Xunheng Jiang
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View article: Sabatier‐Adjusted <i>d</i> ‐Band Centers of Scalable Asymmetric Iron Sites toward Dynamic Nonradical Network for Fast Mineralization with Low‐Amount Oxidant
Sabatier‐Adjusted <i>d</i> ‐Band Centers of Scalable Asymmetric Iron Sites toward Dynamic Nonradical Network for Fast Mineralization with Low‐Amount Oxidant Open
Nonradicals relying on peroxymonosulfate (PMS) activation face inherent kinetic and thermodynamic limitations in pollutant mineralization. This is overcome using asymmetric iron single‐atom catalysts (Fe‐SACs) with Sabatier‐adjusted d ‐ban…
View article: Sulfur Bridge Geometry Boosts Selective Fe<sup>IV</sup>═O Generation for Efficient Fenton‐Like Reactions
Sulfur Bridge Geometry Boosts Selective Fe<sup>IV</sup>═O Generation for Efficient Fenton‐Like Reactions Open
High‐valent iron–oxo species (Fe IV ═O) is a fascinating enzymatic agent with excellent anti‐interference abilities in various oxidation processes. However, selective and high‐yield production of Fe IV ═O remains challenging. Herein, Fe di…
View article: Precise coordination of high-loading Fe single atoms with sulfur boosts selective generation of nonradicals
Precise coordination of high-loading Fe single atoms with sulfur boosts selective generation of nonradicals Open
Nonradicals are effective in selectively degrading electron-rich organic contaminants, which unfortunately suffer from unsatisfactory yield and uncontrollable composition due to the competitive generation of radicals. Herein, we precisely …
View article: Tailoring microenvironments of single-atom catalysts with non-metal p-block elements for selective environmental processes
Tailoring microenvironments of single-atom catalysts with non-metal p-block elements for selective environmental processes Open
Single-atom catalysts (SACs) have emerged as promising materials for efficient environmental remediation due to their unique properties and high catalytic efficiency. The incorporation of non-metal p-block elements into the SACs framework …
View article: Universal Ligand-Assisted Supermolecular Strategy to Synthesize Single-Atom Catalysts for Solar-to-Ethanol Conversion
Universal Ligand-Assisted Supermolecular Strategy to Synthesize Single-Atom Catalysts for Solar-to-Ethanol Conversion Open
Single-atom catalysts (SACs) have attracted significant attention; however, their catalytic properties are not satisfactory due to the sparse and inhomogeneity of the single-atom sites. Herein, we report a novel ligand-assisted supermolecu…