Zhengyu Bai
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View article: Direct single-atom/cluster interactions induce electron decoupling to promote the oxygen reduction reaction
Direct single-atom/cluster interactions induce electron decoupling to promote the oxygen reduction reaction Open
View article: [Ta6O19]8−-mediated interfacial OH− supply for efficient seawater electrolysis
[Ta6O19]8−-mediated interfacial OH− supply for efficient seawater electrolysis Open
Seawater electrolysis is promising yet challenging, as the rapid multi-step deprotonation process of oxygen evolution reaction (OER), along with the Ca2+, Mg2+ ions, would deplete the accessible OH- ions ne…
View article: Trifunctional endogenous mediator orchestrates efficient biocathodes via synergistic electron transfer and enzyme catalytic site modulation
Trifunctional endogenous mediator orchestrates efficient biocathodes via synergistic electron transfer and enzyme catalytic site modulation Open
View article: Graphene‐Based Phthalocyanine‐Assembled Synergistic Fe‐Co‐Ni Trimetallic Single‐Atomic Bifunctional Electrocatalysts by Rational Design for Boosting Oxygen Reduction/Evolution Reactions
Graphene‐Based Phthalocyanine‐Assembled Synergistic Fe‐Co‐Ni Trimetallic Single‐Atomic Bifunctional Electrocatalysts by Rational Design for Boosting Oxygen Reduction/Evolution Reactions Open
Development of high‐efficiency bifunctional oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) electrocatalysts is vital for the widespread application of zinc–air batteries (ZABs). However, it still remains a great challe…
View article: Cascade Hydrogen Peroxide Reduction Reaction Endows Cu‐Fe Dual‐Atom Catalyst with Durable Oxygen Reduction Performance
Cascade Hydrogen Peroxide Reduction Reaction Endows Cu‐Fe Dual‐Atom Catalyst with Durable Oxygen Reduction Performance Open
Durable problems caused by the attack from free radicals are considered as the Achilles’ heel in practical applications for oxygen reduction reaction (ORR) in acidic conditions. Herein, a ligand‐bridging strategy is proposed to design a Cu…
View article: Elucidation of Dynamic Cu0/Cu+/Cu2+ Interface as Superior Active Sites for Efficient Nitrate-to-Ammonia Conversion
Elucidation of Dynamic Cu0/Cu+/Cu2+ Interface as Superior Active Sites for Efficient Nitrate-to-Ammonia Conversion Open
View article: Octahedral Nanocrystals of Ptnicomocu Core/Shell High-Entropy Alloy with Lattice Strain and Low-Coordination Sites Enabling Co2 Pathway of Alcohol Oxidation Reaction
Octahedral Nanocrystals of Ptnicomocu Core/Shell High-Entropy Alloy with Lattice Strain and Low-Coordination Sites Enabling Co2 Pathway of Alcohol Oxidation Reaction Open
View article: Synergistic modulation of valence state and oxygen vacancy induced by surface reconstruction of the CeO<sub>2</sub>/CuO catalyst toward enhanced electrochemical CO<sub>2</sub> reduction
Synergistic modulation of valence state and oxygen vacancy induced by surface reconstruction of the CeO<sub>2</sub>/CuO catalyst toward enhanced electrochemical CO<sub>2</sub> reduction Open
Electrochemical CO 2 reduction reaction (CO 2 RR) offers a promising strategy for CO 2 conversion into value‐added C 2+ products and facilitates the storage of renewable resources under comparatively mild conditions, but still remains a ch…
View article: Conductive Zeolite Supported Indium–Tin Alloy Nanoclusters for Selective and Scalable Formic Acid Electrosynthesis
Conductive Zeolite Supported Indium–Tin Alloy Nanoclusters for Selective and Scalable Formic Acid Electrosynthesis Open
Upgrading excess CO 2 toward the electrosynthesis of formic acid is of significant research and commercial interest. However, simultaneously achieving high selectivity and industrially relevant current densities of CO 2 ‐to‐formate convers…
View article: Recent Progress in Sodium-Ion Batteries: Advanced Materials, Reaction Mechanisms and Energy Applications
Recent Progress in Sodium-Ion Batteries: Advanced Materials, Reaction Mechanisms and Energy Applications Open
