Yanqing Lai
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View article: Magnesium enhances soil carbon sequestration by modulating carbon-cycling microorganisms under reduced fertilisation conditions
Magnesium enhances soil carbon sequestration by modulating carbon-cycling microorganisms under reduced fertilisation conditions Open
Soil organic carbon (SOC) depletion remains a central challenge for tea plantations under intensive fertilisation. We evaluated three fertilisation strategies including farmer fertilisation (FF), optimised fertilisation (OF), and optimised…
View article: Surface Nonbonding Oxygen State Regulation for Reversible Anionic Redox Chemistry in Li‐Rich Mn‐Based Layered Oxides
Surface Nonbonding Oxygen State Regulation for Reversible Anionic Redox Chemistry in Li‐Rich Mn‐Based Layered Oxides Open
Activated by the Li–O–Li configuration with nonbonding O 2p state (lO 2p ), anionic redox reaction (ARR) in Li‐rich layered oxides (LLOs) contributes to additional capacity but exhibits significant irreversibility, leading to severe surfac…
View article: Surface Nonbonding Oxygen State Regulation for Reversible Anionic Redox Chemistry in Li‐Rich Mn‐Based Layered Oxides
Surface Nonbonding Oxygen State Regulation for Reversible Anionic Redox Chemistry in Li‐Rich Mn‐Based Layered Oxides Open
Activated by the Li–O–Li configuration with nonbonding O 2p state (lO 2p ), anionic redox reaction (ARR) in Li‐rich layered oxides (LLOs) contributes to additional capacity but exhibits significant irreversibility, leading to severe surfac…
View article: Accelerated TLPD bonding of reliable IMCs micro joints using Cu–8Ni substrate under thermal gradient: Experiments and theoretical calculations
Accelerated TLPD bonding of reliable IMCs micro joints using Cu–8Ni substrate under thermal gradient: Experiments and theoretical calculations Open
With the rapid development of the third-generation semiconductor power device towards high density, high performance, miniaturization and high temperature resistance, it is now urgent to develop a transient liquid phase diffusion (TLPD) bo…
View article: Adaptive Network Slicing and LSTM‐Based Resource Allocation for Real‐Time Industrial Robot Control in 6G Networks
Adaptive Network Slicing and LSTM‐Based Resource Allocation for Real‐Time Industrial Robot Control in 6G Networks Open
The deployment of industrial robots in time‐critical applications demands ultra‐low latency and high reliability in communication systems. This study presents a novel delay optimisation framework for industrial robot control systems using …
View article: Configurational entropy-tailored NASICON cathode redox chemistry for capacity-dense and ultralong cyclability
Configurational entropy-tailored NASICON cathode redox chemistry for capacity-dense and ultralong cyclability Open
High-entropy engineering is applied to NASICON-type cathodes to overcome long-standing trade-offs between structural stability and electrochemical performance, enabling high capacity, exceptional rate capability, and long-term cycling dura…
View article: Electrolyte tailoring and interfacial engineering for safe and high-temperature lithium-ion batteries
Electrolyte tailoring and interfacial engineering for safe and high-temperature lithium-ion batteries Open
By replacing the inert, strongly positive electrostatic potential of TTE with the active, weakly positive electrostatic potential of MDFSA, thermally resistant interfacial films are formed, enhancing the battery's performance at high tempe…
View article: Recent Progress on Stability of Layered Double Hydroxide-Based Catalysts for Oxygen Evolution Reaction
Recent Progress on Stability of Layered Double Hydroxide-Based Catalysts for Oxygen Evolution Reaction Open
Water electrolysis is regarded as one of the most viable technologies for the generation of green hydrogen. Nevertheless, the anodic oxygen evolution reaction (OER) constitutes a substantial obstacle to the large-scale deployment of this t…
View article: Lignin‐derived hard carbon anode with a robust solid electrolyte interphase for boosted sodium storage performance
Lignin‐derived hard carbon anode with a robust solid electrolyte interphase for boosted sodium storage performance Open
Hard carbon is regarded as a promising anode candidate for sodium‐ion batteries due to its low cost, relatively low working voltage, and satisfactory specific capacity. However, it still remains a challenge to obtain a high‐performance har…
View article: Sodium compensation: a critical technology for transforming batteries from sodium-starved to sodium-rich systems
Sodium compensation: a critical technology for transforming batteries from sodium-starved to sodium-rich systems Open
This review highlights the significance, fundamental principle, and recent advances of sodium compensation technologies, and provides insights into future improvement.
