Ya‐Qian Lan
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View article: CCDC 2495245: Experimental Crystal Structure Determination
CCDC 2495245: Experimental Crystal Structure Determination Open
An entry from the Cambridge Structural Database, the world’s repository for small molecule crystal structures. The entry contains experimental data from a crystal diffraction study. The deposited dataset for this entry is freely available …
View article: Covalent organic framework-based heterojunction photocatalysts
Covalent organic framework-based heterojunction photocatalysts Open
Photocatalysis, as a sustainable, green and low-cost technology that converts solar energy into chemical energy, holds great potential to address the issues of environmental pollution and energy shortages. However, the rapid charge recombi…
View article: Covalent Organic Framework Hollow Rectangular Prism Enables Interfacial Binding of Li <sub>2</sub> S Cathode for High‐Performance Lithium‐Ion Sulfur Battery
Covalent Organic Framework Hollow Rectangular Prism Enables Interfacial Binding of Li <sub>2</sub> S Cathode for High‐Performance Lithium‐Ion Sulfur Battery Open
Since its initial discovery by Dahn et al. in 2002, Li 2 S has emerged as a highly promising cathode material, circumventing the employment of Li metal in battery construction. However, its practical application has been significantly cons…
View article: Correction to: Facile structuring of crystalline porous framework beads for deep purification of nuclear wastewater
Correction to: Facile structuring of crystalline porous framework beads for deep purification of nuclear wastewater Open
[This corrects the article DOI: 10.1093/nsr/nwaf080.].
View article: Steering Yolk–Shell Nanostructures of 1D Unit‐Based Covalent Organic Frameworks as Binder Modulators
Steering Yolk–Shell Nanostructures of 1D Unit‐Based Covalent Organic Frameworks as Binder Modulators Open
Induced by their weak chain interactions, 1D unit‐based covalent organic frameworks (1D COFs) are favorable in molecular assembly, yet their exploration in morphology engineering and related energy storage applications are still rare. Here…
View article: Plasmonic Ion Diode Membrane (PIDM) for Enhanced Nanofluidic Ion Transport
Plasmonic Ion Diode Membrane (PIDM) for Enhanced Nanofluidic Ion Transport Open
Efficient applications of nanofluidic devices are often limited by the insufficient ion permselectivity and inherent ion concentration polarization (ICP) phenomenon. In this work, a bio‐inspired plasmonic ion diode membrane (PIDM) was desi…
View article: Interweaved Nanofiber Anode Coating Based on Covalent Organic Frameworks for High‐Performance Lithium‐Metal Batteries
Interweaved Nanofiber Anode Coating Based on Covalent Organic Frameworks for High‐Performance Lithium‐Metal Batteries Open
High‐rate lithium‐metal batteries call for unique interfacial structures of anode with interfacial compatibility, facilitated lithium insertion/extraction and dendrite suppression properties to meet the growing high‐rate demand. Here, we d…
View article: Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity
Charge‐Transport Divergence in Ultrastable Heterometal‐Oxo Clusters Exerting Significant Effect on Photoreactivity Open
The transfer path of photogenerated charges greatly affects the final photocatalytic performance, but this important fact has not been clearly demonstrated experimentally. Here, we construct an ultrastable crystalline catalytic system incl…
View article: Engineering Covalent Organic Frameworks for Photocatalytic Overall Water Vapor Splitting
Engineering Covalent Organic Frameworks for Photocatalytic Overall Water Vapor Splitting Open
Photocatalytic overall water vapor splitting (OWVS) into H 2 and O 2 not only owns the potential of avoiding the backward reaction of O 2 reduction reaction reforming H 2 O, but also realizes H 2 production without available liquid water. …
View article: Engineering Covalent Organic Frameworks for Photocatalytic Overall Water Vapor Splitting
Engineering Covalent Organic Frameworks for Photocatalytic Overall Water Vapor Splitting Open
Photocatalytic overall water vapor splitting (OWVS) into H 2 and O 2 not only owns the potential of avoiding the backward reaction of O 2 reduction reaction reforming H 2 O, but also realizes H 2 production without available liquid water. …
View article: In situ Doping Coupling With Vacancy Regulation Induced Strong Metal‐Support Interaction in Ni/CaTiO<sub>3</sub> to Boost Supercharged Photothermal CO<sub>2</sub> Methanation
In situ Doping Coupling With Vacancy Regulation Induced Strong Metal‐Support Interaction in Ni/CaTiO<sub>3</sub> to Boost Supercharged Photothermal CO<sub>2</sub> Methanation Open
The “Solar Sabatier” reaction has emerged as a promising sustainable method for the CO 2 hydrogenation. The development of advanced metal‐support catalysts based on Strong Metal‐Support Interaction (SMSI) offers significant advantages in t…
View article: Facile structuring of crystalline porous framework beads for deep purification of nuclear wastewater
Facile structuring of crystalline porous framework beads for deep purification of nuclear wastewater Open
Traces of radionuclide residuals in ground water, with combined radiotoxicity and chemotoxicity, poses a tremendous threat to human health and the environment. Crystalline porous frameworks (CPFs), including metal-organic frameworks (MOFs)…