For energy storage technologies, secondary batteries have the merits of environmental friendliness, long cyclic life, high energy conversion efficiency and so on, which are considered to be hopeful large-scale energy storage technologies. …
View article: Design and Algorithm Integration of High-Precision Adaptive Underwater Detection System Based on MEMS Vector Hydrophone
Design and Algorithm Integration of High-Precision Adaptive Underwater Detection System Based on MEMS Vector Hydrophone Open
Real-time DOA (direction of arrival) estimation of surface or underwater targets is of great significance to the research of marine environment and national security protection. When conducting real-time DOA estimation of underwater target…
View article: Building stabilized Cu<sub>0.17</sub>Mn<sub>0.03</sub>V<sub>2</sub>O<sub>5−□</sub>·2.16H<sub>2</sub>O cathode enables an outstanding room‐/low‐temperature aqueous Zn‐ion batteries
Building stabilized Cu<sub>0.17</sub>Mn<sub>0.03</sub>V<sub>2</sub>O<sub>5−□</sub>·2.16H<sub>2</sub>O cathode enables an outstanding room‐/low‐temperature aqueous Zn‐ion batteries Open
Vanadium oxide cathode materials with stable crystal structure and fast Zn 2+ storage capabilities are extremely important to achieving outstanding electrochemical performance in aqueous zinc‐ion batteries. In this work, a one‐step hydroth…
View article: 3d-Orbital Overlap Modulated D-Band Center of High-Entropy Oxyhydroxide for Efficient Oxygen Evolution Reaction
3d-Orbital Overlap Modulated D-Band Center of High-Entropy Oxyhydroxide for Efficient Oxygen Evolution Reaction Open
View article: Longevous Cycling of Rechargeable Zn‐Air Battery Enabled by “Raisin‐Bread” Cobalt Oxynitride/Porous Carbon Hybrid Electrocatalysts
Longevous Cycling of Rechargeable Zn‐Air Battery Enabled by “Raisin‐Bread” Cobalt Oxynitride/Porous Carbon Hybrid Electrocatalysts Open
Developing commercially viable electrocatalyst lies at the research hotspot of rechargeable Zn‐air batteries, but it is still challenging to meet the requirements of energy efficiency and durability in realistic applications. Strategic mat…
View article: Optimizing 3d spin polarization of CoOOH by in situ Mo doping for efficient oxygen evolution reaction
Optimizing 3d spin polarization of CoOOH by in situ Mo doping for efficient oxygen evolution reaction Open
Transition‐metal oxyhydroxides are attractive catalysts for oxygen evolution reactions (OERs). Further studies for developing transition‐metal oxyhydroxide catalysts and understanding their catalytic mechanisms will benefit their quick tra…
View article: Constructing Nanocaged Enzymes for Synergistic Catalysis of CO<sub>2</sub> Reduction
Constructing Nanocaged Enzymes for Synergistic Catalysis of CO<sub>2</sub> Reduction Open
Promoting the activity of biological enzymes under in vitro environment is a promising technique for bioelectrocatalytic reactions, such as the conversion of carbon dioxide (CO 2 ) into valuable chemicals, which is a promising strategy to …
View article: Sulfide-Based All-Solid-State Lithium–Sulfur Batteries: Challenges and Perspectives
Sulfide-Based All-Solid-State Lithium–Sulfur Batteries: Challenges and Perspectives Open
View article: In Situ Reconstructed Mo‐doped Amorphous FeOOH Boosts the Oxygen Evolution Reaction
In Situ Reconstructed Mo‐doped Amorphous FeOOH Boosts the Oxygen Evolution Reaction Open
Developing a fast and highly active oxygen evolution reaction (OER) catalyst to change energy kinetics technology is essential for making clean energy. Herein, we prepare three‐dimensional (3D) hollow Mo‐doped amorphous FeOOH (Mo‐FeOOH) ba…
View article: Machine-Learning-Guided Prediction of Cu-Based Electrocatalysts Towards Ethylene Production in Co2 Reduction
Machine-Learning-Guided Prediction of Cu-Based Electrocatalysts Towards Ethylene Production in Co2 Reduction Open
View article: Homogeneous Slate-Like Nitrogen-Doped Carbon/Sns Composites Constructed by In-Situ Carbonization and Vulcanization as High-Performance Anode Materials for Sodium-Ion Batteries
Homogeneous Slate-Like Nitrogen-Doped Carbon/Sns Composites Constructed by In-Situ Carbonization and Vulcanization as High-Performance Anode Materials for Sodium-Ion Batteries Open