View article: All‐In‐One Detection, Removal and Recovery of Hg<sup>2+</sup> in Industrial Wastewater with Plasmonic Schottky Heterostructures
All‐In‐One Detection, Removal and Recovery of Hg<sup>2+</sup> in Industrial Wastewater with Plasmonic Schottky Heterostructures Open
The effective governance of Hg 2+ in environmental wastewater is of profound significance to deal with the global pollution issues. However, the present methodologies usually only focused on a single function of either detection or removal…
View article: Local Electronic Structure Modulation Enables Fast‐Charging Capability for Li‐Rich Mn‐Based Oxides Cathodes With Reversible Anionic Redox Activity
Local Electronic Structure Modulation Enables Fast‐Charging Capability for Li‐Rich Mn‐Based Oxides Cathodes With Reversible Anionic Redox Activity Open
Anionic and cationic redox chemistries boost ultrahigh specific capacities of Li‐rich Mn‐based oxides cathodes (LRMO). However, irreversible oxygen evolution and sluggish kinetics result in continuous capacity decay and poor rate performan…
View article: Graphical Abstract: Angew. Chem. Int. Ed. 26/2023
Graphical Abstract: Angew. Chem. Int. Ed. 26/2023 Open
a nonequilibrium precipitation approach for the construction of a highly disordered crystal structure of layered double hydroxides as a model oxygen evolution catalyst.
View article: Stabilized Anionic Redox by Rational Structural Design from Surface to Bulk for Long‐Life Fast‐Charging Li‐Rich Oxide Cathodes
Stabilized Anionic Redox by Rational Structural Design from Surface to Bulk for Long‐Life Fast‐Charging Li‐Rich Oxide Cathodes Open
On account of high capacity and high voltage resulting from anionic redox, Li‐rich layered oxides (LLOs) have become the most promising cathode candidate for the next‐generation high‐energy‐density lithium‐ion batteries (LIBs). Unfortunate…
View article: High‐Entropy Doping Boosts Ion/Electronic Transport of Na<sub>4</sub>Fe<sub>3</sub>(PO<sub>4</sub>)<sub>2</sub>(P<sub>2</sub>O<sub>7</sub>)/C Cathode for Superior Performance Sodium‐Ion Batteries
High‐Entropy Doping Boosts Ion/Electronic Transport of Na<sub>4</sub>Fe<sub>3</sub>(PO<sub>4</sub>)<sub>2</sub>(P<sub>2</sub>O<sub>7</sub>)/C Cathode for Superior Performance Sodium‐Ion Batteries Open
Fe‐based mixed phosphate cathodes for Na‐ion batteries usually possess weak rate capacity and cycle stability challenges resulting from sluggish diffusion kinetics and poor conductivity under the relatively low preparation temperature. Her…
View article: Effect of electric field on leaching valuable metals from spent lithium-ion batteries
Effect of electric field on leaching valuable metals from spent lithium-ion batteries Open
An electric field enhanced leaching process was proposed to improve the leaching efficiency in the process of extracting Li, Ni, Co and Mn from waste lithium ion batteries. The leaching process was optimized and the leaching mechanism was …
View article: “Mn-locking” effect by anionic coordination manipulation stabilizing Mn-rich phosphate cathodes
“Mn-locking” effect by anionic coordination manipulation stabilizing Mn-rich phosphate cathodes Open
Our study introduced light-weight fluorine into Mn-rich cathode to trigger a “Mn-locking” effect: more robust Mn ligand framework, suppressed Mn dissolution, improved structural stability and enhanced electronic conductivity.
View article: Stabilization of Multicationic Redox Chemistry in Polyanionic Cathode by Increasing Entropy
Stabilization of Multicationic Redox Chemistry in Polyanionic Cathode by Increasing Entropy Open
Polyanionic compounds have large compositional flexibility, which creates a growing interest in exploring the property limits of electrode materials of rechargeable batteries. The realization of multisodium storage in the polyanionic elect…
View article: Rationally Designed Sodium Chromium Vanadium Phosphate Cathodes with Multi‐Electron Reaction for Fast‐Charging Sodium‐Ion Batteries
Rationally Designed Sodium Chromium Vanadium Phosphate Cathodes with Multi‐Electron Reaction for Fast‐Charging Sodium‐Ion Batteries Open
Sodium super‐ionic conductor (NASICON)‐structured phosphates are emerging as rising stars as cathodes for sodium‐ion batteries. However, they usually suffer from a relatively low capacity due to the limited activated redox couples and low …