Yongfu Tang
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View article: Revealing interfacial failure mechanism of silicon based all solid state batteries via cryogenic electron microscopy
Revealing interfacial failure mechanism of silicon based all solid state batteries via cryogenic electron microscopy Open
Interfaces are the critical components of all-solid-state batteries, and it is generally believed that high interfacial impedance is the major culprits of battery failure. In this study, the interface impedance has been found not to be a m…
View article: Synthesis, Microstructural Evolution, and Wet Wear Performance of an Fe55-Based Coating Reinforced with CeO2 and TiN Particles Fabricated via Plasma Beam Spraying
Synthesis, Microstructural Evolution, and Wet Wear Performance of an Fe55-Based Coating Reinforced with CeO2 and TiN Particles Fabricated via Plasma Beam Spraying Open
Valve leakage mainly comes from worn sealing surfaces caused by abrasive particles. This study uses plasma beam spraying to create Fe55 alloy coatings with CeO2 and TiN added to improve microstructure and wear resistance. Five coatings wer…
View article: Mechanically and chemically robust ultrahigh-Ni cathodes enabled by localized cation disorder design
Mechanically and chemically robust ultrahigh-Ni cathodes enabled by localized cation disorder design Open
View article: Mechanically and Chemically Co‐Robust Ni‐Rich Cathodes with Ultrahigh Capacity and Prolonged Cycle Life
Mechanically and Chemically Co‐Robust Ni‐Rich Cathodes with Ultrahigh Capacity and Prolonged Cycle Life Open
Ni‐rich layered oxide (NRLO) materials are considered highly promising cathode for lithium‐ion batteries. However, their practical application is limited by capacity loss and interface instability caused by chemical and mechanical failure …
View article: Electrolyte Reconfiguration by Cation/Anion Cross‐coordination for Highly Reversible and Facile Sodium Storage
Electrolyte Reconfiguration by Cation/Anion Cross‐coordination for Highly Reversible and Facile Sodium Storage Open
Hard carbon (HC) materials are promising anodes for sodium‐ion batteries (SIBs) owing to low cost, high specific capacity and low working potential. However, the poor compatibility of the electrolyte with HC leads to low initial coulombic …
View article: Mitigating the Kinetic Hysteresis of Co‐Free Ni‐Rich Cathodes via Gradient Penetration of Nonmagnetic Silicon
Mitigating the Kinetic Hysteresis of Co‐Free Ni‐Rich Cathodes via Gradient Penetration of Nonmagnetic Silicon Open
Co‐free Ni‐rich layered oxides are considered a promising cathode material for next‐generation Li‐ion batteries due to their cost‐effectiveness and high capacity. However, they still suffer from the practical challenges of low discharge ca…
View article: Enriching Nano‐Heterointerfaces in Proton Conducting TiO <sub>2</sub> ‐SrTiO <sub>3</sub> @TiO <sub>2</sub> Yolk–Shell Electrolyte for Low‐Temperature Solid Oxide Fuel Cells
Enriching Nano‐Heterointerfaces in Proton Conducting TiO <sub>2</sub> ‐SrTiO <sub>3</sub> @TiO <sub>2</sub> Yolk–Shell Electrolyte for Low‐Temperature Solid Oxide Fuel Cells Open
A challenging task in solid oxide fuel cells (SOFCs) is seeking for an alternative electrolyte, enabling high ionic conduction at relatively low operating temperatures, i.e., 300–600 °C. Proton‐conducting candidates, in particular, hold a …
View article: Steering lithium and potassium storage mechanism in covalent organic frameworks by incorporating transition metal single atoms
Steering lithium and potassium storage mechanism in covalent organic frameworks by incorporating transition metal single atoms Open
Organic electrodes mainly consisting of C, O, H, and N are promising candidates for advanced batteries. However, the sluggish ionic and electronic conductivity limit the full play of their high theoretical capacities. Here, we integrate th…
View article: Single-Atom Generation Inducing Electrochemical Transformation During Cycling in Transition Metal Sulfides for Na-Ion Batteries
Single-Atom Generation Inducing Electrochemical Transformation During Cycling in Transition Metal Sulfides for Na-Ion Batteries Open
View article: A review of all‐solid‐state lithium‐selenium batteries
