data from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma Open
Purpose: Gastric adenocarcinoma is the third most common cause of cancer mortality worldwide. Accurate and affordable noninvasive detection methods have potential value for screening and surveillance. Herein, we identify novel methylated D…
View article: Supplemental Figure 1 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Figure 1 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Figure 1: The average level of all MDMs assayed from DNA extracted from primary and metastatic CRC tissues was not significantly different in Primary and Metastatic Tissue MDM Concordance Study. (A) Average level of all MDMs i…
View article: Supplemental Table 3 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Table 3 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Table 3 Performance of MDMs in differentiating recurrent CRC from healthy controls in MDM Plasma CRC Surveillance Study. MDM: methylated DNA marker; CRC: colorectal cancer; AUC: area under the receiver operating characteristic…
View article: Supplemental Legends and Tables from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma
Supplemental Legends and Tables from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma Open
Supplemental Table 1: Discrimination for gastric adenocarcinoma (GAC) from normal gastric mucosa by the top 22 methylated DNA marker candidates in Discovery and Technical Validation Sets. Supplemental Table 2: Function of Genes Containing …
View article: Supplemental Figure 5 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Figure 5 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Figure 5: No difference in carcinoembryonic antigen (CEA) values in nanograms per milliliter (ng/mL) was seen in a comparison of available clinical serum versus experimental plasma samples from colorectal cancer patients with …
View article: Data from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Data from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Purpose:We aimed to assess the concordance of colorectal cancer–associated methylated DNA markers (MDM) in primary and metastatic colorectal cancer for feasibility in detection of distantly recurrent/metastatic colorectal cancer in plasma.…
View article: Supplemental Figure 3 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Figure 3 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Figure 3: The distribution of MDMs in MDM Plasma CRC Early Primary Detection Study (i.e., training data) and in MDM Plasma CRC Surveillance Study (i.e., Recurrence data). There are reference lines relative to the healthy contr…
View article: Supplemental Table 1 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Table 1 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Table 1 Baseline characteristics of patients in Primary and Metastatic Tissue MDM Concordance Study
View article: Supplemental Figure 4 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence
Supplemental Figure 4 from Novel Methylated DNA Markers in the Surveillance of Colorectal Cancer Recurrence Open
Supplemental Figure 4: Carcinoembryonic antigen (CEA) levels in nanograms per milliliter assayed from 10 microliters serum in the Early Detection experiment are 1.5 times higher than values assayed from 10 microliters of plasma in the Surv…
View article: Figure S1 from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma
Figure S1 from Detection of Gastric Cancer with Novel Methylated DNA Markers: Discovery, Tissue Validation, and Pilot Testing in Plasma Open
Supplemental Figure 1: Quantitative allele-specific real-time target and signal amplification (QuARTS) assay.