View article: Lithiation‐Induced Defect Engineering to Promote Oxygen Evolution Reaction
Lithiation‐Induced Defect Engineering to Promote Oxygen Evolution Reaction Open
Exploring efficient electrocatalysts for oxygen evolution reaction (OER) is an urgent need to advance the development of sustainable energy conversion. Though defect engineering is considered an effective strategy to regulate catalyst acti…
View article: Partial deligandation activated ZIF-67 for efficient electrocatalytic oxygen reduction reaction
Partial deligandation activated ZIF-67 for efficient electrocatalytic oxygen reduction reaction Open
Removing the blocked molecular groups and fully exposing the intrinsic active sites of metal-organic frameworks (MOFs) could give full play to their advantages of multi-active sites and multi-channel mass transfer, which will benefit the e…
View article: Copper-Based Catalysts for Electrochemical Carbon Dioxide Reduction to Multicarbon Products
Copper-Based Catalysts for Electrochemical Carbon Dioxide Reduction to Multicarbon Products Open
Electrochemical conversion of carbon dioxide into fuel and chemicals with added value represents an appealing approach to reduce the greenhouse effect and realize a carbon-neutral cycle, which has great potential in mitigating global warmi…
View article: Strained Lattice Gold-Copper Alloy Nanoparticles for Efficient Carbon Dioxide Electroreduction
Strained Lattice Gold-Copper Alloy Nanoparticles for Efficient Carbon Dioxide Electroreduction Open
Electrocatalytic conversion of carbon dioxide (CO2) into specific renewable fuels is an attractive way to mitigate the greenhouse effect and solve the energy crisis. AunCu100-n/C alloy nanoparticles (AunCu100−n/C NPs) with tunable composit…
View article: Beads‐on‐string hierarchical structured electrocatalysts for efficient oxygen reduction reaction
Beads‐on‐string hierarchical structured electrocatalysts for efficient oxygen reduction reaction Open
Rational design of hierarchically structured electrocatalysts is particularly important for electrocatalytic oxygen reduction reaction (ORR). Here, ZIF‐67 crystals are stringed on core–shell Ag@C nanocables using a coordination‐modulated p…
View article: Red Blood Cells-Derived Iron Self–Doped 3D Porous Carbon Networks for Efficient Oxygen Reduction
Red Blood Cells-Derived Iron Self–Doped 3D Porous Carbon Networks for Efficient Oxygen Reduction Open
In addition to C, H and O, some biomass is also rich in mineral elements. The recovery and utilization of special mineral elements is of great significance to prepare functional materials and alleviate the current energy shortage. Herein, …
View article: Implementation of Structural and Surface Engineering Strategies to Copper Sulfide for Enhanced Sodium Ion Storage
Implementation of Structural and Surface Engineering Strategies to Copper Sulfide for Enhanced Sodium Ion Storage Open
View article: Three-Dimensionally Ordered Mesoporous Co3o4 Decorated with Mg as Bifunctional Oxygen Electrocatalysts for High-Performance Zinc-Air Batteries
Three-Dimensionally Ordered Mesoporous Co3o4 Decorated with Mg as Bifunctional Oxygen Electrocatalysts for High-Performance Zinc-Air Batteries Open
View article: 3d-Orbital Occupancy Regulated Ir-Co Atomic Pair Toward Superior Bifunctional Oxygen Electrocatalysis
3d-Orbital Occupancy Regulated Ir-Co Atomic Pair Toward Superior Bifunctional Oxygen Electrocatalysis Open
Atomically dispersed metal catalysts are hailed as the most promising catalyst category for oxygen electrocatalysis. However, the challenges in regulating electronic configuration and unveiling the mechanism on the atomic scale are hinderi…
View article: Mesocrystallizing Nanograins for Enhanced Li<sup>+</sup> Storage
Mesocrystallizing Nanograins for Enhanced Li<sup>+</sup> Storage Open
The morphology and crystallinity of electrode materials have a major effect on their charge carrier storage properties when applied in rechargeable batteries. While nanosizing electrode particles (with larger surface area) and maintaining …