A review of all‐solid‐state lithium‐selenium batteries Open
Rechargeable lithium‐selenium batteries (LSeBs) are promising candidates for next‐generation energy storage systems due to their exceptional theoretical volumetric energy density (3253 mAh cm −3 ). However, akin to lithium‐sulfur batteries…
View article: Deciphering the lithium ion conduction mechanism in solid-electrolyte-interphase
Deciphering the lithium ion conduction mechanism in solid-electrolyte-interphase Open
The solid electrolyte interphase (SEI) plays a critical role in determining the performance of lithium batteries, making it an area of increased scrutiny in research. Although the formation mechanism and structural model of SEI have been e…
View article: Prestoring Lithium into SnO2 Coated 3D Carbon Fiber Cloth Framework as Dendrite-Free Lithium Metal Anode
Prestoring Lithium into SnO2 Coated 3D Carbon Fiber Cloth Framework as Dendrite-Free Lithium Metal Anode Open
Three-dimensional (3D) conductive frameworks have been studied extensively in lithium (Li) metal anodes for their good electronic conductivities and superior structural integrity. In this work, we demonstrated a carbon fiber cloth (CFC) fr…
View article: Revealing the Origin of High-Thermal-Stability of Single-Crystal Ni-Rich Cathodes Toward Higher-Safety Batteries
Revealing the Origin of High-Thermal-Stability of Single-Crystal Ni-Rich Cathodes Toward Higher-Safety Batteries Open
View article: Morphodynamics of dendrite growth in alumina based all solid-state sodium metal batteries
Morphodynamics of dendrite growth in alumina based all solid-state sodium metal batteries Open
Atomic scale imaging revealed that the deposition/stripping of Na from the β′′-Al 2 O 3 solid electrolyte causes delamination cracks and the closure of the conduction planes.
View article: Tailoring lithium concentration in alloy anodes for long cycling and high areal capacity in sulfide-based all solid-state batteries
Tailoring lithium concentration in alloy anodes for long cycling and high areal capacity in sulfide-based all solid-state batteries Open
Lithium–indium (Li-In) alloys are important anode materials for sulfide-based all-solid-state batteries (ASSBs), but how different Li concentrations in the alloy anodes impact the electrochemical performance of ASSBs remains unexplored. Th…
View article: Grain Boundary Electronic Insulation for High‐Performance All‐Solid‐State Lithium Batteries
Grain Boundary Electronic Insulation for High‐Performance All‐Solid‐State Lithium Batteries Open
Sulfide electrolytes with high ionic conductivities are one of the most highly sought for all‐solid‐state lithium batteries (ASSLBs). However, the non‐negligible electronic conductivities of sulfide electrolytes (≈10 −8 S cm −1 ) lead to e…
View article: Reviving the rock-salt phases in Ni-rich layered cathodes by mechano-electrochemistry in all-solid-state batteries
Reviving the rock-salt phases in Ni-rich layered cathodes by mechano-electrochemistry in all-solid-state batteries Open
View article: 296 Targeting B-cell malignancies with anti-ROR1 CAR T-cell therapy
296 Targeting B-cell malignancies with anti-ROR1 CAR T-cell therapy Open
Background Anti-CD19 chimeric antigen receptor (CAR) T cell therapy has been shown to induce high complete response rates in the majority of B-cell lymphoma patients. However, over 50% of patients relapse within one year. A major cause of …
View article: Highly Efficient and Selective Carbon-Doped BN Photocatalyst Derived from a Homogeneous Precursor Reconfiguration
Highly Efficient and Selective Carbon-Doped BN Photocatalyst Derived from a Homogeneous Precursor Reconfiguration Open
The modification of inert boron nitride by carbon doping to make it an efficient photocatalyst has been considered as a promising strategy. Herein, a highly efficient porous BCN (p-BCN) photocatalyst was synthesized via precursor reconfigu…
View article: Enabling Long Cycle Life and High Rate Iron Difluoride Based Lithium Batteries by In Situ Cathode Surface Modification
Enabling Long Cycle Life and High Rate Iron Difluoride Based Lithium Batteries by In Situ Cathode Surface Modification Open