View article: 3D N-heterocyclic covalent organic frameworks for urea photosynthesis from NH3 and CO2
3D N-heterocyclic covalent organic frameworks for urea photosynthesis from NH3 and CO2 Open
Artificial photosynthesis of urea from NH 3 and CO 2 seems to remain still essentially unexplored. Herein, three isomorphic three-dimensional covalent organic frameworks with twofold interpenetrated ffc topology are functionalized by benze…
View article: Hydrogen‐Localization Transfer Regulation in 3D COFs Enhances Photocatalytic Acetylene Semi‐Hydrogenation to Ethylene
Hydrogen‐Localization Transfer Regulation in 3D COFs Enhances Photocatalytic Acetylene Semi‐Hydrogenation to Ethylene Open
In this work, a series of new crystalline three‐dimensional covalent organic frameworks (3D COFs) based on [8+4] construction was designed and successfully realized efficient photocatalytic acetylene (C 2 H 2 ) hydrogenation to ethylene (C…
View article: Hydrogen‐Localization Transfer Regulation in 3D COFs Enhances Photocatalytic Acetylene Semi‐Hydrogenation to Ethylene
Hydrogen‐Localization Transfer Regulation in 3D COFs Enhances Photocatalytic Acetylene Semi‐Hydrogenation to Ethylene Open
In this work, a series of new crystalline three‐dimensional covalent organic frameworks (3D COFs) based on [8+4] construction was designed and successfully realized efficient photocatalytic acetylene (C 2 H 2 ) hydrogenation to ethylene (C…
View article: Convergence on the Proton Drip-Line in Thulium
Convergence on the Proton Drip-Line in Thulium Open
Direct observation of proton emission for very small Q-values is often unfeasible due to the long partial half-lives of the proton emission channel associated with tunneling through the Coulomb barrier. Therefore, proton emitters with very…
View article: Bismuth‐Based Metal‐Organic Frameworks for Water Vapor Capture and Energy Storage
Bismuth‐Based Metal‐Organic Frameworks for Water Vapor Capture and Energy Storage Open
Transforming water vapor into electricity is a critical method for advancing renewable energy supply and alleviating the global energy crisis. However, conventional materials typically struggle to achieve a balance between energy storage a…
View article: Growing large single crystals of two- or three-dimensional covalent organic polymers through unconventional Te-O-P linkages
Growing large single crystals of two- or three-dimensional covalent organic polymers through unconventional Te-O-P linkages Open
Understanding precise structures of two-/three- dimensional (2D/3D) covalent organic polymers (COPs) through single-crystal X-ray diffraction (SCXRD) analysis is important. However, how to grow high-quality single crystals for 2D/3D COPs i…
View article: Atomically Precise Metal–Metal Oxide Interface in Polyoxometalate‐Noble Metal Hybrid Clusters
Atomically Precise Metal–Metal Oxide Interface in Polyoxometalate‐Noble Metal Hybrid Clusters Open
Metal‐metal oxide hybrid materials, typically composed of metal nanoparticles anchored on metal oxides matrix, are devoted enormous attentions as famous heterogeneous catalysts. The interactions between noble metals and metal oxides as wel…
View article: Dual Metallosalen‐Based Covalent Organic Frameworks for Artificial Photosynthetic Diluted CO<sub>2</sub> Reduction
Dual Metallosalen‐Based Covalent Organic Frameworks for Artificial Photosynthetic Diluted CO<sub>2</sub> Reduction Open
Directly converting CO 2 in flue gas using artificial photosynthetic technology represents a promising green approach for CO 2 resource utilization. However, it remains a great challenge to achieve efficient reduction of CO 2 from flue gas…
View article: Solid‐Liquid‐Gas Three‐Phase Indirect Electrolysis Enabled by Affinity Auxiliary Imparted Covalent Organic Frameworks
Solid‐Liquid‐Gas Three‐Phase Indirect Electrolysis Enabled by Affinity Auxiliary Imparted Covalent Organic Frameworks Open
The design of efficient heterogeneous redox mediators with favorable affinity to substrate and electrolyte are much desired yet still challenging for the development of indirect electrolysis system. Herein, for the first time, we have deve…
View article: Advancing Single‐Particle Analysis in Synthetic Chemical Systems: A Forward‐Looking Discussion
Advancing Single‐Particle Analysis in Synthetic Chemical Systems: A Forward‐Looking Discussion Open
Single‐particle analysis (SPA) is a fundamental method of cryo‐electron microscopy developed to resolve the structures of biological macromolecules. This method has seen significant success in structural biology, yet its potential applicat…
View article: Dynamic Control of Asymmetric Charge Distribution for Electrocatalytic Urea Synthesis
Dynamic Control of Asymmetric Charge Distribution for Electrocatalytic Urea Synthesis Open
Constructing dual catalytic sites with charge density differences is an efficient way to promote urea electrosynthesis from parallel and CO 2 reduction yet still challenging in static system. Herein, a dynamic system is constructed by prec…
View article: In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production
In situ Construction of Single‐Atom Electronic Bridge on COF to Enhance Photocatalytic H<sub>2</sub> Production Open
Photocatalytic hydrogen production is one of the most valuable technologies in the future energy system. Here, we designed a metal‐covalent organic frameworks (MCOFs) with both small‐sized metal clusters and nitrogen‐rich ligands, named CO…