Metals fluorides (MFs) are potential conversion cathodes to replace commercial intercalation cathodes. However, the application of MFs is impeded by their poor electronic/ionic conductivity and severe decomposition of electrolyte. Here, a …
View article: Interlayer Doping of Pseudocapacitive Hydrated Vanadium Oxide Via Mn2+ for High-Performance Aqueous Zinc-Ion Battery
Interlayer Doping of Pseudocapacitive Hydrated Vanadium Oxide Via Mn2+ for High-Performance Aqueous Zinc-Ion Battery Open
View article: Metal-Organic Frameworks for Nanoconfinement of Chlorine in Rechargeable Lithium-Chlorine Batteries
Metal-Organic Frameworks for Nanoconfinement of Chlorine in Rechargeable Lithium-Chlorine Batteries Open
View article: Size-Dependent Chemomechanical Failure of Sulfide Solid Electrolyte Particles during Electrochemical Reaction with Lithium
Size-Dependent Chemomechanical Failure of Sulfide Solid Electrolyte Particles during Electrochemical Reaction with Lithium Open
The very high ionic conductivity of Li10GeP2S12 (LGPS) solid electrolyte (SE) makes it a promising candidate SE for solid-state batteries in electrical vehicles. However, chemomechanical failure, whose mech…
View article: <i>In situ</i> TEM visualization of single atom catalysis in solid-state Na–O<sub>2</sub> nanobatteries
<i>In situ</i> TEM visualization of single atom catalysis in solid-state Na–O<sub>2</sub> nanobatteries Open
In situ TEM observation and DFT calculation provide an atomic-scale understanding of the electrocatalysis mechanism of single-atom catalysts in an Na–O 2 nanobattery, where single-atomic Co sites facilitate the formation/decomposition of N…
View article: Degradation by Kinking in Layered Cathode Materials
Degradation by Kinking in Layered Cathode Materials Open
Layered cathode materials are commonly used in lithium and sodium ion batteries, but they are prone to degradation under electrochemical cycling during battery operation. Here we report a new type of degradation mechanism through the elect…
View article: Co<sub>3</sub>ZnC@NC Material Derived from ZIF-8 for Lithium-Ion Capacitors
Co<sub>3</sub>ZnC@NC Material Derived from ZIF-8 for Lithium-Ion Capacitors Open
Metal-organic framework (MOF)-derived carbon materials were widely reported as the anodes of lithium-ion capacitors (LICs). However, tunning the structure and electrochemical performance of the MOF-derived carbon materials is still challen…
View article: Novel K2Ti8O17 Anode via Na+/Al3+ Co-Intercalation Mechanism for Rechargeable Aqueous Al-Ion Battery with Superior Rate Capability
Novel K2Ti8O17 Anode via Na+/Al3+ Co-Intercalation Mechanism for Rechargeable Aqueous Al-Ion Battery with Superior Rate Capability Open
A promising aqueous aluminum ion battery (AIB) was assembled using a novel layered K2Ti8O17 anode against an activated carbon coated on a Ti mesh cathode in an AlCl3-based aqueous electrolyte. The intercalation/deintercalation mechanism en…
View article: In situ Observation of Li Deposition‐Induced Cracking in Garnet Solid Electrolytes
In situ Observation of Li Deposition‐Induced Cracking in Garnet Solid Electrolytes Open
Lithium (Li) penetration through solid electrolytes (SEs) induces short circuits in Li solid‐state batteries (SSBs), which is a critical issue that hinders the development of high energy density SSBs. While cracking in ceramic SEs has been…
View article: Lithium Deposition-Induced Fracture of Carbon Nanotubes and Its Implication to Solid-State Batteries
Lithium Deposition-Induced Fracture of Carbon Nanotubes and Its Implication to Solid-State Batteries Open
The increasing demand for safe and dense energy storage has shifted research focus from liquid electrolyte-based Li-ion batteries toward solid-state batteries (SSBs). However, the application of SSBs is impeded by uncontrollable Li dendrit…
View article: Layered LiCoO2–LiFeO2 Heterostructure Composite for Semiconductor-Based Fuel Cells
Layered LiCoO2–LiFeO2 Heterostructure Composite for Semiconductor-Based Fuel Cells Open
Enabling fast ionic transport at a low-temperature range (400–600 °C) is of great importance to promoting the development of solid oxide fuel cells (SOFCs). In this study, a layer-structured LiCoO2–LiFeO2 heterostructure composite is explo…